Polychlorinated biphenyls (PCBs) are a group of 209 persistent organic pollutants, whose documented carcinogenic, neurological and respiratory toxicities are expansive and growing. Existing inhalation estimates demonstrate ubiquitous exposure to World Health Organization (WHO) indicator PCBs and limited other PCB congeners in North America and Europe. However, inhalation exposure estimates of most lower-chlorinated congeners are lacking, and continuing release of PCBs from urban areas demands location-specific assessments of PCB exposure in ambient air and contaminated environments. Using paired indoor and outdoor airborne PCB measurements and activity questionnaires from the AESOP Study, we assess congener-specific exposure rates for adolescent children and their mothers in East Chicago, Indiana and Columbus Junction, Iowa. Our cohorts of 129 (EC) and 135 (CJ) and our detection of 202 individual congeners and coelutions allows unprecedented quantification of congener-specific inhalation exposure, which we compare to dietary exposure using Total Diet Survey PCB concentrations. ∑PCB inhalation is greater for children than for their mothers in both locations, and is greater for East Chicago mothers and children than for Columbus Junction mothers and children, respectively. Schools attended by AESOP Study children have higher indoor PCB concentrations than do homes, and contribute to more than half of children's inhalation PCB exposure. Inhalation of the potentially neurotoxic congeners PCB 11, 40/41/71, and 51 was apparent among individuals at each location. Additional, congener-specific and biological inferences are possible via comparison with sera-based PCB concentrations for these cohorts.

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En nedgång har setts i Sverige och Europa när det gäller luftföroreningar de senast årtiondena. Nedgången beror bland annat på minskade emissioner från industrier, övergång från uppvärmning med olje- och kolpannor till fjärrvärme och förbättrad bränslekvalitet. Denna studie utvärderar lufthalts- och nedfallsmätningar gjorda i närheten av pappers- och massaindustrin Korsnäs i Gävle. Mätserierna startar vid sent 1970-tal och går fram till årsskiftet 2009/2010. Nedfall av stoft, sulfat, natrium, kalcium och lufthalter av svaveldioxid samt sot studerades. Jämförelser gjordes med Korsnäs miljöförbättrande åtgärder och emissioner under tidsperioden och med andra mätningar gjorda i Sverige och Gävleborgs län. Studien visade en nedgång av svaveldioxidhalterna i luften. Detta stämmer bra med en kraftig reduktion av svavelemissionerna från fabriksområdet under tidigt 1990-tal då installationer av reningsanläggningar skedde på de största emissionskällorna av svaveldioxid. En minskning av svavelhalten i eldningsoljan från Karskär Energi AB, ett energikombinat ägt av Korsnäs på samma fabriksområde, bidrog under samma tidperiod även till emissionsminskningen. Sothalten visade ingen nedåtgående trend under perioden men var säsongsberoende med i genomsnitt högre halter på vinterhalvåret. Troligtvis berodde detta på förbränningsanläggningar i närområdet, så som enskild förbränning och Karskär Energi AB. Fördelning av de högsta lufthalterna visade inte högre halter av svaveldioxid och sot när medelvindriktningen var ostlig och därmed blåste från fabriksområdet mot mätstationen utan när vindriktningen var sydvästlig och blåste från inlandet. Det totala stoft- och kalciumnedfallet visade ingen nedgång men hade i genomsnitt högre uppmätta halter på sommarhalvåret. Sulfatnedfallet visade högre halter under sent 1980-tal för att därefter minska och natriumnedfallet minskade något under perioden. Inga tydliga kopplingar kunde ses mellan lufthalter respektive nedfall och emissionerna från fabriksområdet när dataserierna sorterades efter vindriktning, vindhastighet och efter sommar- respektive vinterhalvår. Nedfall och lufthalter var inte högre, förutom för svaveldioxid, när jämförelser gjordes med andra mätningar i Sverige och Gävleborgs län och samtliga mätningar låg under periodens gällande nationella gränsvärden. / A decline has been seen in Sweden and Europe when it comes to air pollution the last decades. The decline is partly due to reduced emissions from industries, switching from heating using oil and coal boilers to district heating and better fuel quality. This study evaluates deposition and air concentration measurements made in the vicinity of the pulp and paper industry Korsnäs in Gävle. The measurement series starts at the late 1970s and goes up to year-end 2009/2010. Deposition of dust, sulphate, sodium, calcium and air concentrations of sulphur dioxide and soot were studied. Comparisons were made with Korsnäs environmental measures and emissions during the same time period and with other measurements made in Sweden and Gävleborgs County. The study showed a decrease in sulphur dioxide concentrations in the air. This fits well with a major reduction of sulphur emissions from the factory area in the early 1990s when installations of treatment plants were made at the largest emission sources of sulphur dioxide. Reducing the sulphur content of fuel oil from Karskär Energi AB, an energy combine owned by Korsnäs in the same factory area, contributed to the decrease during the same time period. Air concentrations of soot showed no downward trend over the years, but were seasonal, with higher average soot concentrations in the winter. This was most likely caused by the burning of fuel oil from both the private sector and Karskär Energi AB. The largest air concentrations did not show higher levels of sulphur dioxide and soot when the mean wind direction was easterly and thus blew from factory area toward the monitoring station but when the wind direction was southwesterly and blew from inland. The total dust and calcium deposition showed no decline but had higher average measured levels in the summer. Sulphate deposition showed high levels during the late 1980s but has thereafter decreased. The sodium deposition decreased a little during the time period. No clear connection was found between deposition/air concentrations and emissions from the factory area when the data series were sorted by wind direction, wind speed and after the summer and winter months. Depositions and air concentrations were not higher except for sulphur dioxide when the comparison was made with other measurements in Sweden and Gävleborg County. All measurements were below the then current national limits.