Spontaneous parametric down-conversion (SPDC) is a nonlinear optical process in which an incident field known as the pump interacts with a nonlinear crystal to produce two output fields known as signal and idler. Due to the conservation of energy and momentum, these output fields are entangled in the temporal and spatial degrees of freedom. The gain, which represents the strength of the interaction, increases in direct proportion to the strength of the pump field. In the low-gain regime, the generated field is an entangled two-photon state. This regime continues to be routinely employed in fundamental quantum optics experiments and quantum technologies. In the high-gain regime, the generated field is a multiphoton entangled state known as a bright squeezed vacuum. The goal of this thesis is to theoretically and experimentally characterize the spatial correlations present in high-gain SPDC. In order to characterize the spatial correlations between the generated fields, we utilize the Schmidt decomposition formalism. In this study, we examine the evolution of the Schmidt modes and spectrum with increasing pump amplitude. Our work shows that the Schmidt modes expand marginally in size, and the Schmidt spectrum narrows with respect to increasing gain. The narrowing of the Schmidt spectrum, as quantified by a decrease in the Schmidt number, indicates a gradual decrease in spatial entanglement.

This thesis describes various methods for producing photon pairs from waveguides. It covers relevant topics such as waveguide coupling and phase matching, along with the relevant measurement techniques used to infer photon pair production. A new proposal to solve the phase matching problem is described along with two conceptual methods for generating entangled photon pairs. Photon pairs are also experimentally demonstrated from a third novel structure called a Bragg Reflection Waveguide (BRW). The new proposal to solve the phase matching problem is called Directional Quasi-Phase Matching (DQPM). It is a technique that exploits the directional dependence of the non-linear susceptiblity ($\chi^{(2)}$) tensor. It is aimed at those materials that do not allow birefringent phase-matching or periodic poling. In particular, it focuses on waveguides in which the interplay between the propagation direction, electric field polarizations and the nonlinearity can change the strength and sign of the nonlinear interaction periodically to achieve quasi-phasematching. One of the new conceptual methods for generating entangled photon pairs involves a new technique that sandwiches two waveguides from two differently oriented but similar crystals together. The idea stems from the design of a Michelson interferometer which interferes the paths over which two unique photon pair processes can occur, thereby creating entanglement in any pair of photons created in the interferometer. By forcing or sandwiching the two waveguides together, the physical space that exists in the standard Micheleson type interferometer is made non-existent, and the interferometer is effectively squashed. The result is that the two unique photon pair processes actually occupy the same physical path. This benefits the stability of the interferometer in addition to miniaturizing it. The technical challenges involved in sandwiching the two waveguides are briefly discussed. The main result of this thesis is the observation of photon pairs from the BRW. By analyzing the time correlation between two single photon detection events, spontaneous parametric down conversion (SPDC) of a picosecond pulsed ti:sapph laser is demonstrated. The process is mediated by a ridge BRW. The results show evidence for type-0, type-I and type-II phase matching of pump light at 783nm, 786nm and 789nm to down converted light that is strongly degenerate at 1566nm, 1572nm, and 1578nm respectively. The inferred efficiency of the BRW was 9.8$\cdot$10$^{-9}$ photon pairs per pump photon. This contrasts with the predicted type-0 efficiency of 2.65$\cdot$10$^{-11}$. This data is presented for the first time in such waveguides, and represents significant advances towards the integration of sources of quantum information into the existing telecommunications infrastructure.

This thesis describes various methods for producing photon pairs from waveguides. It covers relevant topics such as waveguide coupling and phase matching, along with the relevant measurement techniques used to infer photon pair production. A new proposal to solve the phase matching problem is described along with two conceptual methods for generating entangled photon pairs. Photon pairs are also experimentally demonstrated from a third novel structure called a Bragg Reflection Waveguide (BRW). The new proposal to solve the phase matching problem is called Directional Quasi-Phase Matching (DQPM). It is a technique that exploits the directional dependence of the non-linear susceptiblity ($\chi^{(2)}$) tensor. It is aimed at those materials that do not allow birefringent phase-matching or periodic poling. In particular, it focuses on waveguides in which the interplay between the propagation direction, electric field polarizations and the nonlinearity can change the strength and sign of the nonlinear interaction periodically to achieve quasi-phasematching. One of the new conceptual methods for generating entangled photon pairs involves a new technique that sandwiches two waveguides from two differently oriented but similar crystals together. The idea stems from the design of a Michelson interferometer which interferes the paths over which two unique photon pair processes can occur, thereby creating entanglement in any pair of photons created in the interferometer. By forcing or sandwiching the two waveguides together, the physical space that exists in the standard Micheleson type interferometer is made non-existent, and the interferometer is effectively squashed. The result is that the two unique photon pair processes actually occupy the same physical path. This benefits the stability of the interferometer in addition to miniaturizing it. The technical challenges involved in sandwiching the two waveguides are briefly discussed. The main result of this thesis is the observation of photon pairs from the BRW. By analyzing the time correlation between two single photon detection events, spontaneous parametric down conversion (SPDC) of a picosecond pulsed ti:sapph laser is demonstrated. The process is mediated by a ridge BRW. The results show evidence for type-0, type-I and type-II phase matching of pump light at 783nm, 786nm and 789nm to down converted light that is strongly degenerate at 1566nm, 1572nm, and 1578nm respectively. The inferred efficiency of the BRW was 9.8$\cdot$10$^{-9}$ photon pairs per pump photon. This contrasts with the predicted type-0 efficiency of 2.65$\cdot$10$^{-11}$. This data is presented for the first time in such waveguides, and represents significant advances towards the integration of sources of quantum information into the existing telecommunications infrastructure.

The experiments described in this thesis form an investigation into the path towards establishing the requirements of quantum computing in a linear optical system. Our qubits are polarisation encoded photons for which the basic operations of quantum computing, single qubit rotations, are a well understood problem. The difficulty lies in the interaction of photons. To achieve these we use measurement induced non-linearities. The first experiment in this thesis describes the thorough characterisation of a controlled-sign gate based on such non-linearities. The photons are provided as pairs generated through parametric down-conversion, and as such share correlations unlikely to carry over into large scale implementations of the future. En route to such larger circuits, a characterisation of the actions of the controlled-sign gate is conducted, when the input qubits have been generated independently from each other, revealing a large drop in process fidelity. To explore the cause of this degradation of the gate performance a thorough and highly accurate model of the gate is derived including the realistic description of faulty circuitry, photon loss and multi-photon emission by the source. By simulating the effects of the various noise sources individually, the heretofore largely ignored multi-photon emission is identified as the prime cause of the degraded gate performance, causing a drop in fidelity nearly three times as large as any other error source. I further draw the first comparison between the performance of an experimental gate to the error probabilities per gate derived as thresholds for fault-tolerant quantum computing. In the absence of a single vigourous threshold value, I compare the gate performance to the models that yielded the highest threshold to date as an upper bound and to the threshold of the Gremlin-model, which allows for the most general errors. Unsurprisingly this comparison reveals that the implemented gate is clearly insufficient, however just remedying the multi-photon emission error will allow this architecture to move to within striking distance of the boundary for fault-tolerant quantum computing. The utilised methodology can be applied to any gate in any architecture and can, combined with a suitable model of the noise sources, become an important guide for developments required to achieve fault tolerant quantum computing. The final experiment on the path towards linear optical quantum computing is the demonstration of a pair of basic versions of Shor's algorithm which display the essential entanglement for the algorithm. The results again highlight the need for extensive measurements to reveal the fundamental quality of the implemented algorithm, which is not accessible with limited indicative measurements. In the second part of the thesis, I describe two experiments on other forms of entanglement by extending the actions of a Fock-State filter, a filter that is capable of attenuating single photon states stronger than multi-photon states, to produce entangled states. Furthermore this device can be used in conjunction with standard wave-plates to extend the range of operations possible on the bi-photonic qutrit space, showing that this setup suffices to produce any desired qutrit state, thereby giving access to new measurement capabilities and in the process creating and proving the first entanglement between a qubit and a qutrit.

The experiments described in this thesis form an investigation into the path towards establishing the requirements of quantum computing in a linear optical system. Our qubits are polarisation encoded photons for which the basic operations of quantum computing, single qubit rotations, are a well understood problem. The difficulty lies in the interaction of photons. To achieve these we use measurement induced non-linearities. The first experiment in this thesis describes the thorough characterisation of a controlled-sign gate based on such non-linearities. The photons are provided as pairs generated through parametric down-conversion, and as such share correlations unlikely to carry over into large scale implementations of the future. En route to such larger circuits, a characterisation of the actions of the controlled-sign gate is conducted, when the input qubits have been generated independently from each other, revealing a large drop in process fidelity. To explore the cause of this degradation of the gate performance a thorough and highly accurate model of the gate is derived including the realistic description of faulty circuitry, photon loss and multi-photon emission by the source. By simulating the effects of the various noise sources individually, the heretofore largely ignored multi-photon emission is identified as the prime cause of the degraded gate performance, causing a drop in fidelity nearly three times as large as any other error source. I further draw the first comparison between the performance of an experimental gate to the error probabilities per gate derived as thresholds for fault-tolerant quantum computing. In the absence of a single vigourous threshold value, I compare the gate performance to the models that yielded the highest threshold to date as an upper bound and to the threshold of the Gremlin-model, which allows for the most general errors. Unsurprisingly this comparison reveals that the implemented gate is clearly insufficient, however just remedying the multi-photon emission error will allow this architecture to move to within striking distance of the boundary for fault-tolerant quantum computing. The utilised methodology can be applied to any gate in any architecture and can, combined with a suitable model of the noise sources, become an important guide for developments required to achieve fault tolerant quantum computing. The final experiment on the path towards linear optical quantum computing is the demonstration of a pair of basic versions of Shor's algorithm which display the essential entanglement for the algorithm. The results again highlight the need for extensive measurements to reveal the fundamental quality of the implemented algorithm, which is not accessible with limited indicative measurements. In the second part of the thesis, I describe two experiments on other forms of entanglement by extending the actions of a Fock-State filter, a filter that is capable of attenuating single photon states stronger than multi-photon states, to produce entangled states. Furthermore this device can be used in conjunction with standard wave-plates to extend the range of operations possible on the bi-photonic qutrit space, showing that this setup suffices to produce any desired qutrit state, thereby giving access to new measurement capabilities and in the process creating and proving the first entanglement between a qubit and a qutrit.

The experiments described in this thesis form an investigation into the path towards establishing the requirements of quantum computing in a linear optical system. Our qubits are polarisation encoded photons for which the basic operations of quantum computing, single qubit rotations, are a well understood problem. The difficulty lies in the interaction of photons. To achieve these we use measurement induced non-linearities. The first experiment in this thesis describes the thorough characterisation of a controlled-sign gate based on such non-linearities. The photons are provided as pairs generated through parametric down-conversion, and as such share correlations unlikely to carry over into large scale implementations of the future. En route to such larger circuits, a characterisation of the actions of the controlled-sign gate is conducted, when the input qubits have been generated independently from each other, revealing a large drop in process fidelity. To explore the cause of this degradation of the gate performance a thorough and highly accurate model of the gate is derived including the realistic description of faulty circuitry, photon loss and multi-photon emission by the source. By simulating the effects of the various noise sources individually, the heretofore largely ignored multi-photon emission is identified as the prime cause of the degraded gate performance, causing a drop in fidelity nearly three times as large as any other error source. I further draw the first comparison between the performance of an experimental gate to the error probabilities per gate derived as thresholds for fault-tolerant quantum computing. In the absence of a single vigourous threshold value, I compare the gate performance to the models that yielded the highest threshold to date as an upper bound and to the threshold of the Gremlin-model, which allows for the most general errors. Unsurprisingly this comparison reveals that the implemented gate is clearly insufficient, however just remedying the multi-photon emission error will allow this architecture to move to within striking distance of the boundary for fault-tolerant quantum computing. The utilised methodology can be applied to any gate in any architecture and can, combined with a suitable model of the noise sources, become an important guide for developments required to achieve fault tolerant quantum computing. The final experiment on the path towards linear optical quantum computing is the demonstration of a pair of basic versions of Shor's algorithm which display the essential entanglement for the algorithm. The results again highlight the need for extensive measurements to reveal the fundamental quality of the implemented algorithm, which is not accessible with limited indicative measurements. In the second part of the thesis, I describe two experiments on other forms of entanglement by extending the actions of a Fock-State filter, a filter that is capable of attenuating single photon states stronger than multi-photon states, to produce entangled states. Furthermore this device can be used in conjunction with standard wave-plates to extend the range of operations possible on the bi-photonic qutrit space, showing that this setup suffices to produce any desired qutrit state, thereby giving access to new measurement capabilities and in the process creating and proving the first entanglement between a qubit and a qutrit.

Submitted by Fabio Sobreira Campos da Costa (fabio.sobreira@ufpe.br) on 2017-02-13T13:44:40Z No. of bitstreams: 2 license_rdf: 1232 bytes, checksum: 66e71c371cc565284e70f40736c94386 (MD5) dissertação final.pdf: 3576056 bytes, checksum: 4650485627f1eb13bb131bcbf6ab588a (MD5) / Made available in DSpace on 2017-02-13T13:44:40Z (GMT). No. of bitstreams: 2 license_rdf: 1232 bytes, checksum: 66e71c371cc565284e70f40736c94386 (MD5) dissertação final.pdf: 3576056 bytes, checksum: 4650485627f1eb13bb131bcbf6ab588a (MD5) Previous issue date: 2014-03-28 / CAPES / A criação de estados emaranhados em polarização permite testar experimentalmente questões fundamentais da mecânica quântica, tais como os argumentos de EPR sobre a incompletezadateoriaquântica,atravésdadesigualdadeCHSH.Alémdisso,essesestados emaranhados, têm potenciais de aplicações como, por exemplo, em computação quântica e criptografia quântica. Neste trabalho, se estuda uma fonte muito eficiente para a produção de estados de fótons emaranhados em polarização baseada em um interferômetro de tipo Sagnac. Estes fótons correlacionados são criados em um cristal não linear PPKTP mediante o processo de conversão paramétrica descendente (PDC) tipo-II, quando o cristal é bombeado por pulsos de fentossegundos. Verificando as correlações das medidas de polarização produzidas por esta fonte, observamos fortes violações das desigualdades de Bell para estados de polarização, isto é, verificamos a desigualdade CHSH. / Creation of polarization entangled states allows experimentally to test fundamental properties of quantum mechanics, such as the EPR argument about the incompleteness of the quantum theory, through CHSH inequality; in addition to potential applications as in quantum computing and quantum cryptography. This work studies a very efficient sourceofphotonentangledstatesofpolarizationbasedonaSagnacinterferometer. These photons are created from a nonlinear PPKTP crystal pumped by fentosecond pulses by theprocessofparametricdown-conversion(PDC)type-IIpumpedbyfemtosecondpulses. Analysing correlations of polarization measurements produced by this source we observed strong violations of Bell inequalities for the polarization states, i.e, CHSH inequality.

We explore the optical parametric amplifier, an optical device where a pump field creates a pair of lower-frequency fields: signal and idler. The pump field is usually treated classically, but this thesis focuses on scenarios where the pump must be treated quantum mechanically. One of these scenarios is the growing field of nonlinear interferometry, where the fundamental sensitivity of a probed relative phase can beat the classical bounds and reach the maximum limit allowed by quantum mechanics, the Heisenberg limit. Indeed, we show that a fully quantum nonlinear interferometer displays a Heisenberg scaling in terms of the mean number of input pump photons. This result goes beyond the well-accepted Heisenberg scaling with respect to the down-converted photons inside the interferometer, which predicts unphysical phase sensitivities starting at a particular input pump energy. Our theoretical findings are particularly useful when designing a nonlinear interferometer with bright pump fields or optimized optical parametric amplifiers for quantum metrology and quantum imaging applications. The quantum nature of the pump field may also play a central role concerning other physical phenomena, like Hawking radiation in the context of black holes. As suggested by several authors, both the optical parametric amplifier and Hawking radiation comprise the creation of fundamental particle pairs. Thus, if the optical parametric amplifier is fully treated quantum mechanically, we may get insight into an open problem in modern physics, namely the black hole information paradox. According to this paradox, the information stored in a black hole can be destroyed once the black hole has evaporated by emitting Hawking radiation, contradicting quantum mechanics. Despite the experimental efforts to build systems that reproduce event horizons and gravitational effects in the laboratory, the evaporation of black holes due to the emission of Hawking radiation remains a challenging task. In this thesis, we experimentally investigate the impact of an evolving pump field in an optical parametric amplifier by optimizing a parametric down-conversion process. We measure the pump and signal photon number properties, finding that the pump field gets chaotic and the signal coherent when the pump displays some sizeable depletion. We arrive at similar conclusions about the pump field from its measured Wigner function. Our experiment is the first step towards a successful experiment that could suggest that information in the black hole is not destroyed but encoded in the emitted Hawking radiation starting at some point in the black hole evolution. We finally discuss further experimental improvements to investigate the parallel between the optical parametric amplifier and Hawking radiation.

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付記する学位プログラム名: 京都大学卓越大学院プログラム「先端光・電子デバイス創成学」 / 京都大学 / 新制・課程博士 / 博士(工学) / 甲第24621号 / 工博第5127号 / 新制||工||1980(附属図書館) / 京都大学大学院工学研究科電子工学専攻 / (主査)教授 竹内 繁樹, 教授 川上 養一, 教授 木本 恒暢 / 学位規則第4条第1項該当 / Doctor of Philosophy (Engineering) / Kyoto University / DGAM