Thesis (Masters Diploma (Technology)--Cape Technikon, Cape Town,1992 / This research project involved the design, development and manufacture of a krypton gas target system for the production of the radioisotope Rubidium-81 at the National Accelerator Centre (NAC). The newly designed system had to be linked to the existing production facilities, which set certain restraints and fIxed parameters to the design approach. The highl'ressure krypton-filled gas target was designed to link up to the existing transport system which is used for the transportation of all targets to and from the target bombardment station and· the hot-cells where processing takes place. Radiation resistant materials had to be selected for the target, as it would be exposed to high radiation doses during bombardment in the target bombardment station. Target cooling aspects also had to be taken into consideration due to the heat generated during bombardment. A cryopump system for transferring the krypton gas from a gas storage reservoir to the gas target and back during loading and unloading was developed. A further development was a system which would retrieve the formed radioisotopes in a water suspension after bombardment. This demanded the design of a set of spray nozzles which were mounted inside the gas target chamber, a suitable water circulating pump and ruters to trap the suspended radioisotopes. Due to the high radiation levels] which are, of course, dangerous to operating personnel, the whole system was constructed inside a hot-cell, and thus required the design of a fully remote control system together with gas monitoring and safety components. The processing system itself required many switching and monitoring opera.tions which ha.ve to be carried out accurately and sequentially and this further demanded making use of a microcomputer control system. Material strengths, manufacturing methods, performance and selection of the VarIOus components in the system were investigated, as well as the respective routine maintenance and repair aspects.

<p> The decay of 3.5 minute 89Kr to levels in 89Rb has been investigated with small and large volume Ge(Li) detectors used singly and in coincidence. A total of 160 gamma rays have been attributed to the nuclear process, 120 of which have been incorporated into a proposed decay scheme.</p> / Thesis / Master of Science (MSc)

<p> The relative cumulative yields of krypton and xenon isotopes from the thermal neutron fission of 237Np and Np238 and from the fast neutron fission of Np237 have been measured by means of a mass spectrometer. These are the first fission yield results for 238Np, and the first for 237Np at thermal neutron energies. The results are compared with those from other fissioning nuclides.</p> <p> Independent yields of the shielded nuclides 80Br, 82Br, 128I, and 130I from the thermal neutron fission of 235U, 233U, 239Pu, and 238Np have been determined by mass spectrometric analyses of the krypton and xenon β-decay products. The results are discussed in terms of conventional charge distribution theories, and also in terms of neutron emission effects.</p> / Thesis / Doctor of Philosophy (PhD)

The absolute abundances of fission-product xenon and krypton isotopes in six uranium minerals were determined mass spectrometrically using the isotope dilution technique. The fission products were resolved into a U spontaneous fission component, a U 235 neutron-induced fission component, and a U 238 neutron-induced fission component. The presence of U 238 of neutron-induced fission indicated that t he neutron energies in uranium minerals were higher than had been suspected. Internal consistency in the analysis was achieved only when the I 29 yield in u235 thermal neutron fission reported by Purkayastha and Martin was lowered by 20%. The number of U 238 spontaneous fissions was calculated from the lead age, U 238 content, and the U 238 pontaneous fission half life. A comparison of the number of fission products from U 238 spontaneous fission and the number of spontaneous fissions in each of the six minerals showed that five of the six minerals had lost large portions of their noble gases. A fractionation of krypton relative to xenon accompanied this loss. The results obtained for the sixth mineral indicated little or no loss of xenon and krypton. Absolute yields for U 238 spontaneous fission were therefore determined from an analysis of this mineral. / Thesis / Doctor of Philosophy (PhD)

A first-generation LaB6 heaterless hollow cathode with a flat-plate anode is experimentally investigated. The cathode is characterized using krypton as propellant at varying flow rates, discharge currents and cathode-anode distances. Voltage probes, used to make direct voltage measurements in the ignition circuit, are the only diagnostic tool used experimentally. A plasma model is used to infer plasma parameters in the cathode emitter region. The cathode characterization results are consistent with those obtained during previous investigations of 1 A-class LaB6 hollow cathode with krypton. A peak-to-peak anode voltage criterion is used to identify the discharge modes and the occurrence of mode transition. Fourier analysis of the keeper and anode voltage waveforms carried out to study the discharge mode behavior reveals resonant frequencies ranging from 40 to 150 kHz. Lastly, post-test visual observations of the cathode components show signs of emitter poisoning and keeper erosion. / Master of Science / Recent years have seen rapid growth in the development of both stand-alone satellites and satellite constellations. A critical component of these satellites is the on-board propulsion system, which is responsible for controlling their orientation with respect to the object of interest and keeping the spacecraft in the assigned orbit. Generally, electric propulsion systems are used for this purpose. These types of propulsion systems use electrical power to change the velocity of satellite, providing a small thrust for a long duration of time as compared to chemical propulsion systems. Certain types of electric thrusters utilize a hollow cathode device as an electron source to start-off and support the thruster operation. In this research, a non-conventional hollow cathode for low power applications is developed and tested. The main characteristic of the developed cathode is the heaterless configuration, which eliminates the heater module used in conventional cathodes to enable the cathode to reach its operational temperature. The absence of a heater reduces the complexity of the cathode and the electrical power system. The cathode utilizes an electron emitter material which is insensitive to impurities and air exposure. Additionally, unlike typical electric thrusters which use xenon as the fuel, this cathode uses krypton which is similar to xenon but is less expensive. The presented work includes an overview of electric propulsion and the hollow cathode operation, followed by a detailed discussion of the heaterless hollow cathode design, the experimental setup and the test results. Several noteworthy findings regarding cathode operation are included as well. This research shows that the non-conventional heaterless hollow cathode and its operation with krypton have the potential to improve the overall thruster performance by reducing the weight and the cost, thus contributing to an integral aspect of satellite on-board propulsion.

Thesis (M.S.)--Miami University, Dept. of Physics, 2008. / Title from first page of PDF document. Includes bibliographical references (p. 36-37).

Thesis (Ph.D.)--McMaster University, 2004. / Advisor: G. J. Schrobilgen. Includes bibliographical references (leaves 333-352). Also available online.

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Introduction Krypton-81m is a radioactive gas with a half-life of 13 s, and found to be useful in many applications in nuclear medicine, particularly for lung perfusion studies and ventilations. Due to high demands for 81mKr, we have developed an automated Krypton system to be installed in one of the Cyclotron’s beamlines at King Faisal Specialist Hospital and Research Centre (KFSH&RC) and to deliver large activity of the radioactive gas. Material and Methods The effective cross section of producing 81Rb is between 15 and 30 MeV [1]. Therefore, range and stopping power of the effective cross section were calculated with respect to gas density of 0.0185 g/cm3. This value is equivalent to gas density at 5.0 bars at room temperature. SRIM calculations resulted in a range of 589 mm. However, due to limitation in fabricating such long target chamber, the target length is chosen to be 250 mm. Attached to the end of target body is a special water circulating flange ‘back-pool’, its purpose is to absorb the rest of the energy and protons Bragg peak. The target body is made of Aluminum with the inner part being electroplated with nickel. The target body is of conical shape. The target body is electrically isolated from other parts to allow accurate beam current reading. Full access to the target loading/unloading steps is made through touch screen technology (FIG. 2) for user access. Additionally, the target control system is designed to be protected through chain of interlock steps. The production cycle of 81Rb is explained as follow. Target is evacuated to approximately 10−3 mbar before being filled with natKr at pressure of 5 bars. At the end of bombardment, recovery of natKr is done via cryogenic vessel. Finally, the radioactivity is washed with KCl and pushed to Hotcells through the nitrogen gas for chemistry processing. Irradiation time was approximately 30 min. Results and Conclusion Experimental results clearly showed a fairly good activity of 81mKr as shown in TABLE 1. In all experiments, the radionuclidic purity of 81mKr was above 99.59%. 79mKr and 79Kr were also measured with a percentage of, respectively, 0.34 and 0.07 %. Special attention has to be drawn to last experiment where the yield significantly in-creased, due to the period where the KCl left inside the target (10 min) before pushing the solution to the Hotcells