This thesis presents a theoretical study of the collective effects of a large number of photon emitters coupled to optical cavities. The ensemble effects are accounted for by considering both the light emitting and scattering by the photon emitters. It suggests that, to correctly estimate the emitters ensemble coupled cavity mode, it is necessary to consider the existence of the excited excitons ensemble and optical pumps. This thesis shows that optical pumps can excite more excitons and scattering channels as pumping power increases. The change in exciton population can lead to comprehensive spectral behaviors by changing the cavity spectral shapes, bandwidth and resonance positions, through the inhomogeneous broadening and frequencies repulsion effects of collective emissions. The existence of the exciton ensemble can also enhance optical coupling effects between target excitons and the cavity mode. The target exciton, which has a relatively large coupling strength and is close to the cavity peak, can affect the properties of the background dipoles and their coupling to the cavity. All these collective effects are sensitive to the number, the resonances distribution, and the optical properties of the background excitons in the frequency domain and the property of the target exciton, if any. This study provides a perspective on the control of the optical properties of cavities and individual excitons through collective excitation. / Thesis (Master, Physics, Engineering Physics and Astronomy) -- Queen's University, 2012-07-30 14:51:15.914

Thesis (M.S.)--Miami University, Dept. of Physics, 2009. / Title from first page of PDF document. Includes bibliographical references (p. Xx-Xx).

Dans cette thèse, nous étudions d’un point de vue théorique les propriétés physiques de nanostructures couplées à des cavités micro-ondes. L’électrodynamique quantique (QED) en cavité en présence d’une boîte quantique s’est révélée être une technique expérimentale puissante, permettant d'étudier cette dernière par des mesures photoniques en plus des mesures de transport électronique conventionnelles. Dans cette thèse, nous proposons d'utiliser le champ micro-ondes de la cavité afin d’extraire des informations supplémentaires sur les propriétés des conducteurs quantiques : le coefficient de transmission optique est directement lié à la susceptibilité électronique de ces conducteurs quantiques. Nous appliquons ce cadre général à différents systèmes mésoscopiques couplés à une cavité supraconductrice micro-ondes comme  une jonction tunnel, une boîte quantique couplée à des réservoirs, un fil topologique et un anneau supraconducteur. La QED en cavité peut être utilisée pour sonder, par l'intermédiaire de mesures photoniques, la dépendance en fréquence de l’admittance du puits quantique couplé à la cavité micro-ondes. En ce qui concerne le fil topologique, nous avons montré que la cavité permet de caractériser la transition de phase topologique, l'émergence de fermions de Majorana, ainsi que la parité de l'état fondamental. Pour l'anneau supraconducteur, nous étudions par l'intermédiaire de la réponse optique de la cavité l’effet Josephson et le passage à l'effet Josephson fractionnaire, qui est associé à l'apparition de fermions de Majorana dans le système. Le cadre théorique proposé dans cette permet de sonder de manière non-invasive un large éventail de nanostructures, des boîtes quantiques aux supraconducteurs topologiques. En outre, il donne de nouvelles informations sur les propriétés de ces conducteurs quantiques, informations non accessibles via des expériences de transport. / In this thesis, we study theoretically various physical properties of nanostructures that are coupledto microwave cavities. Cavity quantum electrodynamics (QED) with a quantum dot has been proven to be a powerful experimental technique that allows to study the latter by photonic measurements in addition to electronic transport measurements. In this thesis, we propose to use the cavity microwave field to extract additional information on the properties of quantum conductors: optical transmission coefficient gives direct access to electronic susceptibilities of these quantum conductors. We apply this general framework to different mesoscopic systems coupled to a superconducting microwave cavity, such as a tunnel junction, a quantum dot coupled to the leads, a topological wire and a superconducting ring. Cavity QED can be used to probe the finite frequency admittance of the quantum dot coupled to the microwave cavity via photonic measurements. Concerning the topological wire, we found that the cavity allows for determining the topological phase transition, the emergence of Majorana fermions, and also the parity of the ground state. For the superconducting ring, we propose to study the Josephson effect and the transition from the latter to the fractional Josephson effect, which is associated with the emergence of the Majorana fermions in the system, via the optical response of the cavity. The proposed framework allows to probe a broad range of nanostructures, including quantum dots and topological superconductors, in a non-invasive manner. Furthermore, it gives new information on the properties of these quantum conductors, which was not available in transport experiments.

<p>Due to the rapid development of nanophotonics, microring resonators suspended on a membrane holds promises for a scalable optical circuit with strong light-atom interaction. In this dissertation, I introduce a efficiently-coupled microring circuits for on-chip cavity QED with cold atoms and report my experimental efforts to integrate the optical chip into a ultrahigh-vacuum chamber with a magneto-optical trap for Rb atoms. My attempts to load single atoms into optical tweezers are also discussed.</p> <p>  </p> <p>  Although the loading of atom into optical tweezers above the top surface of resonator remains a challenge in experiment, I propose an alternative of cavity cooling based on cavity QED to facilitate the loading of atom into a two-color evanescent field trap around the waveguide. Assuming that the strong interaction between atoms and resonator modes is realized, I theoretically investigate the synthesis via photoassociation and the direct optical detection of a single ground-state cold molecule, whose corresponding excited-state has multiple decay channels. Similarly to the Purcell effect, the decay in a specific decay channel could be enhanced based on cavity QED, and therefore the synthesis efficiency can approach unity when the interaction between the resonator modes and a single cold molecule becomes stronger. In addition, for a single cold molecule without closed optical transition, the electromagnetically induced transparency is possible to be observed on our nanophotonic platform in the case of strong resonator-molecule coupling.</p>

Diese Arbeit beschreibt eine ausfŸhrliche Untersuchung der physikalischen Eigenschaften von Mikrokugelresonatoren aus Quarzglas. Diese Resonatoren unterstŸtzen sogennante whispering-gallery Moden (WGM), die GŸten so hoch bis 109 bieten. Als experimentelle Hilfsmittel wurden ein Nahfeld- und ein Konfokalmikroskop benutzt, um die Struktur der Moden bezŸglich der Topographie des Resonators eindeutig zu identifizieren, oder um einzelne Quantenemitter zu detektieren und anzuregen. Die resonante †berhšhung des elektromagnetischen Feldes in den Moden des Resonators wurde ausgenutzt, um stimulierte Raman-Streuung mit extrem niedrigem Schwellenwert im Quarzglas zu beobachten. Ein Rekordschwellenwert von 4.5 Mikrowatts wurde gemessen. Mittels einer Nahfeldsonde wurde die Modenstruktur des Mikro-Ramanlasers gemessen. Mikroresonatoren stellen einen Grundbaustein der Resonator-Quantenelektrodynamik dar. In dieser Arbeit wurde die Kopplung von einem einzelnen strahlenden Dipol an die WGM sowohl theoretisch als auch experimentell untersucht. Die kontrollierte Kopplung von einem einzelnen Nanoteilchen an die WGM eines Mikrokugelresonators wurde nachgewiesen. Erste Ergebnisse in der Kopplung eines einzelnen Emitters an die Moden des Resonators wurden erzielt. Die resonante Wechselwirkung mit Resonatormoden wurde ausgenutzt, um den Photonentransfer zwischen zwei Nanoteilchen dramatisch zu verstŠrken. Schlie§lich wurde die bislang unbeachtete Analogie zwischen dem Quantensystem eines einzelnen Emitters in Wechselwirkung mit einer einzelnen Resonatormode und dem klassischen System zweier gekoppelten Moden experimentell untersucht. Es wurde bewiesen, wie die aus der Resonatorquantenelektrodynamik bekannten Kopplungsregime der starken und schwachen Kopplung in Analogie auch an einem klassischen System beobachtet werden kšnnen. Der †bergang von schwacher zu starker Kopplung wurde beobachtet, und bislang gemessene unerwartet hohe Kopplungsraten konnten einfach erklŠrt werden. / This work presents an extensive study of the physical properties of silica microsphere resonators, which support whispering-gallery modes (WGMs). These modes feature Q-factors as high as 109 corresponding to a finesse of 3 millions for spheres with a diameter of about 80 micrometers. These are to date among the highest available Q-factors, leading to cavity lifetimes of up to few microseconds. A near-field microscope and a confocal microscope are used as tools to unequivocally identify the mode structure related to the sphere topography, and for excitation and detection of single quantum emitters. The high field enhancement of the cavity modes is exploited to observe ultra-low threshold stimulated Raman scattering in silica glass. A record ultra-low threshold of 4.5 microwatts was recorded. The mode structure of the laser is investigated by means of a near-field probe, and the interaction of the probe itself with the lasing properties is investigated in a systematic way. Microcavities also one of the building blocks of Cavity QED. Here, the coupling of a radiative dipole to the whispering-gallery modes has been studied both theoretically and experimentally. The controlled coupling of a single nanoparticle to the WGMs is demonstrated, and first results in coupling a single quantum emitter to the modes of a microsphere are reported. The resonant interaction with these modes is exploited to enhance photon exchange between two nanoparticles. Finally a novel analogy between a system composed of a single atom interacting with one cavity mode on one side and intramodal coupling in microsphere resonators induced by a near-field probe on the other side is presented and experimentally explored. The induced coupling regimes reflect the different regimes of weak and strong coupling typical of Cavity QED. The transition between the two coupling regimes is observed, and a previously observed unexpectedly large coupling rate is explained.

Devices that exploit the properties of quantum mechanics for their operation can offer unique advantages over their classical counterparts. Interference of matter waves can be used to dramatically increase the rotational sensitivity of gyroscopes. Complete control of the quantum evolution of a system could produce a new powerful computational device known as a quantum computer. Research into these technologies offers a deeper understanding of quantum mechanics as well as exciting new insights into many other areas of science. Currently, a limiting factor in many quantum devices using neutral atoms is accurate motional control over the atoms. This thesis describes two recent advancements in neutral atom motional control using both magnetic and electromagnetic confining fields. Part I reports on the demonstration of the first storage ring for neutral atoms. This storage ring may one day provide the basis for the world's most sensitive gyroscope. Part II describes the optical delivery of neutral atoms into the mode of a high-finesse cavity for applications in quantum computing and communication.

A neutral atom interacting with a single mode of a high finesse cavity provides an opportunity to study uncharted quantum mechanical systems and to explore the field of quantum computing and networking. Ranging from being a deterministic single photon source to a coherent storage unit for quantum information, a strong coupling cavity QED system has proven to be a powerful tool. In this thesis, single atoms are deterministically delivered over long distances and probed in an optical cavity. Once in the cavity, a single atom is stored and continuously observed for over 15 seconds. Progress towards using atoms in the cavity to produce entangled photon pairs is presented. Dual 1D optical lattices are implemented to create a foundation for advancements in two qubit quantum operations and entanglements.

One of today’s challenges to realise computing based on quantum mechanics is to reliably and scalably encode information in quantum systems. Here, we present a photon source to on-demand deliver photonic quantum bits of information based on a strongly coupled atom-cavity system. The source operates intermittently for periods of up to 100 <i>μ</i>s, with a single-photon repetition rate of 1 MHz, and an intra-cavity production efficiency of up to 85%. Our ability to arbitrarily control the photons’ wavepackets and phase profiles, together with long coherence times of 500 ns, allows to store time-bin encoded quantum information within a single photon. To do so, the spatio-temporal envelope of a single photon is sub-divided in d time bins which allows for the delivery of arbitrary qu-d-its. This is done with a fidelity of > 95% for qubits, and 94% for qutrits verified using a newly developed time-resolved quantum-homodyne measurement technique. Additionally, we combine two separate fields of quantum physics by using our deterministic single-photon source to seed linear optics quantum computing (LOQC) circuits. As a step towards quantum networking, it is shown that this photon source can be combined with quantum gates, namely a chip-integrated beam splitter, a controlled-NOT (CNOT) gate as well as a CNOT4 gate. We use this CNOT4 gate to entangle photons deterministically emitted from our source and observe non-classical correlations between events separated by periods exceeding the travel time across the chip by three orders of magnitude. Additionally, we use time-bin encoded qubits to systematically study the de- and re-phasing of quantum states as well as the the effects of time-varying internal phases in photonic quantum circuits.

Les phénomènes quantiques les plus fondamentaux comme la cohérence quantique et l’intrication sont aujourd'hui explorés pour réaliser de nouvelles technologies. C'est le domaine des technologies quantiques, qui promettent de révolutionner le calcul, la communication et la métrologie. En encodant l'information dans les systèmes quantiques, il serait possible de résoudre des problèmes inaccessibles aux ordinateurs classiques, de garantir une sécurité absolue dans les communications et de développer des capteurs dépassant les limites classiques de précision. Les photons uniques, en tant que vecteurs d'information quantique, ont acquis un rôle central dans ce domaine, car ils peuvent être manipulés facilement et être utilisés pour mettre en œuvre de nombreux protocoles quantiques. Pour cela, il est essentiel de développer des interfaces très efficaces entre les photons et les systèmes quantiques matériels, tels les atomes uniques, une fonctionnalité fondamentale à la fois pour la génération et la manipulation des photons. La réalisation de tels systèmes dans l'état solide permettrait de fabriquer des dispositifs quantiques intégrés et à large échelle. Dans ce travail de thèse, nous étudions l'interface lumière-matière réalisée par une boîte quantique unique, utilisée comme un atome artificiel, couplée de façon déterministe à une cavité de type micropilier. Un tel dispositif s'avère être un émetteur et un récepteur efficace de photons uniques, et il est utilisé ici pour implémenter des fonctionnalités quantiques de base. Tout d'abord, sous une excitation optique résonante, nous montrons comment nos composants sont des sources très brillantes de photons uniques. L’accélération de l'émission spontanée de la boîte quantique dans la cavité et le contrôle électrique de la structure permettent de générer des photons très indiscernables avec une très haute brillance. Cette nouvelle génération de sources de photons uniques peut être utilisée pour générer des états de photons intriqués en chemin appelés états NOON. Ces états intriqués sont des ressources importantes pour la détection de phase optique, mais leur caractérisation optique a été peu étudiée jusqu’à présent. Nous présentons une nouvelle méthode de tomographie pour caractériser les états de NOON encodés en chemin et implémentons expérimentalement cette méthode dans le cas de deux photons. Enfin, nous étudions le comportement de nos composants comme filtres non-linéaires de lumière. L'interface optimale entre la lumière et la boîte quantique permet l'observation d'une réponse optique non-linéaire au niveau d'un seul photon incident. Cet effet est utilisé pour démontrer le filtrage des états Fock à un seul photon à partir d’impulsions classiques incidentes. Ceci ouvre la voie à la réalisation efficace d’interactions effectives entre deux photons dans un système à l’état solide, une étape fondamentale pour surmonter les limitations dues au fonctionnement probabilistes des portes optiques linéaires. / Quantum phenomena can nowadays be engineered to realize fundamentally new applications. This is the field of quantum technology, which holds the promise of revolutionizing computation, communication and metrology. By encoding the information in quantum mechanical systems, it appears to be possible to solve classically intractable problems, achieve absolute security in distant communications and beat the classical limits for precision measurements. Single photons as quantum information carriers play a central role in this field, as they can be easily manipulated and can be used to implement many quantum protocols. A key aspect is the interfacing between photons and matter quantum systems, a fundamental operation both for the generation and the readout of the photons. This has been driving a lot of research toward the realization of efficient atom-cavity systems, which allows the deterministic and reversible transfer of the information between the flying photons and the optical transition of a stationary atom. The realization of such systems in the solid-state gives the possibility of fabricating integrated and scalable quantum devices. With this objective, in this thesis work, we study the light-matter interface provided by a single semiconductor quantum dot, acting as an artificial atom, deterministically coupled to a micropillar cavity. Such a device is shown to be an efficient emitter and receiver of single photons, and is used to implement basic quantum functionalities.First, under resonant optical excitation, the device is shown to act as a very bright source of single photons. The strong acceleration of the spontaneous emission in the cavity and the electrical control of the structure, allow generating highly indistinguishable photons with a record brightness. This new generation of single photon sources can be used to generate path entangled NOON states. Such entangled states are important resources for sensing application, but their full characterizatiob has been scarcely studied. We propose here a novel tomography method to fully characterize path entangled N00N state and experimentally demonstrate the method to derive the density matrix of a two-photon path entangled state. Finally, we study the effect of the quantum dot-cavity device as a non-linear filter. The optimal light matter interface achieved here leads to the observation of an optical nonlinear response at the level of a single incident photon. This effect is used to demonstrate the filtering of single photon Fock state from classical incident light pulses. This opens the way towards the realization of efficient photon-photon effective interactions in the solid state, a fundamental step to overcome the limitations arising from the probabilistic operations of linear optical gates that are currently employed in quantum computation and communication.

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