Doctor Educationis / The progressive development of scintillator detectors has made it possible to perform direct electronic lifetime determination up to a few hundred nanoseconds. The 2” by 2” LaBr3:Ce detectors provide a combination of excellent time resolution and good energy resolution. Recently a fast timing array has been commissioned at iThemba LABS, Cape Town consisting of eight 2” by 2” LaBr3:Ce detectors. Test measurements using radioactive sources produced at the laboratory were conducted. Six 2” by 2” LaBr3:Ce detectors were coupled to the AFRODITE array as their first in-beam experiment. AFRODITE consisted of eight HPGe clover detectors as well as two 3.5” x 8” LaBr3:Ce detectors. A particle telescope was used to select the desired reaction channels. The reactions of interest 45Sc(p,d)44Sc and 45Sc(p,α) 42Ca were carried out at a beam energy of 27 MeV. The current analysis also investigates the rare earth nucleus 150Gd which was populated through 150Sm(α,4n)150Gd at a beam energy of 48 MeV. Through these reactions, excited states that have lifetimes which are apt for the characterization of the 2” by 2” LaBr3:Ce detectors were populated. Various techniques such as the slope method and the centroid shift method have been employed to extract the lifetimes of excited states. Lifetimes that were previously measured for 44Sc and 42Ca were measured again in this work. New lifetimes were obtained 44Sc and 150Gd. Shell Model calculation were done to compare experimental and theoretical results. All these endeavours will seek to unveil the quadrupole moment of nuclei and their intrinsic behaviour.

<p>A Monte Carlo simulation of the Neutron Wall detector system has been performed using Geant4, in order to define optimum conditions for the detection and identification of multiple neutrons. Emphasis was put on studying the scattering of neutrons between different detectors, which is the main source of the apparent increase of the number of detected neutrons. The simulation has been compared with experimental data. The quality of neutron gated γ-ray spectra was improved for both two- and three-neutron evaporation channels. The influence of small amounts of γ rays mis-interpreted as neutrons was investigated. It was found that such γ rays dramatically reduce the quality of neutron gated γ-ray spectra.</p><p>The interaction properties of fast neutrons in a closed-end coaxial and a planar high-purity germanium detector (HPGe) were studied. Digitised waveforms of HPGe preamplifier signals were recorded for time-of-flight separated neutrons and γ rays, emitted by a ²⁵²Cf source. The experimental waveforms from the detectors were compared to simulated pulse shapes. In the analysis, special emphasis was given to the detection of elastically scattered neutrons, which may be an important effect to take into account in future spectrometers based on γ-ray tracking. No differences between neutron and γ-ray induced pulse shapes were found in this work.</p><p>A Monte Carlo simulation of the interactions of fast neutrons in the future 4π γ-ray spectrometer AGATA was also performed, in order to study the influence of neutrons on γ-ray tracking. It was shown that although there is a large probability of detecting neutrons in AGATA, the neutrons decrease the photo-peak efficiency of AGATA by only about 1% for each neutron emitted in coincidence with γ rays. The peak-to-background ratios in γ-ray spectra are, however, reduced to a much larger extent. The possibility of using AGATA as a neutron detector system was also investigated.</p>

A Monte Carlo simulation of the Neutron Wall detector system has been performed using Geant4, in order to define optimum conditions for the detection and identification of multiple neutrons. Emphasis was put on studying the scattering of neutrons between different detectors, which is the main source of the apparent increase of the number of detected neutrons. The simulation has been compared with experimental data. The quality of neutron gated γ-ray spectra was improved for both two- and three-neutron evaporation channels. The influence of small amounts of γ rays mis-interpreted as neutrons was investigated. It was found that such γ rays dramatically reduce the quality of neutron gated γ-ray spectra. The interaction properties of fast neutrons in a closed-end coaxial and a planar high-purity germanium detector (HPGe) were studied. Digitised waveforms of HPGe preamplifier signals were recorded for time-of-flight separated neutrons and γ rays, emitted by a 252Cf source. The experimental waveforms from the detectors were compared to simulated pulse shapes. In the analysis, special emphasis was given to the detection of elastically scattered neutrons, which may be an important effect to take into account in future spectrometers based on γ-ray tracking. No differences between neutron and γ-ray induced pulse shapes were found in this work. A Monte Carlo simulation of the interactions of fast neutrons in the future 4π γ-ray spectrometer AGATA was also performed, in order to study the influence of neutrons on γ-ray tracking. It was shown that although there is a large probability of detecting neutrons in AGATA, the neutrons decrease the photo-peak efficiency of AGATA by only about 1% for each neutron emitted in coincidence with γ rays. The peak-to-background ratios in γ-ray spectra are, however, reduced to a much larger extent. The possibility of using AGATA as a neutron detector system was also investigated.