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This work aims to implement 3D microstructures that generate light with orbital angular momentum towards applications in Biophotonics. Over the past few decades, 3D printing has established itself as the most versatile technology with effortless adaptability. Parallel to this, the concept of miniaturiza tion has seen tremendous growth irrespective of the field and has become an estab lished trend motivated by the need for compact, portable and multi-function devices. Therefore, when these two concepts get together, i.e., 3D printing of miniaturized objects, it could lead to an exciting path with endless opportunities. When it comes to optics, miniaturized 3D printing offers the potential to create compact optical micro-systems and exhibits a way to manufacture freeform µ-optics. In particular, two-photon lithography (TPL) is a cutting edge 3D printing technology that has re cently demonstrated groundbreaking solutions for optics as it offers high resolution with a great degree of flexibility. With a TPL 3D printer, it is possible to fabricate complex µ-optical elements and employ them for compelling applications. In recent years, light with orbital angular momentum (OAM), or ”twisted” light, has captured the interests of several researchers due to its inspiring applications. Tra ditionally, to generate OAM beams, one would require bulk, table-top optics, restrict ing their applications to over-the-table setup. An alternative approach of OAM beam generation is through µ-structures over the fiber, as they can open up new opportu nities, especially in Bioscience, and facilitate in-vivo operations. In particular, this probe-like setup can be used for processes such as optical trapping, high-resolution microscopy, etc. Hence, I propose the development of a novel approach with un precedented capabilities for generating OAM beams right from single-mode optical fibers, by transforming its Gaussian-like output beam by using complex 3D printed microstructures. In this document, I will showcase designs and results on generating Bessel beams (both zeroth- and high-order) and high-NA converging beams (with and without OAM) for optical trapping from the fiber. Remarkably, I achieved the first-ever fiber-based high-order Bessel beam generation and the first-ever fiber optical tweezers with OAM.

<p> A high speed recoil transport system is developed making possible the simultaneous study of many decay products of the compound nucleus 221*Ac. Oeterminati ons of the efficiency properties of the transport system, essential for absolute cross section measurements , are discussed in detail. </p> <p> A study of angular momentum effects is made possibly by synthesis of 221*Ac using three heavy ion reactions. Absolute cross sections for (HI,xn) and (HI,pxn) reaction products are determined relative to established cross sections for production of 150Dy. Relative cross sections for francium production are also determined. </p> <p> A sophisticated statistical model calculation is adapted to provide a framework for interpretation of the results. Some insight is gained into the roles played by basic physical concepts in the systematic of compound nucleus decay in this mass region </p> / Thesis / Doctor of Philosophy (PhD)

In absence of external fields, vibrational modes of periodic systems are usually considered as linearly polarized and, as such, they do not carry angular momentum. Our work proves that non-adiabatic effects due to the electron-phonon coupling are time-reversal symmetry breaking interactions for the vibrational field in systems with non-collinear magnetism and large spin-orbit coupling. Since in these systems the deformation potential matrix elements are necessarily complex, a nonzero synthetic gauge field (Berry curvature) arises in the dynamic equations of the ionic motion. As a result, phonon modes are elliptically polarized in the non-adiabatic framework and intrinsic vibrational angular momenta occur even for non-degenerate modes and without external probes. These results are validated by performing fully relativistic ab-initio calculations on two insulating platinum clusters and a metallic manganese compound, with non-collinear magnetism. In both cases, non-adiabatic vibrational modes carry sizeable angular momenta comparable to the orbital electronic ones in itinerant ferromagnets.

The growth of data capacity in optical communications links, which form the critical backbone of the modern internet, is facing a slowdown due to fundamental nonlinear limitations, leading to an impending "capacity crunch" on the horizon. Current technology has already exhausted degrees of freedom such as wavelength, amplitude, phase and polarization, leaving spatial multiplexing as the last available dimension to be efficiently exploited. To minimize the significant energy requirements associated with digital signal processing, it is critical to explore the upper limit of unmixed spatial channels in an optical fiber, which necessitates ideally packing spatial channels either in real space or in momentum space. The former strategy is realized by uncoupled multi-core fibers whose channel count has already saturated due to reliability constraint limiting fiber sizes. The later strategy is realized by the unmixed multimode fiber whose high spatial efficiency suggest the possibility of high channel-count scalability but the right subset of mode ought to be selected in order to mitigate mode coupling that is ever-present due to the plethora of perturbations a fiber normally experiences. The azimuthal modes in ring-core fibers turn out to be one of the most spatially efficient in this regard, by exploiting light’s orbital angular momentum (OAM). Unmixed mode counts have reached 12 in a ~1km fiber and 24 in a ~10m fiber. However, there is a fundamental bottleneck for scalability of conventionally bound modes and their relatively high crosstalks restricts their utility to device length applications. In this thesis, we provide a fundamental solution to further fuel the unmixed-channel count in an MMF. We utilize the phenomenon of topological confinement, which is a regime of light guidance beyond conventional cutoff that has, to the best of our knowledge, never been demonstrated till publications based on the subject matter of this thesis. In this regime, light is guided by the centrifugal barrier created by light’s OAM itself rather than conventional total internal reflection arising from the index inhomogeneity of the fiber. The loss of these topologically confined modes (TCMs) decreases down to negligible levels by increasing the OAM of fiber modes, because the centrifugal barrier that keeps photons confined to a fiber core increases with the OAM value of the mode. This leads to low-loss transmission in a km-scale fiber of these cutoff modes. Crucially, the mode-dependent confinement loss of TCMs further lifts the degeneracy of wavevectors in the complex space, leading to frustration of phase-matched coupling. This thus allows further scaling the mode count that was previously hindered by degenerate mode coupling in conventionally bound fiber modes. The frustrated coupling of TCMs thus enables a record amount of unmixed OAM modes in any type of fiber that features a high index contrast, whether specially structured as a ring-core, or simply constructed as a step-index fiber. Using all these favorable attributes, we achieve up to 50 low-loss modes with record low crosstalk (approaching -45 dB/km) over a 130-nm bandwidth in a ~1km-long ring-core fiber. The TCM effect promises to be inherently scalable, suggesting that even higher modes counts can be obtained in the future using this design methodology. Hence, the use of TCMs promises breaking the record spectral efficiency, potentially making it the choice for transmission links in future Space-Division-Multiplexing systems. Apart from their chief attribute of significantly increasing the information content per photon for quantum or classical networks, we expect that this new light guidance may find other applications such as in nonlinear signal processing and light-matter interactions.

In this thesis, an investigation into the modal characteristics of novel beam shapes is presented. Sculpting the phase profile of a Gaussian beam can result in the generation of a beam with unique properties. Described in this thesis are Laguerre-Gaussian (LG), Hermite-Gaussian (HG) and Bessel beams (BBs). The diffraction of LG beam modes from a triangular aperture is explored and this effect can be used for the efficient measurement of the azimuthal mode index l that indicates the number of multiples of 2π of phase changes that the field displays around one circumference of the optical axis. In this study, only LG beams with zero radial mode index p, with p + 1 denoting the number of bright high intensity concentric rings around the optical axis, were considered. Then, a powerful approach to simultaneously determine both mode indices of a pure LG beam using the principal component analysis (PCA) algorithm on the observed far-field diffraction patterns was demonstrated. Owing to PCA algorithm, the shape of the diffracting element used to measure the mode indices is in fact of little importance and the crucial step is ‘training' any diffracting optical system and transforming the observed far-field diffraction patterns into the uncorrelated variables (principal components). Our PCA method is generic and it was extended to other families of light fields such as HG, Bessel and superposed beams. This reinforces the widespread applicability of this method for various applications. Finally, both theoretically and experimentally investigations using interferometry show the definitive linkage between both the radial and azimuthal mode indices of a partially coherent LG beam and the dislocation rings in the far-field cross-correlation function (CCF).

La génération d’harmoniques d’ordre élevé est un processus d’interaction lumière-matière hautement non-linéaire permettant la synthèse d’impulsions sub-femtosecondes, dites attosecondes (1 as = 10⁻¹⁸ s). Mes travaux de thèse portent sur l’étude du transfert de moment angulaire lors de ce processus, afin de contrôler les caractéristiques spatiales et de polarisation du rayonnement émis dans l’extrême ultraviolet. Comme pour la matière, le moment angulaire de la lumière peut être séparé en une composante de spin, associée à l’état de polarisation du faisceau, et une composante orbitale, reliée à la forme du front d’onde. La maitrise complète du moment angulaire des harmoniques nécessite de recourir à des schémas de génération à deux faisceaux non-colinéaires, créant un réseau de diffraction dans le milieu générateur. Nous avons montré que, bien que les règles de transfert obéissent à des lois de conservation du moment angulaire, la description fine du phénomène requiert une analyse précise du champ laser dans le milieu de génération. Ces travaux ouvrent des perspectives de mise en forme avancée des impulsions attosecondes. / High-order harmonic generation is a highly nonlinear laser-matter interaction process which allows the synthesis of sub-femtosecond pulses, also called attosecond (1 as = 10⁻¹⁸ s) pulses. My PhD is centered around the study of angular momentum transfer during this process, in order to control spatial and polarization features of the radiation which is emitted in the extreme ultraviolet. As for matter, the angular momentum of light can be divided into a spin component, associated with the beam’s polarization, and an orbital component, related to the shape of the wavefront. The control of high harmonics’ angular momentum requires generating schemes involving two crossing beams, thus creating a diffraction grating in the generating medium.We have shown that, although the transfer rules obey conservation laws of the angular momentum, the fine description of the phenomenon requires an accurate analysis of the laser field in the generation medium. This work opens the road for advanced shaping of attosecond pulses.

The physical-layer security of a line-of-sight (LOS) free-space optical (FSO) link using orbital angular momentum (OAM) multiplexing is studied. We discuss the effect of atmospheric turbulence to OAM-multiplexed FSO channels. We numerically simulate the propagation of OAM-multiplexed beam and study the secrecy capacity. We show that, under certain conditions, the OAM multiplexing technique provides higher security over a single-mode transmission channel in terms of the total secrecy capacity and the probability of achieving a secure communication. We also study the power cost effect at the transmitter side for both fixed system power and equal channel power scenarios.

The algebra of SU(2) is ubiquitous in physics, applicable both to the atomic spin states and the polarisation states of light. The method developed by Majorana and Schwinger to represent pure, symmetric spin-states of arbitrary value as a product of spin-1/2 states is a powerful tool that allows for a great conceptual and practical simplification. Foremost, it allows the representation of a qudit on the same geometry as a qubit, i.e., the Bloch sphere. An experimental implementation of the Majorana representation in the realm of quantum optics is presented. The technique allows the projection of arbitrary quantum states from a coherent state input. It is also shown that the method can be used to synthesise arbitrary interference patterns with unit visibility, and without resorting to quantum resources. In this context, it is argued that neither the shape nor the visibility of the interference pattern is a good measure of quantumness. It is only the measurement scheme that allows for the perceived quantum behaviour. The Majorana representation also proves useful in delineating uncertainty limits of states with a particular spin value. Issues with traditional uncertainty relations involving the SU(2) operators, such as trivial bounds for certain states and non-invariance, are thereby resolved with the presented pictorial solution. / <p>QC 20170428</p>

Orientador: Prof. Dr. Rodrigo Fresneda / Dissertação (mestrado) - Universidade Federal do ABC, Programa de Pós-Graduação em Matemática , 2016. / O modelo de Ponzano-Regge é um modelo de gravitação quântica em três dimensões. O principal objetivo deste trabalho é apresentar os fundamentos para construção desse modelo. Buscamos introduzir conceitos necessários para entendê-lo, abordando a teoria de representações de grupos de Lie compactos, tais como: redutibilidade de uma representação, representações de produto direto, e representações no espaço de funções. Tratamos especialmente do caso particular do grupo SU(2). Nesse contexto particular, apresentamos os símbolos 3j e 6j e suas propriedades. O modelo de Ponzano-Regge descreve uma geometria tridimensional discretizada, dada em termos de uma triangulação por simplexos (tetraedros, em três dimensões), de tal forma que o comprimento de cada aresta corresponde a uma representação irredutível do grupo de Lie SU(2). Estes tetraedros são descritos como símbolos 6j, cuja fórmula assintótica possibilita a passagem ao limite clássico, levando a uma expressão para a função de partição que representa uma soma sobre geometrias em três dimensões. / The Ponzano-Regge model is a quantum gravity model in three dimensions. The main goal of this work is to present the foundations for the construction of this model. We aim at introducing the necessary concepts to understand it, taking into account the theory of representations of compact Lie groups, such as: reducibility of representations, direct product representations, and representations in function spaces. We treat the particular case of the SU(2) group. In this special case, we present the 3j and 6j symbols and their properties. The Ponzano-Regge model describes a discretized 3-geometry, given in terms of a triangulation through simplices (tetrahedrons, in 3 dimensions), such that the length of each edge corresponds to an irreducible representation of the Lie group SU(2). These tetrahedrons are described as 6j symbols, whose asymptotic formula allows taking the classical limit, leading to an expression of the partition function that represents a sum over 3-geometries.