This thesis is part of a broader project that examines three different approaches to evaluating trace metal contamination in urban brownfields: the measure of total soil metals; calculating bioavailable metals; and the use of species as bioindicators of trace metals in soils. Chapter 1 discusses the problems inherent in each approach such as; inconsistent results due to differences in techniques, extrapolation from laboratory to field, and the influence of species differences and environmental conditions. Chapter 2 is a site description measuring biodiversity, community structure and activity of three urban brownfields. The site description was used to select organisms that were subsequently evaluated for their usefulness as bioindicators of trace metals (chapter 3). Of the three plant species used (dandelion, bladder campion, and chicory), dandelion has the possibility of being a suitable bioindicator of Cd, Ni, and Zn, while bladder campion may be suitable for evaluating Cd, Ni, Pb, and Zn.

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Due to mining activities, the natural vegetation cover in Gatumba area was removed and replaced either by crops or bare wasteland with reduced available arable land. The main aim of the study was to assess the impact of the mining activities on the plant mineral uptake and the dynamics of the vegetation. The vegetation in this area under investigation was diversified and heterogeneous. Trace element concentrations in soils were similar to those in plant parts but some elements were highly concentrated in soils than in plants. According to the bioaccumulation factors of the analyzed trace elements in plant parts, two categories of plants were identified, and these are excluders and accumulators. No toxic levels of the evaluated trace elements were found in the analyzed plant samples. As a recommendation for the adaptation of plants to Gatumba mining environment, the most useful plant species for the revegetation/restitution of the technosols should be Sesbania sesban, Crotalaria dewildemaniana and Tithonia diversifolia subject to further experiments on trace elements bioaccumulation and organic matter production / Environmental Sciences / M.A. Science (Environmental Sciences)

Due to mining activities, the natural vegetation cover in Gatumba area was removed and replaced either by crops or bare wasteland with reduced available arable land. The main aim of the study was to assess the impact of the mining activities on the plant mineral uptake and the dynamics of the vegetation. The vegetation in this area under investigation was diversified and heterogeneous. Trace element concentrations in soils were similar to those in plant parts but some elements were highly concentrated in soils than in plants. According to the bioaccumulation factors of the analyzed trace elements in plant parts, two categories of plants were identified, and these are excluders and accumulators. No toxic levels of the evaluated trace elements were found in the analyzed plant samples. As a recommendation for the adaptation of plants to Gatumba mining environment, the most useful plant species for the revegetation/restitution of the technosols should be Sesbania sesban, Crotalaria dewildemaniana and Tithonia diversifolia subject to further experiments on trace elements bioaccumulation and organic matter production / Environmental Sciences / M.A. Science (Environmental Sciences)

Indiana University-Purdue University Indianapolis (IUPUI) / Mercury (Hg) has proven to be a risk to the public, mainly through the consumption of fish. Because of this, many fish consumption advisories have been issued in Indiana. Although much is known about the global cycle of mercury, little is known about how local and regional emission sources of mercury impact local and regional mercury cycling. This study’s objective was to determine the scope of mercury concentration in central Indiana by using a broad grid of soil mercury measurements. Sampling was designed to capture the net retained mercury content in soils, and to determine whether spatial patterns in exist in soil mercury contents that could be related to emission sources of mercury and post-emission transport patterns from wind. Results from this study revealed significant differences in mercury concentrations for soils in central Indiana. The core of the study area, concentrated in the urban area of Indianapolis, exhibited soil mercury contents that were 20 times higher than values in the outskirts of the study area. The spatial pattern resembled a bulls-eye shape centered on Indianapolis, and with comparison to the reported Hg emission from local sources, including a coal-fired power plant, indicates a strong regional deposition signal linked to those emission sources but marked by wind-driven transport to the northeast. This effect of local emission sources resulting in local deposition indicates that limiting mercury emissions will have a net beneficial impact on local environmental quality and human health.