<p> The potential of a mode-locked semiconductor laser oscillator as a short pulse source for two-photon fluorescence microscopy is explored. Amplification of the 1075 nrn laser is performed with a single pass semiconductor optical amplifier or a ytterbium-doped fibre amplifier. The mode-locked diode oscillator amplified by the Yb-doped fibre amplifier has been shown to produce uncompressed pulses of 4-10 ps with an average power of up to ~0.8 W. Compression with a single pass modified grating pair compressor reduces the pulse duration to as short as 860 fs. The output power level can be easily scaled to higher values. </p> <p> The ability to tightly focus the Yb-doped fibre amplifier beam and semiconductor optical amplifier beam for the purpose of microscopy is studied. Results indicate that the fibre performs close to an ideal Gaussian laser beam source. The semiconductor optical amplifier beam does not focus as well. Measurements suggest that regions of the beam, when focused, do not significantly contribute to the generation of two-photon fluorescence. </p> <p> The efficiency of two-photon fluorescence generation of the two amplifiers is compared to that of the conventional two-photon excitation source: the mode-locked titanium sapphire laser. Results illustrate the need to improve certain operating parameters of the laser oscillator and two amplifiers to be considered practical for two-photon fluorescence microscopy. The mode-locked semiconductor laser oscillator amplified by the Yb-doped fibre amplifier is deemed to be close to being ready for two-photon imaging applications. </p> / Thesis / Master of Applied Science (MASc)

[pt] Esta dissertação de mestrado demonstra o princípio do funcionamento de um sistema gerador e multiplexador óptico utilizando pulsos curtos. Através do efeito de mode locked fiber ring laser pulsos curtos ópticos são gerados para taxa de repetição de 2.48 GHz ao passo que o escalonamento é atribuído ao uso de dispositivos passivos ópticos os quais compõem o conjunto experimental permitindo que a freqüência de 9.95 GHz seja atingida mediante a combinação exata das técnicas utilizadas. O coração de sistema está contido na geração e controle dos pulsos os quais determinarão a taxa de repetição em baixa freqüência e posteriormente a multiplexação através de linhas de atraso devidamente combinadas fornecerão o valor escalonado de operação de frequência. / [en] This master thesis demonstrates the principle of the functioning of an optical time domain multiplex system using short pulses. Through the effect of mode locked to fiber ring laser, optical short pulses are generated at repetition of 2.48 GHz to the step that the scheduling is attributed to the use of optic passive devices which compose the experimental setup allowing that the frequency of 9.95 GHz is reached by means of the accurate combination of the used techniques. The system heart is contained in the generation and control of the pulses which will later determine the rate of repetition in low frequency and multiplexing through lines of delay duly combined.

In this dissertation, an all-fiber-based single frequency nanosecond pulsed laser system at ~ 1918.4 nm in master-oscillator-power-amplifier (MOPA) configuration is present. The nanosecond pulse seed is achieved by directly modulating a continuous wave (CW) single frequency fiber laser using a fast electro-optical modulator (EOM) driven by an arbitrary waveform generator (AWG). One piece of single mode, large core, polarization-maintaining (PM) highly thulium-doped (Tm-doped) germanate glass fiber (LC-TGF) is used to boost the pulse power and pulse energy of these modulated pulses in the final power amplifier. This laser system can work in both high power and high energy regime: in high power regime, to the best of our knowledge, the highest average power 16 W and peak power 78.1 kW are achieved for single frequency transform-limited ~2.0 ns pulses at 500 kHz and 100 kHz repetition rate, respectively: In high energy regime, nearly 1 mJ and half mJ pulse energy is obtained for ~15 ns pulses at 1 kHz repetition rate and 5 kHz repetition rate, respectively. Theoretical modeling of the large-core highly Tm-doped germanate glass double-cladding fiber amplifier (LC-TG-DC-FA) is also present for 2&mum nanosecond pulse amplification. A good agreement between the theoretical and experimental results is achieved. The model can simulate the evolution of pump power, signal energy, pulse shape and the amplified stimulated emission (ASE) in the amplifier. It can also be utilized to investigate the dependence of the stored energy in the LC-TGF on the pump power, seed energy and repetition rate, which can be used to design and optimize the LC-TG-DC-FA to achieve higher pulse energy and average power. Two channel of high energy nanosecond pulses (at 1918.4 nm and 1938 nm) are utilized to generate THz wave in a quasi-phase-matched (QPM) gallium arsenide (GaAs) based on difference frequency generation. THz wave with ~ 5.4μW average power and ~18 mW peak power has been achieved. Besides, one model is built to simulate a singly resonated THz parametric oscillator. The threshold, the dependence of output THz energy on pump energy has been investigated through this model. One pump enhanced THz parametric oscillator has been proposed. The enhancement factor of the nanosecond pulses in a bow-tie ring cavity has been calculated for different pulse duration, cavity length and the transmission of the coupler. And the laser resonances in the ring cavity have been observed by using a piezo to periodically adjust the cavity length. We also build an all-fiber thulium-doped wavelength tunable mode-locked laser operating near 2&mum. Reliable self-starting mode locking over a large tuning range (>50 nm) using fiber taper based carbon nanotube (FTCNT) saturable absorber (SA) is observed. Spectral tuning is achieved by stretching another fiber taper. To the best of our knowledge, this is the first demonstration of an all-fiber wavelength tunable mode-locked laser near 2&mum.

The concern of this dissertation is the understanding and improvement of a class of lasers that is responsible for some of the shortest optical pulses available today. In particular, we seek ways to produce from synchronously pumped mode-locked dye laser systems, shorter pulses of higher intensity with improved pulse-to-pulse consistency. Specific topics.that are discussed herein include the study of the role of the pump pulse in synchronously pumped mode-locked lasers, the study of the pulse shaping and shortening due to an intracavity saturable absorber, and the study of a fundamental pulse train instability associated with these lasers.

A dual-wavelength mode-locked semiconductor vertical-external-cavity-surface-emitting laser is demonstrated. A semiconductor saturable absorber mirror allows for simultaneous mode locking of pulses centered at two center wavelengths with variable frequency spacing. The difference-frequency control is achieved with an intracavity etalon. Changing the finesse of the etalon enables the adjustment of the pulse duration between 6 and 35 ps. The emitted two-color pulses are modulated by a beat frequency in the terahertz range. Self-starting mode-locking with 0.8-W average output power is demonstrated.

We comprehensively investigated the concentration effect of dispersed single-walled carbon nanotubes (SWCNTs) in polymer films for being a saturable absorber (SA) to stabilize the mode locking performance of the Erbium-doped fiber laser (EDFL) pulse through the diagnosis of its nonlinear properties of SA. The measured modulation depth was 1 to 4.5% as the thickness increased from 18 to 265 £gm. We obtained the stable pulse of the mode-locked EDFL (MLEDFL) when the full-width half-maximum (FWHM) decreased from 3.43 to 2.02 ps as the concentrations of SWCNTs SA increased from 0.125 to 0.5 wt%. At constant concentration of 0.125 wt%, the similar pulse shortening effect of the MLEDFL was also observed when the FWHM decreased from 3.43 to 1.85 ps was the thickness of SWCNTs SA increased from 8 to 100 £gm. In EDFL system, we vary group-velocity dispersion (GVD) with different cavity length to achieve optical pulse compression. We got the shortest pulsewidth was 713 fs, and the time-bandwidth product (TBP) was 0.345. An in-depth study on the stable mode-locked pulse formation employing SWCNTs SA, it is possible to fabricate the SWCNT films for use in high performance MLEDFL and utilization of many other low-cost nanodevices.

The dependence of thickness and concentration product (TCP) of single-wall carbon nanotubes saturable absorber (SWCNTs SA) on stabilizing and shortening pulse width in passively mode-locked erbium-doped fiber ring laser (MLEDFL) was investigated and measured. The TCP represented the amounts of SWCNTs, which the optical beam encountered when passing through the SWCNTs SA. If the TCP was smaller than 8.25 (£gm x wt%), the spectral bandwidth was below 2 nm. The pulse shaping was dominated by its own self amplitude modulation (SAM) of SWCNTs SA. With further increasing TCP, the soliton-like ML operation was achieved and the spectral bandwidth was expanded to 6 nm. For soliton-like mode locking (ML) operation, the area theorem dominated the pulse shaping. Through area theorem analysis, the estimation of SPM increased as the TCP increased. The adequate enhanced SPM for balancing the slight negative GVD was provided to generate soliton-like ML pulses shorten the pulse width. However, as the TCP increased, the soliton pulse energy decreased. The decreasing soliton pulse energy restricted the further pulse shortening. The results showed that the dependence of the pulse energy and nonlinear self phase modulation (SPM) on TCP enabled to determine the shortest pulse width in MLEDFL based on the area theorem. At optimized TCP of 70.93 (£gm x wt%), it was found that the shortest pulse width of 418 fs. In addition, based on the estimated SPM from area theorem, the nonlinear refractive index n2 was calculated at the level of 0.4 - 1 x 10^-15 m^2/W that was close to the literature values of 10^-15 - 10^-16 m2/W. It provides another way to estimate the nonlinear refractive index except for the Z-scan measurement. We could also estimate the SPM if an active Z-scan measurement was taken to obtain the nonlinear refractive index of the sample. We realized the trend of pulse energy through few samples in MLEDFL, the behavior of pulse width could be theoretically simulated based on area theorem. Hence, with the area theorem analysis, the optimized TCP of SWCNTs SA could be simulated and estimated to generate the shortest pulse width from the trends of pulse energy and estimated SPM. The significant effect of TCP on pulse energy, SPM, pulse width, and spectral bandwidth of MLFLs suggests that the TCP represents the total amount of SWCNTs in SA, which can be used as one of key parameters for characterizing the passive MLFL pulse width. Through the study of the dependence of TCP on ML pulses in MLEDFL, it may provide a guideline to fabricate an effective SWCNTs SA to generate the shortest pulse width of the MLEDFL.

Coherent nonlinear effects such as Electromagnetically Induced Transparency (EIT), Coherent Population Trapping (CPT), and Slow light are studied in thermal Rb vapor by both continuous and pulsed laser fields. This work primarily includes three parts: (I) mode-locked rubidium laser and its applications (II) enhanced coupling between optical and sound waves in the forward direction via ultra-slow light (III) optical steering via ultra-slow light in rubidium vapor. In part(I), I describe the construction and study of a mode-locked rubidium laser operating at the Rb D1 line using an active mode-locking technique inside the laser cavity. The mode-locked laser field is used to observe coherent effects in a dense rubidium gas. In part(II), I experimentally demonstrate enhanced acoustic-optic coupling that occurs when the velocity of sound is close to the group velocity of light. Dragging of the light by effective motion of the gas in a Rb cell is the origin of enhanced coupling. Good agreement between theory and experiment is found. In part(III), I experimentally demonstrate optical beam deflection in coherently driven rubidium vapor due to the steep refraction index profile in the region of EIT.

Single-frequency and mode-locked silver film ion-exchanged glass waveguide lasers as well as all-optical clock recovery based on birefringent fiber resonators have been experimentally and theoretically studied. The theory, modeling and fabrication process of silver film ion-exchange techniques, have been discussed and presented.The UV-written gratings on both IOG-1 active and passive glass have been studied. For the first time, with a high quality narrowband grating UV-printed on the passive section of a hybrid glass, a DBR waveguide single-frequency laser is demonstrated with the linewidth less than 1 MHz and the output power of 9 mW.Novel saturable absorbers based on a fiber taper embedded in carbon nanotubes (CNTs)/polymer composite were demonstrated. The saturable absorbers were utilized to build mode-locked fiber lasers, which were studied experimentally. A mode-locked ring laser utilizing an Er-Yb-codoped glass waveguide as the gain medium was also demonstrated. In addition, short cavity mode-locked waveguide lasers with CNTs film on the top were theoretically investigated, which shows a short cavity mode-locked waveguide laser is very promising.A new concept to perform multi-channel multi-rate all-optical clock recovery based on birefringent fiber-optic waveguide resonators was discussed. The concept has been advanced to polarization-insensitive operation. The experimental results, obtained as a proof-of-concept, agree well with numerical simulations.

Yb-ion doped gain media have become the material of choice for reliable generation of ultrashort pulses at wavelength around 1 μm. At present, however, operation at high average power (>1 W) with sub-100 fs pulses still remains challenging. The efforts of developing an Yb-ion oscillator towards this goal, therefore, are the main focus of this thesis. In this work, the Yb:KGd(WO4)2 (Yb:KGW) crystals were chosen to serve as the gain media. To achieve high power operation, two fundamental issues have been carefully considered: 1) a new pumping scheme was proposed to alleviate the thermal issues in the Yb:KGW crystals; 2) a new method was introduced to characterize intracavity losses in the broadband Yb-ion oscillators. As a side effect observed during the optimization of the CW operation, simultaneous two-wavelength emission was also discussed. With the knowledge and experimental understanding of the fundamental issues in laser oscillators operated in the continuous-wave regime, the next step of this work demonstrated their operation in a pulsed regime. The dual action of the Kerr-lens and saturable absorber (KLAS) mode locking was proposed in this work and resulted in greatly enhanced laser performance. The laser delivered pulses with 67 fs duration at a repetition rate of 77 MHz. The average output power reached 3 W, which, to the best of our knowledge, is the highest average output power produced to date from the Yb-ion based bulk lasers with such a short pulse duration. The scalability of pulse energy and peak power was also demonstrated by reducing the repetition rate to either 36 MHz or 18 MHz. The cavity with the latter repetition rate produced 85 fs pulses with the pulse energy up to 83 nJ, which corresponds to a peak power as high as 1 MW. As required by many biomedical applications, the wavelength of the generated pulses (~1 μm) can be tuned in the near-infrared region by coupling them into an optical parametric oscillator (OPO). The feasibility of this approach was demonstrated in the last part of this thesis, through a thorough theoretical analysis of two OPO materials suitable for excitation at 1.04 μm.