Zugl.: Kiel, Universiẗat, Diss., 2000.

Im Rahmen der vorliegenden Arbeit ist es erstmals gelungen, mit einem ps-Pumplaser (10 ps) Weißlicht mit einer spektralen Breite von mehr als einer optischen Oktave in einer mikrostrukturierten Faser (MSF) bei einer Pumpwellenlänge von 1064 nm zu generieren. Es ließ sich, abgesehen von nichtkonvertierten Resten der Pumpstrahlung, ein unstrukturiertes und zeitlich stabiles Weißlichtspektrum von 700 nm bis 1650 nm generieren. Die maximale Ausgangsleistung dieser Weißlichtstrahlung betrug 3,1 W. Es konnten sehr gute Einkoppeleffizienzen von maximal 62 % erzielt werden. Die an der Weißlichterzeugung beteiligten dispersiven und nichtlinear optischen Effekte, wie z.B. Selbstphasenmodulation, Vierwellenmischung, Modulationsinstabilitäten oder Solitoneneffekte, werden detailliert theoretisch untersucht und erläutert. Die Arbeit beinhaltet ebenfalls eine umfangreiche Beschreibung der Wirkungsweise und Eigenschaften von mikrostrukturierten Fasern mit einem festen Faserkern. Aufgrund der großen Variationsvielfalt des mikrostrukturierten Fasermantels und der damit verbundenen Wellenleitereigenschaften ergeben sich, insbesondere für die Anwendung in der nichtlinearen Optik, eine Reihe von interessanten Eigenschaften. Es wurden insgesamt vier verschiedene mikrostrukturierte Fasern experimentell untersucht. Für die Interpretation der experimentellen Ergebnisse ist die Pulsausbreitung der ps-Pumppulse in einer dispersiven, nichtlinear optischen Faser anhand der verallgemeinerten nichtlinearen Schrödinger-Gleichung berechnet worden. Durch einen Vergleich der Berechnungen mit den Messdaten ließen sich verstärkte Modulationsinstabilitäten und verschiedene Solitoneneffekte als hauptsächlich für die Weißlichterzeugung bei ps-Anregungspulsen verantwortlich identifizieren. Auf der Basis der durchgeführten Untersuchungen wurde in Kooperation mit der Fa. Jenoptik Laser, Optik, Systeme GmbH eine kompakte und leistungsstarke Weißlichtquelle entwickelt. Diese wurde erfolgreich in einer Kohärenztomographiemessung (Optical Coherence Tomography - OCT) getestet: Es konnte in ex vivo-Untersuchungen gezeigt werden, dass sich mit dieser ps-Weißlichtquelle eine hohe Eindringtiefe von ca. 400 µm in die Netzhaut eines Affen erreichen lässt. / With the present work it succeeded for the first time to generate white-light with a spectral width of more than an optical octave in a microstructured fiber (MSF) with a pump wavelength of 1064 nm and ps-pump pulses (10 ps). Apart from non-converted remainders of the pumping radiation, an unstructured and temporally stable white-light spectrum from 700 nm to 1650 nm could be generated. The maximum output power of this white-light radiation amounted to 3.1 W. Very good coupling efficiencies of max. 62 % could be obtained. At the white light generation different dispersive and nonlinear optical effects took part, e.g. self-phase modulation, four-wave mixing, modulation instabilities and soliton effects. These processes are theoretically examined and described in detail. Likewise the work contained an extensive description of the principle of operation and characteristics of microstructured fibers with a solid fiber core. Due to the large variation variety of the microstructured fiber cladding and the associated wave-guiding characteristics arise, in particular for application in the nonlinear optics, a set of interesting properties. Altogether four different microstructured fibers were experimentally examined. For the interpretation of the experimental results the pulse propagation of ps-pump pulses in a dispersive, nonlinear optical fiber was computed on the basis of the generalized nonlinear Schroedinger equation. By a comparison of the calculation results with the measuring data amplified modulation instabilities and different soliton effects could be identified as main responsible for the white light generation with ps-pump pulses. With respect to the accomplished experimental and theoretical investigations in co-operation with the company Jenoptik laser, optics, systems GmbH a compact and high-performance white-light source was developed. This broadband light source was tested successfully in an optical coherence tomography measurement (OCT): It could be shown in ex vivo investigations that with this white-light source high penetration depths of approx. 400 µm into the retina of a monkey could be achieved.

No description available.

Photoinduced atom transfer radical polymerization (ATRP) was achieved using a simple household fluorescent lamp as the light source. In solution, methyl methacrylate could be polymerized to welldefined polymers; the photoinduced ATRP system did only convert monomers during irradiation and was inactive in the dark. In situ monitoring by UV-vis spectroscopy revealed the photoredox cycle between Cuᶦᶦ and Cuᶦ species. The linear development of the polymer number average molar mass with monomer conversion, the low dispersity as well as chain extension experiments showed the controlled nature of the polymerization. Photoinduced ATRP was also used to prepare homo- and block copolymer brushes and patterned brushes on surfaces by photoinduced surface-initiated ATRP (PSI-ATRP).

The use of supercontinuum light sources in different optical measurement methods, like microscopy or optical coherence tomography, has increased significantly compared to classical wideband light sources. The development of various optical measurement techniques benefits from the high brightness and bandwidth, as well as the spatial coherence of these sources. For some applications, only a portion of the broad spectral range can be used. Therefore, an increase of the spectral power density in limited spectral regions would provide a clear advantage over spectral filtering. This study describes a method to increase the spectral power density of supercontinuum sources by amplifying the excitation wavelength inside a nonlinear photonic crystal fiber (PCF). An ytterbium doped photonic crystal fiber was manufactured by a nanopowder process (drawn by the company fiberware) and used in a fiber amplifier setup as the nonlinear fiber medium. In order to characterize the fiber’s optimum operational characteristics, group-velocity dispersion (GVD) measurements were performed on the fiber during the amplification process. For this purpose, a notch-pass mirror was used to launch the radiation of a stabilized laser diode at 976 nm into the fiber sample for pumping. The performance of the fiber was compared with a conventional PCF. Finally, the system as a whole was characterized in reference to common solid state-laser-based photonic supercontinuum light sources. An improvement of the power density up to 7.2 times was observed between 1100 nm to 1380 nm wavelengths.

Supercontinuum light sources provide a high power spectral density with a high spatial coherence. Coherent octavespanning supercontinuum can be generated in photonic crystal fibers (PCFs) by launching short pulses into the fiber. In the field of optical metrology, these light sources are very interesting. For most applications, only a small part of the entire spectrum can be utilized. In biological tissue scattering, absorption and fluorescence limits the usable spectral range. Therefore, an increase of the spectral power density in limited spectral regions would provide a clear advantage over spectral filtering. This study describes a method to increase the spectral power density of supercontinuum sources by amplifying the excitation wavelength inside a nonlinear photonic crystal fiber (PCF). An all-fiber-based setup enables higher output power and power stability. An ytterbium-doped photonic crystal fiber was manufactured by a nanopowder process (drawn by the fiberware GmbH, Germany) and used in a fiber amplifier setup as the nonlinear fiber medium. In order to characterize the fiber’s optimum operational characteristics, group-velocity dispersion (GVD) measurements were performed. The performance of the fiber-based setup was compared with a free space setup. Finally, the system as a whole was characterized in reference to common solid state-laser-based supercontinuum light sources. An improvement of the power density was observed in the spectral range between 1100 nm to 1400 nm.

Helmholtz Zentrum Berlin (HZB) baut seit 2011 eine Testanlage Energy Recovery Linac (ERL) Project – BERLinPro. Das Ziel dieses Projektes ist den hohen Strom und hohe Brillanz von dem Elektronenstrahl in einem ERL zu demonstrieren. Die angestrebten Strahlparameter sind vergleichbar mit den Parametern von e.g. zukünftigen ERL-basierten Lichtquellen. Eine von solchen Anlagen ist Femto-Science Factory (FSF), die am HZB konzipiert wurde. FSF ist eine Lichtquelle in Röntgenbereich auf Basis von einem mehrumläufigen ERL mit zweistüfiger Injektion und Energie von einigen GeV. Die Quelle soll Diffraktionslimitiert sein und kurze (Femtosekundenbereich) Lichtpulse erzeugen. Die durchschnittliche und spitzen- Brillanz soll mindesten eine Größenordnung höher liegen als die Brillanz der modernen Speicherring-basierten Lichtquellen. Ein Überblick von BERLinPro und FSF ist gegeben. Eine potentielle Schwäche von ERL besteht in Strahlinstabilitäten, insbesondere regenerative Beam Break Up (BBU). Die Instabilität kann den erreichbaren durchschnittlichen Strom in einem ERL begrenzen. Der Grenzstrom von der BBU für BERLinPro ist berechnet in der Dissertation. Vergleich von zwei Linacs mit zwei verschiedenen supraleitenden Kavitätendesigns ist vorgestellt. Drei Methoden für Strahlstabilisierung (Einfluss von Strahlrotation mit einem Soleniod, Pseudoreflektor, und Tripleten von Quadrupolen in dem Linac auf den Grenzstrom) sind untersucht. Analytische Lösungen für die Twiss-Parameter wurden gefunden für die beste Linacoptik mit und ohne zusätzliche optische Elemente. Zukünftige große ERLs können unterschiedliche Beschleunigungsschemen benutzen. Diese Dissertation vergleicht drei Schemas: unmittelbare Injektion in einen 6 GeV Linac; zweistufige Injektion in einen 6 GeV Linac; und zweistufige Injektion in einen mehrumläufigen Beschleuniger mit geteiltem Hauptlinac in zwei 1 GeV Linacs. Der Basis für den Vergleich ist die Vollkostenanalyse sowie erreichbarer Grenzstrom von den Instabilitäten. / In January 2011 Helmholtz-Zentrum Berlin officially started the realization of the Berlin Energy Recovery Linac (ERL) Project – BERLinPro. The goal of this compact ERL is to develop the accelerator physics and technology required to accelerate a high-current (100 mA) low emittance beam. The parameters are desired for future large scale facilities based on ERLs, e.g. ERL-based synchrotron light sources. One of such large scale facilities is in the design phase at Helmholtz-Zentrum Berlin. This facility is called Femto-Science Factory (FSF). It is a GeV-scale multi-turn ERL-based light source. This light source will operate in the diffraction limited regime for X-rays and offer a short length of a light pulse in the femtosecond region. The average and peak brightness will be at least an order of magnitude higher than achievable from storage rings. In this work an overview of these two projects is given. One potential weakness of the Energy Recovery Linacs is a regenerative form of BBU – transverse beam break up instability. This instability can limit a beam current. In this work the threshold current of the BBU instability was calculated for BERLinPro. The comparison of two linacs based on different types of superconducting cavities is made. Different methods of BBU suppression are investigated (e.g. the influence of solenoid, pseudo-reflector and quadruple triplets in the linac structure on the BBU threshold). Analytic solutions of the Twiss parameters are used to find the best optic in the linac with and without external focusing are presented. Large scale ERL facilities can be realized on different schemes of beam acceleration. This dissertation compares a direct injection scheme with acceleration in a 6 GeV linac, a two-stage injection with acceleration in a 6 GeV linac and a multi-turn (3-turn) scheme with a two-stage injection and two main 1 GeV linacs. The key points of the comparison were total costs and BBU instability. Linac optic solutions are presented.

Optical coherence tomography benefits from the high brightness and bandwidth, as well as the spatial coherence of supercontinuum (SC) sources. The increase of spectral power density (SPD) over conventional light sources leads to shorter measuring times and higher resolutions. For some applications, only a portion of the broad spectral range can be used. Therefore, an increase of the SPD in specific limited spectral regions would provide a clear advantage over spectral filtering. This study describes a method to increase the SPD of SC sources by amplifying the excitation wavelength inside of a nonlinear photonic crystal fiber (PCF). An ytterbium-doped PCF was manufactured by a nanopowder process and used in a fiber amplifier setup as the nonlinear fiber medium. The performance of the fiber was compared with a conventional PCF that possesses comparable parameters. Finally, the system as a whole was characterized in reference to common solid-state laser-based photonic SC light sources. An order-of-magnitude improvement of the power density was observed between the wavelengths from 1100 to 1350 nm.