Traditionally, adaptive optics (AO) systems for microscopy have focused on AO at the pupil plane, however this produces poor performance in samples with both spatially-variant aberrations, such as non-flat sample interfaces, and spatially-invariant aberrations, such as spherical aberration due to a difference between the sample index of refraction and the sample for which the objective was designed. Here, we demonstrate well-corrected, wide field-of-view (FOV) microscopy by simultaneously correcting the two types of aberrations using two AO loops. Such an approach is necessary in wide-field applications where both types of aberration may be present, as each AO loop can only fully correct one type of aberration. Wide FOV corrections are demonstrated in a trans-illumination microscope equipped with two deformable mirrors (DMs), using a partitioned aperture wavefront (PAW) sensor to directly control the DM conjugated to the sample interface and a sensor-less genetic algorithm to control the DM conjugated to the objective’s pupil.

The ability to perceive the dynamics of nature is ultimately limited by the temporal resolution of the instruments available. With the help of the ultrashort optical pulse, people now are able to observe and steer the electronic dynamics on the atomic scale. Meanwhile, high power attainable in such short time scale helps to boost the study of nonlinear physics. Most commercial femtosecond lasers are based on Ti:sapphire, but such systems can only be tuned in a spectral range around 800 nm. Few applications need only a single wavelength in this spectral region and pulses tunable from the UV to the IR are highly desirable. Based on the soliton characteristics of ultrashort laser pulses, we are the first ones who propose to make use of resonant dispersive waves, which are phase-matched non-solitonic linear waves, to extend the spectral tuning range of ultrashort laser without involving complicated amplifiers. Experimentally, we achieve the tuning of dispersive wave wavelengths by changing the dispersion parameters of the laser cavity, and confirm dispersive waves are ultrashort pulses under appropriate conditions. We successfully apply such a system into a multi-wavelength operation Ti:sapphire laser. The proposed idea is general, and can be applied to systems where solitons dominate, for example fiber lasers. Thanks to the newly developed novel fiber -photonic crystal fiber- we obtain widely tunable and gap-free femtosecond pulse by extending this mechanism to waveguides. This is the largest reported tuning range for efficient nonlinear optical frequency conversion obtained with such a simple and low energy laser. We apply such a Ti:sapphire laser to Raman micro-spectroscopy. Because of the different temporal behaviors of the Raman process and other parametric processes, we can efficiently separate the coherent Raman signal from the unwanted background, and obtain a high chemical contrast and high resolution image. This high repetition rate and low energy laser oscillator makes it very suitable for biological Raman micro-spectroscopy, especially living samples for which damage is a big concern.

Thesis (Ph. D.)--University of Texas at Austin, 2001. / Vita. Includes bibliographical references. Available also from UMI/Dissertation Abstracts International.

Thesis (Ph. D.)--University of Texas at Austin, 2001. / Vita. Includes bibliographical references (leaves 88-98). Available also in a digital version from Dissertation Abstracts.

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The subject of this dissertation is design, physics, and applications of organic photorefractive polymers which are a recently discovered new class of multifunctional polymeric composites suitable for real-time holographic recording. Design principles of amorphous guest-host photorefractive polymers are described, and their performance is investigated. Also, the use of these materials as recording media in dynamic holographic applications is evaluated. Diffraction efficiency of η ∼ 86%, limited only by absorption and reflection losses, two-beam coupling net gain coefficient of Γ = 200 cm⁻¹, and light-induced refractive index modulations as high as Δn =7x10⁻³ are demonstrated. Hologram growth rates of the order of 500 ms are observed with recording light intensities > 10 mW/cm² using either low-power laser diodes (675 nm) or a HeNe laser (633 nm). The materials have been synthesized that show good sensitivity in red and near-infrared part of the light spectrum. Physical mechanisms leading to high performance of photorefractive polymeric composites and the influence of the polymer composite structure on optical performance are investigated. The experimental results are compared with a phenomenological model based on Kukhtarev's equations. Experiments showing possible applications of PR polymers, such as dynamic time-average interferometry and document security verification are demonstrated.

A sodium laser guide star (LGS) adaptive optics (AO) system developed at Stewart Observatory is to be used at the 6.5m MMT. Annual measurements at Kitt Peak show that the mean mesospheric sodium column density varies from ∼2x10⁹cm⁻² (summer) to ∼5x10⁹cm⁻² (winter). The sodium column density also varies by a factor of two during a one hour period. The first simultaneous measurements of sodium LGS brightness, sodium column density and laser power were obtained. The absolute sodium return for a continuous wave circularly polarized beam is 1.2(±0.3)x10⁶ photons s⁻¹m⁻²W⁻¹ for the sodium column density of 3.7x10⁹cm⁻². Theoretical studies demonstrate that the 6.5m MMT LGS AO can provide Strehl ratios better than 0.15 and about 50% flux concentration within 0.2" aperture for 1-5.5μm under median seeing. This correction will be available for the full sky. Better Strehl and higher flux concentration can be achieved with natural guide stars, but limited sky coverage. The AO corrected field-of-view is about 60". The Arizona IR Imager and Echelle Spectrograph (ARIES) was designed to match the 6.5m MMT AO. Detection limits of more than 2 magnitude fainter can be reached with the AO over without the AO. A pre-ARIES wide field near-IR camera was designed, built and tested. The camera provides 1" images in the near-IR over an 8.5 x 8.5arcmin² field. The 10-σ detection limit with one minute exposures is 17.9 mag. in the K band. A prototype very high resolution cross-dispersed optical echelle spectrograph was designed and built to match the Starfire Optical Range 1.5m AO images. Interstellar KI 7698Å absorption lines have been detected in the spectra of αCyg and ζPer. The spectral resolution is 250.000. About 300Å wavelengths were covered in a single exposure. Total detection efficiency of 1% has been achieved. For the first time, a near-single-mode fiber with 10μm core size was applied to transmit the Mt. Wilson 100inch AO corrected beams to a spectrograph. The coupling efficiency of the fiber reached up to 70%. Spectra of αOri were recorded. The spectral resolution is 200,000. The total wavelength coverage is about 650Å per exposure.

Ever since the first laser demonstration in 1960, applications for laser systems have increased to include diverse fields such as: national defense, biology and medicine, entertainment, imaging, and communications. In order to serve the growing demand, a wide range of laser types including solid-state, semiconductor, gas, and dye lasers have been developed. For most applications it is critical to have lasers with both high optical power and excellent beam quality. This has traditionally been difficult to simultaneously achieve in semiconductor lasers. In the mid 1990's, the advent of an optically pumped semiconductor vertical-external-cavity surface-emitting laser (VECSEL) led to the demonstration of high (multi-watt) output power with near diffraction limited (TEM00) beam quality. Since that time VECSELs covering large wavelength regions have been developed. It is the objective of this dissertation to investigate and explore novel cavity designs which can lead to increased functionality in high power, high brightness VECSELs. Optically pumped VECSELs have previously demonstrated their potential for high power, high brightness operation. In addition, the "open" cavity design of this type of laser makes intracavity nonlinear frequency conversion, linewidth narrowing, and spectral tuning very efficient. By altering the external cavity design it is possible to add additional functionality to this already flexible design. In this dissertation, the history, theory, design, and fabrication are first presented as VECSEL performance relies heavily on the design and fabrication of the chip. Basic cavities such as the linear cavity and v-shaped cavity will be discussed, including the role they play in wavelength tuning, transverse mode profile, and mode stability. The development of a VECSEL for use as a sodium guide star laser is presented including the theory and simulation of intracavity frequency generation in a modified v-cavity. The results show agreement with theory and the measurement of the sodium D1 and D2 lines are demonstrated. A discussion of gain coupled VECSELs in which a single pump area accommodates two laser cavities is demonstrated and a description of mode competition and the importance of spontaneous emission in determining the lasing condition is discussed. Finally the T-cavity configuration is presented. This configuration allows for the spatial overlap of two VECSEL cavities operating with orthogonal polarizations. Independent tuning of each cavity is presented as well as the quality of the beam overlap and demonstration of Type II intracavity sum frequency generation. Future applications to this configuration are discussed in the generation of high power, high brightness lasers operating from the UV to far-infrared and even terahertz regimes.

No description available.

<p>If electronics are ever to be completely replaced by optics, a significant possibility in the wake of the fiber revolution, it is likely that nonlinear materials will play a central and enabling role. Indeed, nonlinear optics is the study of the mechanisms through which light can change the nature and properties of matter and, as a corollary, how one beam or color of light can manipulate another or even itself within such a material. However, of the many barriers preventing such a lofty goal, the narrow and limited range of properties supported by nonlinear materials, and natural materials in general, stands at the forefront. Many industries have turned instead to artificial and composite materials, with homogenizable metamaterials representing a recent extension of such composites into the electromagnetic domain. In particular, the inclusion of nonlinear elements has caused metamaterials research to spill over into the field of nonlinear optics. Through careful design of their constituent elements, nonlinear metamaterials are capable of supporting an unprecedented range of interactions, promising nonlinear devices of novel design and scale. In this context, I cast the basic properties of nonlinear metamaterials in the conventional formalism of nonlinear optics. Using alternately transfer matrices and coupled mode theory, I develop two complementary methods for characterizing and designing metamaterials with arbitrary nonlinear properties. Subsequently, I apply these methods in numerical studies of several canonical metamaterials, demonstrating enhanced electric and magnetic nonlinearities, as well as predicting the existence of nonlinear magnetoelectric and off-diagonal nonlinear tensors. I then introduce simultaneous design of the linear and nonlinear properties in the context of phase matching, outlining five different metamaterial phase matching methods, with special emphasis on the phase matching of counter propagating waves in mirrorless parametric amplifiers and oscillators. By applying this set of tools and knowledge to microwave metamaterials, I experimentally confirm several novel nonlinear phenomena. Most notably, I construct a backward wave nonlinear medium from varactor-loaded split ring resonators loaded in a rectangular waveguide, capable of generating second-harmonic opposite to conventional nonlinear materials with a conversion efficiency as high as 1.5\%. In addition, I confirm nonlinear magnetoelectric coupling in two dual gap varactor-loaded split ring resonator metamaterials through measurement of the amplitude and phase of the second-harmonic generated in the forward and backward directions from a thin slab. I then use the presence of simultaneous nonlinearities in such metamaterials to observe nonlinear interference, manifest as unidirectional difference frequency generation with contrasts of 6 and 12 dB in the forward and backward directions, respectively. Finally, I apply these principles and intuition to several plasmonic platforms with the goal of achieving similar enhancements and configurations at optical frequencies. Using the example of fluorescence enhancement in optical patch antennas, I develop a semi-classical numerical model for the calculation of field-induced enhancements to both excitation and spontaneous emission rates of an embedded fluorophore, showing qualitative agreement with experimental results, with enhancement factors of more than 30,000. Throughout these series of works, I emphasize the indispensability of effective design and retrieval tools in understanding and optimizing both metamaterials and plasmonic systems. Ultimately, when weighed against the disadvantages in fabrication and optical losses, the results presented here provide a context for the application of nonlinear metamaterials within three distinct areas where a competitive advantage over conventional materials might be obtained: fundamental science demonstrations, linear and nonlinear anisotropy engineering, and extremely compact resonant all-optical devices.</p> / Dissertation