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The purpose of this report is to present the results of the study and analysis of loss-of-coolant and loss-of-flow simulations performed on the Modular Helium Reactor developed by General Atomics using the thermal-hydraulics code RELAP5-3D/ATHENA. The MHR is a high temperature gas cooled reactor. It is a prismatic core concept for New Generation Nuclear Plant (NGNP). Very few reactors of that kind have been designed in the past. Furthermore, the MHR is supposed to be a highly passively safe concept. So there are high needs for numerical simulations in order to confirm the design. The project is dedicated to the assessment of the passive decay heat capabilities of the reactor under abnormal transient conditions. To comply with the requirements of the NGNP, fuel and structural temperatures must be kept under design safety limits under any circumstances. During the project, the MHR has been investigated: first under steady-state conditions and then under transient settings. The project confirms that satisfying passive decay heat removal by means of natural heat transfer mechanisms (convection, conduction and radiation) occurs.

The purpose of this report is to present the results of the study and analysis of loss-of-coolant and loss-of-flow simulations performed on the Modular Helium Reactor developed by General Atomics using the thermal-hydraulics code RELAP5-3D/ATHENA. The MHR is a high temperature gas cooled reactor. It is a prismatic core concept for New Generation Nuclear Plant (NGNP). Very few reactors of that kind have been designed in the past. Furthermore, the MHR is supposed to be a highly passively safe concept. So there are high needs for numerical simulations in order to confirm the design. The project is dedicated to the assessment of the passive decay heat capabilities of the reactor under abnormal transient conditions. To comply with the requirements of the NGNP, fuel and structural temperatures must be kept under design safety limits under any circumstances. During the project, the MHR has been investigated: first under steady-state conditions and then under transient settings. The project confirms that satisfying passive decay heat removal by means of natural heat transfer mechanisms (convection, conduction and radiation) occurs.

To safely encase and store spent fuel assemblies in its final geological storage, accurate measurements of their heat output must be performed. To this end, information about the geometry and sensor set-up of the calorimeter at the interim storage facility CLAB was gathered. The data from the temperature sensors where compared to each other and an analytical expression was proposed to fit the data. A methodology for calculating calibration curves was formulated and its uncertainties were evaluated. Differences were found between the fits of measurements from differing measurement campaigns. The measurement campaigns resulted in calibration curves with notable offset from each other. The computer code SERPENT2 was used to construct a 3d geometry model of the calorimeter and the ratio of photons entering and escaping the calorimeter wall was calculated for photon energies which dominate the gamma spectrum from spent fuel assemblies of about 5 to 40 years cooling time.

This thesis is devoted to the investigation of passivesafety and inherent features of subcritical nucleartransmutation systems - accelerator-driven systems. The generalobjective of this research has been to improve the safetyperformance and avoid elevated coolant temperatures inworst-case scenarios like unprotected loss-of-ow accidents,loss-of-heat-sink accidents, and a combination of both theseaccident initiators. The specific topics covered are emergencydecay heat removal by reactor vessel auxiliary cooling systems,beam shut-off by a melt-rupture disc, safety aspects fromlocating heat-exchangers in the riser of a pool-type reactorsystem, and reduction of pressure resistance in the primarycircuit by employing bypass routes. The initial part of the research was focused on reactorvessel auxiliary cooling systems. It was shown that an 80 MWthPb/Bi-cooled accelerator-driven system of 8 m height and 6 mdiameter vessel can be well cooled in the case of loss-of-owaccidents in which the accelerator proton beam is not switchedoff. After a loss-of-heat-sink accident the proton beam has tobe interrupted within 40 minutes in order to avoid fast creepof the vessel. If a melt-rupture disc is included in the wallof the beam pipe, which breaks at 150 K above the normal coreoutlet temperature, the grace period until the beam has to beshut off is increased to 6 hours. For the same vessel geometry,but an operating power of 250 MWth the structural materials canstill avoid fast creep in case the proton beam is shut offimmediately. If beam shut-off is delayed, additional coolingmethods are needed to increase the heat removal. Investigationswere made on the filling of the gap between the guard and thereactor vessel with liquid metal coolant and using water spraycooling on the guard vessel surface. The second part of the thesis presents examinationsregarding an accelerator-driven system also cooled with Pb/Bibut with heat-exchangers located in the risers of the reactorvessel. For a pool type design, this approach has advantages inthe case of heat-exchanger tube failures, particularly if wateris used as the secondary uid. This is because a leakage ofwater from the secondary circuit into the Pb/Bi-cooled primarycircuit leads to upward sweeping of steam bubbles, which wouldcollect in the gas plenum. In the case of heatexchangers in thedowncomer steam bubbles may be dragged into the ADS core andadd reactivity. Bypass routes are employed to increase the owspeed in loss-of-ow events for this design. It is shown thatthe 200 MWth accelerator-driven system with heat-exchangers inthe riser copes reasonably well with both a loss-of-ow accidentwith the beam on and an unprotected loss-of-heat-sink accident.For a total-loss-of-power (station blackout) and an immediatebeam-stop the core outlet temperature peaks at 680 K. After acombined loss-of-ow and loss-of-heat-sink accident the beamshould be shut off within 4 minutes to avoid exceeding the ASMElevel D of 977 K, and within 8 minutes to avoid fast creep.Assuming the same core inlet temperature, both the reactordesign with heat-exchanger in the risers and the downcomershave similar temperature evolutions after a total-loss-ofpoweraccident. A large accelerator-driven system of 800 MWth with a 17 mtall vessel may eventually become a standard size. For thishigher power ADS, the location of the heat-exchangers hasgreater impact on the natural convection capability. This isdue to that larger heatexchangers have more inuence on thedistance between the thermal centers during a lossof- owaccident. The design with heat-exchangers in the downcomers,the long-term vessel temperature peaks at 996 K during aloss-of-ow accident with the beam on. This does not pose athreat of creep rupture for the vessel. However, the locationof the heat-exchangers in the downcomers will probably requiresecondary coolant other than water, like for example oil (fortemperatures not higher than 673 K) or Pb/Bi coolant.

The accumulation of spent nuclear fuel may be hindering the expansion of nuclear electricity production. However, the reprocessing and recycling of spent fuel may reduce its volume and environmental burden. Although fast spectrum reactors are the preferred modality for transuranic element transmutation, such fast spectrum systems are in very short supply. It is therefore legitimate to investigate the recycling potential of thermal spectrum systems, which constitute the overwhelming majority of nuclear power plants worldwide. To do so efficiently, several new fuel assembly designs are proposed in this Thesis: these include (1) Mixed Oxide Fuel (MOX), (2) MOX fuel with Americium coating, (3) Inert-Matrix Fuel (IMF) with UOX as inner zone, and (4) IMF with MOX as inner zone. All these designs are investigated in a multi-recycling strategy, whereby the spent fuel from a given generation is re-used for the next generation. The accumulation of spent nuclear fuel may be hindering the expansion of nuclear electricity production. However, the reprocessing and recycling of spent fuel may reduce its volume and environmental burden. Although fast spectrum reactors are the preferred modality for transuranic element transmutation, such fast spectrum systems are in very short supply. It is therefore legitimate to investigate the recycling potential of thermal spectrum systems, which constitute the overwhelming majority of nuclear power plants worldwide. To do so efficiently, several new fuel assembly designs are proposed in this Thesis: these include (1) Mixed Oxide Fuel (MOX), (2) MOX fuel with Americium coating, (3) Inert-Matrix Fuel (IMF) with UOX as inner zone, and (4) IMF with MOX as inner zone. All these designs are investigated in a multi-recycling strategy, whereby the spent fuel from a given generation is re-used for the next generation.

<p>This thesis is devoted to the investigation of passivesafety and inherent features of subcritical nucleartransmutation systems - accelerator-driven systems. The generalobjective of this research has been to improve the safetyperformance and avoid elevated coolant temperatures inworst-case scenarios like unprotected loss-of-ow accidents,loss-of-heat-sink accidents, and a combination of both theseaccident initiators. The specific topics covered are emergencydecay heat removal by reactor vessel auxiliary cooling systems,beam shut-off by a melt-rupture disc, safety aspects fromlocating heat-exchangers in the riser of a pool-type reactorsystem, and reduction of pressure resistance in the primarycircuit by employing bypass routes.</p><p>The initial part of the research was focused on reactorvessel auxiliary cooling systems. It was shown that an 80 MWthPb/Bi-cooled accelerator-driven system of 8 m height and 6 mdiameter vessel can be well cooled in the case of loss-of-owaccidents in which the accelerator proton beam is not switchedoff. After a loss-of-heat-sink accident the proton beam has tobe interrupted within 40 minutes in order to avoid fast creepof the vessel. If a melt-rupture disc is included in the wallof the beam pipe, which breaks at 150 K above the normal coreoutlet temperature, the grace period until the beam has to beshut off is increased to 6 hours. For the same vessel geometry,but an operating power of 250 MWth the structural materials canstill avoid fast creep in case the proton beam is shut offimmediately. If beam shut-off is delayed, additional coolingmethods are needed to increase the heat removal. Investigationswere made on the filling of the gap between the guard and thereactor vessel with liquid metal coolant and using water spraycooling on the guard vessel surface.</p><p>The second part of the thesis presents examinationsregarding an accelerator-driven system also cooled with Pb/Bibut with heat-exchangers located in the risers of the reactorvessel. For a pool type design, this approach has advantages inthe case of heat-exchanger tube failures, particularly if wateris used as the secondary uid. This is because a leakage ofwater from the secondary circuit into the Pb/Bi-cooled primarycircuit leads to upward sweeping of steam bubbles, which wouldcollect in the gas plenum. In the case of heatexchangers in thedowncomer steam bubbles may be dragged into the ADS core andadd reactivity. Bypass routes are employed to increase the owspeed in loss-of-ow events for this design. It is shown thatthe 200 MWth accelerator-driven system with heat-exchangers inthe riser copes reasonably well with both a loss-of-ow accidentwith the beam on and an unprotected loss-of-heat-sink accident.For a total-loss-of-power (station blackout) and an immediatebeam-stop the core outlet temperature peaks at 680 K. After acombined loss-of-ow and loss-of-heat-sink accident the beamshould be shut off within 4 minutes to avoid exceeding the ASMElevel D of 977 K, and within 8 minutes to avoid fast creep.Assuming the same core inlet temperature, both the reactordesign with heat-exchanger in the risers and the downcomershave similar temperature evolutions after a total-loss-ofpoweraccident.</p><p>A large accelerator-driven system of 800 MWth with a 17 mtall vessel may eventually become a standard size. For thishigher power ADS, the location of the heat-exchangers hasgreater impact on the natural convection capability. This isdue to that larger heatexchangers have more inuence on thedistance between the thermal centers during a lossof- owaccident. The design with heat-exchangers in the downcomers,the long-term vessel temperature peaks at 996 K during aloss-of-ow accident with the beam on. This does not pose athreat of creep rupture for the vessel. However, the locationof the heat-exchangers in the downcomers will probably requiresecondary coolant other than water, like for example oil (fortemperatures not higher than 673 K) or Pb/Bi coolant.</p>

Aujourd’hui, l’énergie nucléaire représente une partie non-négligeable du marché énergétique mondial, très probablement vouée à croître dans les prochaines décennies. Les réacteurs du futur devront notamment répondre à des critères supplémentaires économiques mais surtout de sûreté, de non-prolifération, de gestion optimisée du combustible et d’une gestion responsable des déchets nucléaires. Dans le cadre de cette thèse, des études concernant la non-prolifération des armes nucléaires sont abordées, dans le cadre de la recherche et développement d’un nouvel outil potentiel de surveillance des réacteurs nucléaires ; la détection des antineutrinos des réacteurs. En effet, les propriétés de ces particules pourraient intéresser l’Agence Internationale de l’Energie Atomique (AIEA) en charge de l’application du Traité de non-prolifération des armes nucléaires. L’AIEA encourage ainsi ses états membres à mener une étude de faisabilité. Une première étude de non-prolifération est réalisée avec la simulation d’un scénario proliférant utilisant un réacteur de type CANDU et de l’émission en antineutrinos associée. Nous en déduisons une prédiction de la sensibilité d’un détecteur d’antineutrinos de taille modeste à la diversion d’une quantité significative de plutonium. Une seconde étude est réalisée dans le cadre du projet Nucifer, détecteur d’antineutrinos placé auprès du réacteur de recherche OSIRIS. Nucifer est un détecteur d’antineutrinos dédié à la non-prolifération à l’efficacité optimisée conçu pour être un démonstrateur pour l’AIEA. La simulation du réacteur OSIRIS est développée ici pour le calcul de l’émission d’antineutrinos qui sera comparée aux données mesurées par le détecteur ainsi que pour caractériser le bruit de fond important émis par le réacteur détecté dans Nucifer. De façon générale, les antineutrinos des réacteurs sont émis lors des décroissances radioactives des produits de fission. Ces décroissances radioactives sont également à l’origine de la puissance résiduelle émise après l’arrêt d’un réacteur nucléaire, dont l’estimation est un enjeu de sûreté. Nous présenterons dans cette thèse un travail expérimental dont le but est de mesurer les propriétés de décroissance bêta de produits de fission importants pour la non-prolifération et la puissance résiduelle des réacteurs. Des premières mesures utilisant la technique de Spectroscopie par Absorption Totale (TAGS) ont été réalisées auprès du dispositif de l’Université de Jyväskylä. Nous présenterons la technique employée, le dispositif expérimental ainsi qu’une partie de l’analyse de cette expérience. / Today, nuclear energy represents a non-negligible part of the global energy market, most likely a rolling wheel to grow in the coming decades. Reactors of the future must face the criteria including additional economic but also safety, non-proliferation, optimized fuel management and responsible management of nuclear waste. In the framework of this thesis, studies on non-proliferation of nuclear weapons are discussed in the context of research and development of a new potential tool for monitoring nuclear reactors, the detection of reactor antineutrinos, because the properties of these particles may be of interest for the International Agency of Atomic Energy (IAEA), in charge of the verification of the compliance by States with their safeguards obligations as well as on matters relating to international peace and security. The IAEA encouraged its member states to carry on a feasibility study. A first study of non-proliferation is performed with a simulation, using a proliferating scenario with a CANDU reactor and the associated antineutrinos emission. We derive a prediction of the sensitivity of an antineutrino detector of modest size for the purpose of the diversion of a significant amount of plutonium. A second study was realized as part of the Nucifer project, an antineutrino detector placed nearby the OSIRIS research reactor. The Nucifer antineutrino detector is dedicated to non-proliferation with an optimized efficiency, designed to be a demonstrator for the IAEA. The simulation of the OSIRIS reactor is developed here for calculating the emission of antineutrinos which will be compared with the data measured by the detector and also for characterizing the level of background noises emitted by the reactor detected in Nucifer. In general, the reactor antineutrinos are emitted during radioactive decay of fission products. These radioactive decays are also the cause of the decay heat emitted after the shutdown of a nuclear reactor of which the estimation is an issue of nuclear safety. In this thesis, we present an experimental work which aims to measure the properties of beta decay of fission products important to the non-proliferation and reactor decay heat. First steps using the technique of Total Absorption Gamma-ray Spectroscopy (TAGS) were carried on at the radioactive beam facility of the University of Jyvaskyla. We will present the technique used, the experimental setup and part of the analysis of this experiment.

The predominant nuclear fuel used globally at present is uranium which is a finite resource. Thorium has been identified as an alternative nuclear fuel source that can be utilized in almost all existing uranium–based reactors and can significantly help in conserving limited uranium reserves. Furthermore, the elimination of proliferation risks associated with thorium–based fuel cycles is a key reason for re–evaluating the possible utilization of thorium in high temperature reactors. In addition to the many advantages that thorium–based fuel has over uranium–based fuel, there are vast thorium resources in the earth's crust that up until the present have not been exploited optimally. This study focuses on determining the amount of uranium ore that can be saved using thorium as a nuclear fuel in HTR's. Four identical 200 MWth high temperature reactors are considered which make use of different fuel cycles. These fuel cycles range from the conventional uranium fuel cycle to a thorium–based fuel cycle in which no U–238 is present and have been simulated using the VSOP–A system of computer codes. This study also considers the effect that protactinium, an isotope that occurs in thorium–based fuel cycles, will have on the decay heat production in the case of a depressurized loss of coolant (DLOFC) accident. / Thesis (M.Ing. (Nuclear Engineering))--North-West University, Potchefstroom Campus, 2011.

The predominant nuclear fuel used globally at present is uranium which is a finite resource. Thorium has been identified as an alternative nuclear fuel source that can be utilized in almost all existing uranium–based reactors and can significantly help in conserving limited uranium reserves. Furthermore, the elimination of proliferation risks associated with thorium–based fuel cycles is a key reason for re–evaluating the possible utilization of thorium in high temperature reactors. In addition to the many advantages that thorium–based fuel has over uranium–based fuel, there are vast thorium resources in the earth's crust that up until the present have not been exploited optimally. This study focuses on determining the amount of uranium ore that can be saved using thorium as a nuclear fuel in HTR's. Four identical 200 MWth high temperature reactors are considered which make use of different fuel cycles. These fuel cycles range from the conventional uranium fuel cycle to a thorium–based fuel cycle in which no U–238 is present and have been simulated using the VSOP–A system of computer codes. This study also considers the effect that protactinium, an isotope that occurs in thorium–based fuel cycles, will have on the decay heat production in the case of a depressurized loss of coolant (DLOFC) accident. / Thesis (M.Ing. (Nuclear Engineering))--North-West University, Potchefstroom Campus, 2011.