We are interested in the onset of instability of the axisymmetric flow between two concentric spherical shells that differentially rotate about a common axis in the narrow-gap limit. The expected mode of instability takes the form of roughly square axisymmetric Taylor vortices which arise in the vicinity of the equator and are modulated on a latitudinal length scale large compared to the gap width but small compared to the shell radii. At the heart of the difficulties faced is the presence of phase mixing in the system, characterised by a non-zero frequency gradient at the equator and the tendency for vortices located off the equator to oscillate. This mechanism serves to enhance viscous dissipation in the fluid with the effect that the amplitude of any initial disturbance generated at onset is ultimately driven to zero. In this thesis we study a complex Ginzburg-Landau equation derived from the weakly nonlinear analysis of Harris, Bassom and Soward [D. Harris, A. P. Bassom, A. M. Soward, Global bifurcation to travelling waves with application to narrow gap spherical Couette flow, Physica D 177 (2003) p. 122-174] (referred to as HBS) to govern the amplitude modulation of Taylor vortex disturbances in the vicinity of the equator. This equation was developed in a regime that requires the angular velocities of the bounding spheres to be very close. When the spherical shells do not co-rotate, it has the remarkable property that the linearised form of the equation has no non-trivial neutral modes. Furthermore no steady solutions to the nonlinear equation have been found. Despite these challenges Bassom and Soward [A. P. Bassom, A. M. Soward, On finite amplitude subcritical instability in narrow-gap spherical Couette flow, J. Fluid Mech. 499 (2004) p. 277-314] (referred to as BS) identified solutions to the equation in the form of pulse-trains. These pulse-trains consist of oscillatory finite amplitude solutions expressed in terms of a single complex amplitude localised as a pulse about the origin. Each pulse oscillates at a frequency proportional to its distance from the equatorial plane and the whole pulse-train is modulated under an envelope and drifts away from the equator at a relatively slow speed. The survival of the pulse-train depends upon the nonlinear mutual-interaction of close neighbours; as the absence of steady solutions suggests, self-interaction is inadequate. Though we report new solutions to the HBS co-rotation model the primary focus in this work is the physically more interesting case when the shell velocities are far from close. More specifically we concentrate on the investigation of BS-style pulse-train solutions and, in the first part of this thesis, develop a generic framework for the identification and classification of pulse-train solutions. Motivated by relaxation oscillations identified by Cole [S. J. Cole, Nonlinear rapidly rotating spherical convection, Ph.D. thesis, University of Exeter (2004)] whilst studying the related problem of thermal convection in a rapidly rotating self-gravitating sphere, we extend the HBS equation in the second part of this work. A model system is developed which captures many of the essential features exhibited by Cole's, much more complicated, system of equations. We successfully reproduce relaxation oscillations in this extended HBS model and document the solution as it undergoes a series of interesting bifurcations.

In this dissertation, I study a nonlinear partial differential equation, the complex Ginzburg-Landau (CGL) equation. I first employed the perturbative field-theoretic renormalization group method to investigate the critical dynamics near the continuous non-equilibrium transition limit in this equation with additive noise. Due to the fact that time translation invariance is broken following a critical quench from a random initial configuration, an independent ``initial-slip'' exponent emerges to describe the crossover temporal window between microscopic time scales and the asymptotic long-time regime. My analytic work shows that to first order in a dimensional expansion with respect to the upper critical dimension, the extracted initial-slip exponent in the complex Ginzburg-Landau equation is identical to that of the equilibrium model A. Subsequently, I studied transient behavior in the CGL through numerical calculations. I developed my own code to numerically solve this partial differential equation on a two-dimensional square lattice with periodic boundary conditions, subject to random initial configurations. Aging phenomena are demonstrated in systems with either focusing and defocusing spiral waves, and the related aging exponents, as well as the auto-correlation exponents, are numerically determined. I also investigated nucleation processes when the system is transiting from a turbulent state to the ``frozen'' state. An extracted finite dimensionless barrier in the deep-quenched case and the exponentially decaying distribution of the nucleation times in the near-transition limit are both suggestive that the dynamical transition observed here is discontinuous. This research is supported by the U. S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Science and Engineering under Award DE-FG02-SC0002308 / Doctor of Philosophy / The complex Ginzburg-Landau equation is one of the most studied nonlinear partial differential equation in the physics community. I study this equation using both analytical and numerical methods. First, I employed the field theory approach to extract the critical initial-slip exponent, which emerges due to the breaking of time translation symmetry and describes the intermediate temporal window between microscopic time scales and the asymptotic long-time regime. I also numerically solved this equation on a two-dimensional square lattice. I studied the scaling behavior in non-equilibrium relaxation processes in situations where defects are interactive but not subject to strong fluctuations. I observed nucleation processes when the system under goes a transition from a strongly fluctuating disordered state to the relatively stable “frozen” state where its dynamics cease. I extracted a finite dimensionless barrier for systems that are quenched deep into the frozen state regime. An exponentially decaying long tail in the nucleation time distribution is found, which suggests a discontinuous transition. This research is supported by the U. S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Science and Engineering under Award DE-FG02-SC0002308.

Nous présentons une étude de la dynamique de la lumière et des mesures des caractéristiques non-linéaires optiques dans le disulfure de carbone.Dans la première partie, nous calculons dans le cadre d’un modèle classique des expressions des susceptibilités non-linéaires jusqu’au cinquième ordre, en tenant compte des corrections de champ local. Nous formulons différentes hypothèses que nous confirmons ou infirmons par la mesure des indices d’absorption et de réfraction non-linéaires. Celles-ci sont obtenues en combinant deux méthodes de caractérisation des non-linéarités au sein d’un système 4fd’imagerie. L’analyse des données expérimentales utilise une méthode nouvellement développée, qui consiste à inverser numériquement, par la méthode de Newton, les solutions analytiques des équations différentielles qui décrivent l’évolution du faisceau.Dans la deuxième partie, nous observons la filamentation d’un faisceau laser à la longueur d’onde de 532 nm et en régime picoseconde. Puis nous procédons à la mesure de l’indice de réfraction non-linéaire effectif du troisième ordre n2,eff en fonction de l’intensité incidente. Par un ajustement de la courbe de saturation de l’effet Kerr,nous développons un nouveau modèle. La résolution numérique de celui-ci reproduit la filamentation observée.La dernière partie est consacrée à l’étude de la dynamique des solitons dissipatifs au sein de milieux à gains et pertes non-linéaires. La résolution numérique de l’équation complexe de Ginzburg-Landau cubique-quintique est réalisée suivant différentes configurations :soliton fondamental, dipôle, quadrupôle,vortex carré et rhombique. / We present a study of light dynamics and measurements of the nonlinear optical characteristics of carbon disulphide. In the first part, we calculate using the classical model, the nonlinear susceptibilities up to the fifth order taking into account local field corrections. We express different assumptions that we confirm or refute by measuring the nonlinear absorption coefficient and the nonlinear refractive index. The measurements are performed by means of two nonlinear characterization methods combined with an imaging 4f system. We analyse the experimental data using a newly developed method which numerically inverts the analytical solutions of the differential equations which describe the evolution of the beam, using Newton’s method. In the second part, we observe light filamentation at wavelength 532 nm, in the picoseconds regime. Then we measure the effective third order nonlinear refractive index n2,eff versus the incident intensity. By fitting the curve of the Kerr effect saturation, we develop a new model. Numerically solving this model, allows us to reproducethe experimentally observed filamentation. The last part is dedicated to the study of dissipative solitons dynamics. The complex Ginzburg-Landau equation with cubic-quintic nonlineraties is numerically solved in various configurations : soliton fundamental dipole, quadrupole, vortex and square rhombic.

Ausgedehnte dissipative Systeme können fernab vom thermodynamischen Gleichgewicht instabil gegenüber Oszillationen bzw. Wellen oder raumzeitlichem Chaos werden. Die komplexe Ginzburg-Landau Gleichung (CGLE) stellt ein universelles Modell zur Beschreibung dieser raumzeitlichen Strukturen dar. Diese Arbeit ist der theoretischen Analyse komplexer Muster gewidmet. Mittels numerischer Bifurkations- und Stabilitätsanalyse werden Instabilitäten einfacher Muster identifiziert und neuartige Lösungen der CGLE bestimmt. Modulierte Amplitudenwellen (MAW) und Super-Spiralwellen sind Beispiele solcher komplexer Muster. MAWs können in hydrodynamischen Experimenten und Super-Spiralwellen in der Belousov-Zhabotinsky-Reaktion beobachtet werden. Der Grenzübergang von Phasen- zu Defektchaos wird durch den Existenzbereich der MAWs erklärt. Mittels der selben numerischen Methoden wird Bursting vom Fold-Hopf-Typ in einem Modell der Kalziumsignalübertragung in Zellen identifiziert.

Ausgedehnte dissipative Systeme können fernab vom thermodynamischen Gleichgewicht instabil gegenüber Oszillationen bzw. Wellen oder raumzeitlichem Chaos werden. Die komplexe Ginzburg-Landau Gleichung (CGLE) stellt ein universelles Modell zur Beschreibung dieser raumzeitlichen Strukturen dar. Diese Arbeit ist der theoretischen Analyse komplexer Muster gewidmet. Mittels numerischer Bifurkations- und Stabilitätsanalyse werden Instabilitäten einfacher Muster identifiziert und neuartige Lösungen der CGLE bestimmt. Modulierte Amplitudenwellen (MAW) und Super-Spiralwellen sind Beispiele solcher komplexer Muster. MAWs können in hydrodynamischen Experimenten und Super-Spiralwellen in der Belousov-Zhabotinsky-Reaktion beobachtet werden. Der Grenzübergang von Phasen- zu Defektchaos wird durch den Existenzbereich der MAWs erklärt. Mittels der selben numerischen Methoden wird Bursting vom Fold-Hopf-Typ in einem Modell der Kalziumsignalübertragung in Zellen identifiziert.