Hall probe magnetometry measurements have been used to investigate the magnetic state of various Pb microcrystals grown by electrodeposition, where careful control of deposition parameters has allowed the tuning of their architectures. The internal flux distribution when in the superconducting state is seen to be highly dependent on the size and geometry of the investigated samples. In nanowires single flux vortex states are seen to form, showing typical type II behaviour. As the diameter of the nanowires increases these vortex states are seen to bunch together, behaviour that begins to approach that of a type I superconductor. Measurements of Pb triangles with sloped sides show the formation of giant vortex states typical of type I behaviour. These results also highlight the importance of geometry on surface barriers and the corresponding effect these have on flux distribution. Investigation of an icosahedron shows how symmetry effects can determine the stability of different flux states. Experimental results are in good agreement with Ginzburg-Landau calculations.

The detailed observational analysis of three massive B- and O-type stars was carried out in this study in order to characterize their fundamental, magnetic, and variability properties. The bulk of the data acquired were obtained with the high-resolution ESPaDOnS spectropolarimeter at the Canada-France-Hawaii telescope, within the context of the Magnetism in Massive Stars (MiMeS) project. Two of these stars (HR5907 and HD57682) are newly detected magnetic stars, discovered from observations acquired as part of the broader survey component of the MiMeS program, while the last star, ω Ori, was previously reported as magnetic in the literature. The rotation periods of HR5907 and HD57682 were inferred from photometric, Hα emission and longitudinal field variations. A period of 0.508276 was inferred for HR5907, making this the shortest period, non-degenerate, magnetic massive star identified to date. Furthermore, ultraviolet and optical spectroscopy were combined to infer the fundamental properties of HR5907 and HD57682. Direct modelling of the Least-Squares Deconvolved line profiles and the longitudinal magnetic field measurements were used to infer the magnetic properties of HR5907, HD57682, and ω Ori. A detailed investigation of the newly obtained and archival polarimetric data of ω Ori revealed no convincing evidence for a magnetic field, despite evidence of variability in some emission quantities in this dataset, which had been previously attributed to a large-scale magnetic field. The strength and variability of the optical photospheric helium lines of HR5907 suggests that this star is He-rich, with a non-uniform distribution of its surface chemistry. Lastly, the emission variations in the hydrogen lines of HR5907 suggest this star hosts a highly-structured, rigidly-rotating, centrifugally supported magnetosphere. Similarly, line profile variations throughout the optical spectrum of HD57682 are attributed to emission variations caused by a rotationally-modulated, dynamical magnetosphere. As magnetism in massive stars is a relatively rare and poorly-studied phenomenon, these studies comprise the bulk of the detailed investigations of magnetic massive stars carried out to date. The results of these investigations are also discussed in the context of addressing the current outstanding issues related to magnetism in massive stars. / Thesis (Ph.D, Physics, Engineering Physics and Astronomy) -- Queen's University, 2012-09-28 17:22:35.115

Thesis (Ph. D.)--University of Texas at El Paso, 2008. / Title from title screen. Vita. CD-ROM. Includes bibliographical references. Also available online.

Thesis advisor: Brian B. Zhou / This thesis presents work in the context of multimodal magnetometry for two-dimensional (2d) materials. Research on van der Waals materials has been rapidly emerging and several imaging techniques have been developed in the past decades. Among the modern techniques, solid-state spins feature outstanding sensitivity and nano-scale spatial resolution. Yet their full capacity in sensing still has room for improvement, as the quantum nature of their properties haven't been fully utilized. My research involves developing state-of-the-art sensing techniques to add new `function modules' to the nitrogen-vacancy (NV) centers, with the goal of uncovering dynamical magnetic and electrical phenomena of 2d materials. In the first chapter I will briefly discuss the basic opto-spin properties of the NV center. One shall see why NV is preferred as a quantum sensing probe: the opto-spin property comes handy as one simply counts photons to manipulate and read out quantum states, and the stability and long quantum coherence time makes NV adaptive with various environments and engineering. In the second chapter I will discuss the experimental setup with the focus on the home-built confocal microscope, which equips our sensing technique with the pump-probe scanning ability of sub-um 2d resolution. In the third chapter I will discuss the developments of the sensing protocols, including the ac susceptometry and the opto-magnetization mapping, based on the lock-in method using the quantum dynamical decoupling sequences. In the fourth chapter I will describe the ac susceptibility measurements on thin CrBr3 flakes. The magnetization behaviors under kHz to MHz excitations reveal the domain morphology and domain wall mobility, providing insights to the exchange interaction of the chromium trihalides in the 2d limit. In the fifth chapter I will describe the pump-probe measurements on few-layer CrCl3 flakes. The mapping result demonstrates a photo-generated enhancement of the in-plane magnetization. Along with the time-resolved photoluminescence measurement, the results are indicative of a defect-assisted Auger recombination process of excitons. To conclude, the multimodal sensing techniques with NV developed in this thesis allow for more versatile experiments with sensitivity for low-dimensional systems. The developments bring up new perspectives on fundamental physics in atomically thin materials, providing new ideas for future technological applications such as spintronics and quantum memory. / Thesis (PhD) — Boston College, 2024. / Submitted to: Boston College. Graduate School of Arts and Sciences. / Discipline: Physics.

The magnetic and physical properties of oxide-free, ligand passivated, iron nanoparticles were studied using superconducting quantum interference device (SQUID) magnetometry and synchrotron based X-ray radiation. Particles used for this study ranged in diameter between 2 and 10 nm, which made it possible to distinguish between bulk and surface effects in the nanoparticles’ properties. Additionally, the effects of two different weakly interacting ligands (2,4-pentanedione and hexaethylene glycol monododecylether) on the nanoparticles’ behavior were studied. The results of this study were compared to theoretical predictions of magnetic transition metal behavior in both thin films and nanoparticles, as well as experimental results from measurements of transition metal clusters formed in an inert carrier gas and measured with a Stern-Gerlach magnet. Magnetometry revealed that the iron nanoparticles have a magnetocrystalline anisotropy an order of magnitude greater than bulk iron. At the same time, these particles exhibit a saturation mass magnetization up to 209 Am2/kg, which is only slightly lower than bulk iron. The structural properties of these particles were characterized using high energy X-ray diffraction analyzed using the atomic pair distribution function method (PDF). The PDF analysis indicates that the Fe particles have a distorted and expanded form of the bcc lattice, which could, at least in part, explain the magnetocrystalline anisotropy of these nanoparticles. X-ray absorption fine structure (XAFS) was used to study the surface properties of the iron nanoparticles and further characterize their structural properties. XAFS showed that oxidized species of iron exist at the nanoparticles’ surface and can be attributed to iron/ligand interactions. The percentage of oxidized species scales with the surface to volume ratio of the nanoparticles, and therefore appears limited to the nanoparticle surface. The layer of Fe(II) species present at the nanoparticles’ surface accounts for the reduction in saturation mass magnetization values (when compared to bulk iron) observed in these particles. XAFS analysis also provided further confirmation of the nanoparticles’ expanded crystalline lattice. / text

Thesis (M.A.)--Portland State University, 2002. / Computer-produced typeface. Includes bibliographical references (leaves 119-123).

Oriented archaeomagnetic samples were collected from 158 in situ features at 33 sites in the southwestern U.S. Seventy-three independently dated features were used for analysis of secular variation. A moving-window smoothing technique with outlier rejection was developed to objectively compute a virtual geomagnetic pole (VGP) path. Weighted Fisher statistics, accounting for errors in both dating and archaeomagnetic direction, were used to compute a mean VGP and standard error (A95) within each window of time. The VGP moves from 86°N, 83°E at A.D. 750 to 74°N, 192°E at A.D. 1075, and then to 85°N, 236°E at A.D. 1425. Secular variation of the VGP ranges from .00423-.350°/yr with a median of .0359°/yr. The A95s for the VGP curve range from 1.33-5.28°. Archaeomagnetic declinations and inclinations in Tucson range from 346-359°E and 47-60°. The close agreement with a similarly constructed VGP curve for Arkansas implies a small nondipole field in North America between A.D. 1150-1450. The VGP curve is significantly different from that of R. L. DuBois. Three case histories of archaeomagnetic dating suggest the validity of the new curve. The Thellier-Thellier paleointensity experiment was performed on 187 specimens from 77 potsherds. A significant magnetic fabric anisotropy, typically 30%, was found. Using an easy-plane model of magnetization, the anisotropy correction systematically increased the paleointensities by 5%. Paleointensities were interpreted for 127 samples from 54 sherds. All ceramics were independently dated and used along with other results to construct a virtual axial dipole moment (VADM) curve. A moving-window smoother using weighted statistics within each interval of time and incorporating outlier analysis was used. The Southwestern VADM at 300 B.C. is 14 x 10('22)Am('2), decreases to 8.6 x 10²²Am² at A.D. 800, and increases to 12.9 x 10²²Am² at A.D. 1500. Paleointensities from Hohokam ceramics compare favorably with paleointensities from other Southwestern ceramics, regardless of whether the long Hohokam chronology beginning at 300 B.C. or the short chronology beginning at A.D. 500 are used. There is also reasonable agreement between the Southwest and Mesoamerican VADM records.

No description available.

The existence of the matter in the universe is still an unsolved puzzle. After the Big Bang, both matter and antimatter should have been created in equal amounts, and subsequently annihilated. The leading theories to explain the existence of matter require an imbalance in the production of matter and antimatter in the early universe. This in turn requires CP violation, an asymmetry of the laws of physics between matter and antimatter. cryoEDM is designed to explore the total amount of CP violation and resolve this issue. cryoEDM is a next-generation neutron electric dipole moment search in a commissioning phase of development at the Institut Laue-Langevin, Grenoble. A critical requirement of EDM searches is knowledge of the magnetic environment. This work is concerned with the development, implementation, and performance of the currently operating magnetometry system based on SQUID magnetometers. An analysis scheme to provide magnetometry data over the volume occupied by the neutrons, from measurements using the available magnetometers, is developed. An updated method to calibrate the magnetometers using internal sources of magnetic fields is presented, and found to give good agreement with independent measurements. A new method of calibration using the neutrons as a reference is discussed, and tests on an example arrangement are shown to be promising. Algorithms for detecting and correcting for hardware induced artefacts in the data are produced, and demonstrated to reconstruct the field with good agreement in all but the noisiest environments. A software framework is developed to combine these into a real-time analysis that provides feedback and diagnostics to the experiment. Using this new system the resolution of the magnetometers installed in cryoEDM is found to be limited by the environmental noise, and would give a false EDM signal that is greater than the statistical uncertainty in neutron counting. However, the resolution has been somewhat artificially limited to reduce the susceptibility to the RF interference present. This still allows the magnetometry to act as a useful diagnostic tool on any issues in the current magnetic environment, even if in a sub-optimal configuration. For example, investigation of the magnetic shielding of the experiment finds a reduction in the shielding relative to the design, a situation which is being addressed with the design of additional shielding. Once this shielding is installed the resolution of the magnetometers will improve as well as the slew rate of the SQUIDs, which is found to be lower than the $47,mu extup{Ts}^{-1}$ required to measure AC fields applied during a measurement. The current system can also determine sources of magnetic perturbations created within the experiment, which will require addressing before a full EDM run can be performed. For example, cryogenic effects are observed to occur approximately hourly causing large shifts in the magnetic field. Also operation of valves controlling the flow of neutrons around the experiment are found to produce both AC magnetic fields from the driving motors, and shifts in the field from their movement. Situations which can be resolved by reexamination of installation and operational procedures.

Among several hundred impurities and defects that can occur in diamond, the nitrogenvacancy (NV) center is one of the most interesting for quantum technologies at room temperature. Several properties make it an excellent platform for many applications, from nanosensor to quantum information processing. This thesis presents the first explorations of NV-based technologies in our laboratory, investigating three sets of studies aimed at learning the know-how of this field of research and developing the necessary infrastructure to explore them in future quantum technologies. The first set of studies focus on magnetometry and how to improve NV-based magnetic sensing. We show that, using engineered ensembles of NV centers in ultrapure synthetic diamonds, one can build a relatively simple apparatus to do magnetic imaging of relatively large areas while determining the full vector field with high spatial resolution and very good sensitivity. We also show that these measurements can be used to reconstruct the current density distribution of nearby sources, opening exciting possibilities to study two-dimensional materials. Another set of studies involve spin coherence of an ensemble of NV centers. For that, we developed a method based on a CCD camera and an imaging protocol that allows implementing pulse sequences like Rabi, Ramsey and Hahn echo, performing Electron Spin Resonance (ESR) spectroscopy over extended areas. Using this method we extract parameters from our sample, including measurements for T1, T2 and T*2. The method was also used to observe Electron Spin Echo Envelope Modulation (ESEEM), due to hyperfine interaction with nearby 15N nucleus, resulting in improved frequency sensitivity. The third set of studies explore how to use femtosecond lasers to produce NV centers in diamond and investigated the nonlinear index of refraction (n2) of the diamond (type IIa) in a broad spectral region, from the infrared (1500 nm) to the ultraviolet (260 nm). / Entre várias centenas de impurezas e defeitos que podem ocorrer no diamante, o centro Nitrogênio-Vacância (NV) é um dos mais interessantes para tecnologias quânticas em temperatura ambiente. Diversas propriedades fazem dele uma excelente plataforma para muitas aplicações, desde nanosensores até o processamento de informações quânticas. Esta tese apresenta a primeira exploração de tecnologias baseadas em NV no nosso laboratório, investigando três conjuntos de estudos com objetivo de aprender o know-how desta área de pesquisa e desenvolver a infra-estrutura necessária para explorá-los em futuras tecnologias quânticas. O primeiro conjunto de estudos enfoca a magnetometria e como melhorar o sensores magnético baseado em centros NV. Mostramos que um aparato relativamente simples pode ser usado para produzir imagens magnéticas do campo vetorial, usando ensembles de centros NV em diamantes sintéticos ultrapuros. Também mostramos que essas medidas podem ser usadas para reconstruir a distribuição de densidade de corrente de fontes próximas, abrindo possibilidades interessantes para o estudo de materiais bidimensionais. Outro conjunto de estudos envolve a coerência de spin de um ensemble de centros NV. Para isso, desenvolvemos um método baseado em uma câmera CCD e um protocolo de imagem que permite implementar sequências de pulsos como Rabi, Ramsey e eco Hahn, realizando espectroscopia de ressonância de spin eletrônico (ESR) sobre áreas estendidas. Usando esse método, extraímos parâmetros de nossa amostra, incluindo medidas para T1, T2 e T*2. O método também foi usado para observar o efeito ESEEM (Envelope de Modulação de Eco de Spin Eletrônico), devido à interação hiperfina com o núcleo próximo de 15N, resultando numa melhor sensibilidade de freqüência. Finalmente, o terceiro conjunto de estudos explorou como usar lasers de femtossegundos para produzir centros NV em diamante e investigou o índice de refração não-linear (n2) do diamante (tipo IIa) em uma ampla região espectral, desde o infravermelho (1500 nm) até o ultravioleta (260 nm).