Optical response of an active medium can substantially be modified when coherent superpositions of states are excited, that is, when systems display quantum coherence and interference. This has led to fascinating applications in atomic and molecular systems. Examples include coherent population trapping, lasing without inversion, electromagnetically induced transparency, cooperative spontaneous emission, and quantum entanglement. We study quantum coherence effects in several quantum optical systems and find interesting applications. We show that quantum coherence can lead to transient Raman lasing and lasing without inversion in short wavelength spectral regions--extreme ultraviolet and x-ray--without the requirement of incoherent pumping. For example, we demonstrate transient Raman lasing at 58.4 nm in Helium atom and transient lasing without inversion at 6.1 nm in Helium-like Boron (triply-ionized Boron). We also investigate dynamical properties of a collective superradiant state prepared by absorption of a single photon when the size of the sample is larger than the radiation wavelength. We show that for large number of atoms such a state, to a good approximation, decays exponentially with a rate proportional to the number of atoms. We also find that the collective frequency shift resulting from repeated emission and reabsorption of short-lived virtual photons is proportional to the number of species in the sample. Furthermore, we examine how a position-dependent excitation phase affects the evolution of entanglement between two dipole-coupled qubits. It turns out that the coherence induced by position-dependent excitation phase slows down the otherwise fast decay of the two-qubit entanglement. We also show that it is possible to entangle two spatially separated and uncoupled qubits via interaction with correlated photons in a cavity quantum electrodynamics setup. Finally, we analyze how quantum coherence can be used to generate continuous-variable entanglement in quantum-beat lasers in steady state and propose possible implementation in quantum lithography.

Title: The spectroscopy study of focused short-wavelength laser-matter interactions Author: Tomas Burian Department: Department of Surface and Plasma Science Supervisor: Ing. Libor Juha, CSc., Department of Radiation and Chemical Physics, Institute of Physics of the Czech Academy of Sciences, Prague Abstract: This thesis is focused on processes occurring during and immediately after an interaction of intense short-wavelength laser pulses with matter. Extreme states of matter (warm dense matter - WDM and hot dense matter - HDM), induced by EUV/SXR/X-ray lasers of two kinds, i.e., free-electron lasers (FEL) and plasma-based lasers, were investigated by emission spectroscopy over various spectral ranges and mass spectroscopic techniques. Absorption/transmission experiments revealed an effect of saturable absorption of soft X-ray laser radiation in aluminium WDM. Then, an ionisation potential depression (IPD) in dense plasmas was investigated by means of X-ray emission spectroscopy. Results obtained with the X-ray FEL-produced plasma exhibit very good agreement with computer simulations considering the Ecker-Kröll model. Analysis of optical emission spectra (OES) supports the key role played by fast recombination processes in the ablation plume created by focused short-wavelength laser beams on the solid target...

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Dans cette thèse, la dynamique de photodissociation de l'azoture de chlore (ClN3) est étudiée dans le domaine temporel par imagerie de vecteur vitesse des photofragments, spécialement du chlore et de N3. Cette imagerie résolue à l'échelle femtoseconde permet d'extraire les temps de dissociation, l'établissement temporel de la balance d'énergie de la réaction ainsi que la conservation des moments. Cette étude a permis de différencier deux domaines d'énergie: l'un menant à la formation d'un fragment N3 linéaire (étude autour de 4.5 eV d'excitation électronique) et le plus intéressant aboutissant à la formation d'un fragment N3 cyclique (autour de 6 eV). Dans une seconde étude, la dynamique de relaxation électronique du tétrathiafulvalène (C6H4S4-TTF) est étudiée autour de 4 eV par spectroscopie de masse résolue en temps ainsi que par spectroscopie de photoélectron. Les seuils d'ionisation dissociative sont extraits d'une détection en coïncidence entre les photoélectrons de seuil et les fragments ionisés réalisée sur rayonnement synchrotron. Les deux dernières expériences sont basées sur la génération d'harmoniques d'ordre élevé dans l'XUV d'une impulsion femtoseconde à 800 nm ou à 400 nm. Dans la première expérience, les harmoniques sont couplées à un imageur de vecteur vitesse en tant que rayonnement secondaire VUV. Par imagerie de photoélectron résolue en temps, nous avons révélé ainsi les dynamiques de relaxation des états de Rydberg initiée par une impulsion femtoseconde XUV à 15.5 eV dans l'argon et à 9.3 eV dans l'acétylène. Dans la seconde expérience, couramment nommée spectroscopie attoseconde, les harmoniques constituent le signal pompe sonde. Deux types de spectroscopie attoseconde ont été réalisés pour étudier la dynamique vibrationnelle de SF6: une expérience en réseau transitoire créé par deux impulsions pompe Raman avec une impulsion sonde intense générant les harmoniques à partir du réseau d'excitation et une expérience d'interférence de deux rayonnement XUV en champ lointain créés par deux impulsions sonde intenses.

Made available in DSpace on 2016-03-15T19:35:52Z (GMT). No. of bitstreams: 1 DENIS PAVEL CABEZAS HUAMAN.pdf: 1718725 bytes, checksum: b98f52c6b4dac9b37a33cc5bc62d871e (MD5) Previous issue date: 2015-03-26 / Coordenação de Aperfeiçoamento de Pessoal de Nível Superior / The project aims to study the disturbances (responses) of the low solar atmosphere caused by solar flares, using Hα, 30 THz (10 μm), UV/EUV, soft and hard X-rays observations, and a wide range of radio waves emissions (microwaves, millimeter, sub-millimeter). This set of multispectral data enabled us to (i) examine in detail various aspects of the phenomena, (ii) determine the origin of the radio emission during the gradual phase, and therefore (iii) understand the mechanism of the particles acceleration. The data we used for the completion of this study are based on Hα and 30 THz (10 μm) observations, made by the high cadence flare imaging system installed at OSM4 and CASLEO5 observatories, additionally data from HASTA (H-Alpha Solar Telescope for Argentina) telescope installed at OAFA6 observatory. In the sub-millimeter and millimeter domain at 212, 405 GHz and 45, 90 GHz, were from SST (Solar Sub-millimeter Telescope) and from POEMAS (POlarization Emission of Millimeter Activity at the Sun) solar radio telescopes, respectively. Complementary radio observations in the microwave range (0.2-15 GHz) from RSTN (Radio Solar Telescope Network) were considered. In addition, solar observations obtained by RHESSI (Reuven Ramaty High Energy Solar Spectroscopic Imager), Fermi and GOES (Geostationary Operational Environmental Satellite) satellites in X-ray channels, and from AIA (Atmospheric Imaging Assembly) and HMI (Helioseismic and Magnetic Imager) instruments, onboard the SDO (Solar Dynamics Observatory) satellite, respectively. / O trabalho tem como objetivo estudar as perturbações da baixa atmosfera solar produzidas pelas explosões solares, usando observações em Hα, 30 THz (10 μm), UV/EUV, raios X e uma ampla faixa de emissões em ondas de rádio (microondas, milimétrica, submilimétrica); com o propósito de determinar a natureza dos processos físicos envolvidos. Este conjunto de dados multiespectrais nos permitiu (i) analisar os diferentes aspectos das explosões tanto na fase impulsiva como gradual, (ii) determinar a origem da emissão em rádio durante a fase gradual, e consequentemente (iii) entender melhor os mecanismos de aceleração das partículas. Os dados em Hα e 30 THz foram fornecidos pelo sistema de aquisição de dados com alta resolução temporal, instalado nos observatórios OSM1 e CASLEO2, adicionalmente dados do telescópio HASTA (H-Alpha Solar Telescope for Argentina) instalado no observatório OAFA3. Enquanto as observações em rádio, os dados foram do rádio polarímetro POEMAS (POlarization Emission of Millimeter Activity at the Sun) nas frequências de 45 e 90 GHz, do telescópio SST (Sub-millimeter Solar Telescope) nas frequências 212 e 405 GHz, ambos instalados no CASLEO. Dados na faixa de microondas (0,2-15 GHz) obtidos pela rede RSTN (Radio Solar Telescope Network). Além disso, foram considerados observações do Sol obtidas pelos satélites RHESSI (Reuven Ramaty High Energy Solar Spectroscopic Imager), Fermi e GOES (Geostationary Operational Environmental Satellite) para raios X, e dos instrumentos AIA (Atmospheric Imaging Assembly), HMI (Helioseismic and Magnetic Imager), a bordo do satélite SDO (Solar Dynamics Observatory), respectivamente.