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Studies of Nuclear Resonance Fluorescence Excitations Measured with LaBr3(Ce)detectors for Nuclear Security Applications / 核セキュリティ応用のためのLaBr3(Ce)検出器による核共鳴散乱測定に関する研究Abdelsanad, Mohamed Omer Nagy 24 September 2013 (has links)
京都大学 / 0048 / 新制・課程博士 / 博士(エネルギー科学) / 甲第17918号 / エネ博第290号 / 新制||エネ||60(附属図書館) / 30738 / 京都大学大学院エネルギー科学研究科エネルギー応用科学専攻 / (主査)教授 大垣 英明, 教授 白井 康之, 教授 松田 一成 / 学位規則第4条第1項該当 / Doctor of Energy Science / Kyoto University / DGAM
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The design of a mobile synthetic aperture collimated gamma detector for passive HEU sourcesChin, Michael Raymond 13 January 2014 (has links)
This thesis covers the individual work of Michael Chin as part of the sponsored research project funded by the U.S. State Department in support of a computational design of a "Mobile Pit Verification System" (MPVS), a mobile “drive by” passive radiation detection system to be applied in special nuclear materials (SNM) storage facilities for validation and compliance purposes. The MPVS system is intended to enable a comprehensive, rapid verification and validation of stored nuclear weapon core physics packages containing SNM, or so-called “weapon pits,” in weapon materials and stockpile storage facilities. The MPVS platform is designed to move at a constant speed and accumulate a signal for each stored weapon pit container. The gamma detector was selected to be a 4 × 4 × 8 cubic inch CsI detector while the neutron detector array designed for the “Transport Simulation and Validation of a Synthetic Aperture SNM Detection System (“T-SADS”) project was used in conjunction with this work; T-SADS was a 3 year project funded by DOE-NNSA which was completed on May 2013.
The computational design effort for this project was completed in April 2013, and leveraged novel computational radiation transport methods, algorithms, and SNM identification methods, including a synthetic aperture collection approach, and a new gamma ratio methodology for distinguishing between naturally occurring radiation materials and weapon class SNM materials. Both forward and adjoint transport methods were utilized to characterize the adjoint reaction rate as a function of inter-source spacing, collimation thickness, linear and angular field of view, source age, source type, source geometry, and mobile platform speed. The integrated count was then compared with background radiation and the associated probabilities of detection and false alarm were then computed.
Publications resulting from this research were published in PHYSOR 2012, presented at the 53rd annual Proceedings of the INMM, and at the Mathematics & Computation 2013 Conference.
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Safeguards for Uranium Extraction (UREX) +1a ProcessFeener, Jessica S. 2010 May 1900 (has links)
As nuclear energy grows in the United States and around the world, the expansion
of the nuclear fuel cycle is inevitable. All currently deployed commercial reprocessing
plants are based on the Plutonium - Uranium Extraction (PUREX) process. However,
this process is not implemented in the U.S. for a variety of reasons, one being that it is
considered by some as a proliferation risk. The 2001 Nuclear Energy Policy report
recommended that the U.S. "develop reprocessing and treatment technologies that are
cleaner, more efficient, less waste-intensive, and more proliferation-resistant." The
Uranium Extraction (UREX+) reprocessing technique has been developed to reach these
goals. However, in order for UREX+ to be considered for commercial implementation, a
safeguards approach is needed to show that a commercially sized UREX+ facility can be
safeguarded to current international standards.
A detailed safeguards approach for a UREX+1a reprocessing facility has been
developed. The approach includes the use of nuclear material accountancy (MA),
containment and surveillance (C/S) and solution monitoring (SM). Facility information
was developed for a hypothesized UREX+1a plant with a throughput of 1000 Metric
Tons Heavy Metal (MTHM) per year. Safeguard goals and safeguard measures to be
implemented were established. Diversion and acquisition pathways were considered;
however, the analysis focuses mainly on diversion paths. The detection systems used in
the design have the ability to provide near real-time measurement of special fissionable
material in feed, process and product streams. Advanced front-end techniques for the
quantification of fissile material in spent nuclear fuel were also considered. The
economic and operator costs of these systems were not considered. The analysis shows
that the implementation of these techniques result in significant improvements in the
ability of the safeguards system to achieve the objective of timely detection of the diversion of a significant quantity of nuclear material from the UREX+1a reprocessing
facility and to provide deterrence against such diversion by early detection.
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