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In dieser Arbeit werden elektronische und strukturelle Dynamiken durch Femtosekundenpuls injizierte kleine Polaronen in Lithiumniobat betrachtet, sowie die Auswirkungen auf die nichtlineare Optik mit Schwerpunkt auf die Holographie und den mittleren infraroten Spektralbereich untersucht.

Monolithic passively mode-locked colliding pulse semiconductor lasers generating pico- to sub-picosecond terahertz optical pulse trains are promising sources for future applications in ultra-high speed data transmission systems and optical measurements. However, in the absence of external synchronization, these passively mode-locked lasers suffer from large amplitude and timing jitter instabilities resulting in broad comb linewidths, which precludes many applications in the field of coherent communications and signal processing where a much narrower frequency line set is needed. In this dissertation, a novel quantum dot based coupled cavity laser is presented, where for the first time, four-wave mixing (FWM) in the monolithically integrated saturable absorber is used to injection lock a monolithic colliding pulse mode-locked (CPM) laser with a mode-locked high-Q ring laser. Starting with a passively mode-locked master ring laser, a stable 30 GHz optical pulse train is generated with more than 10 dB reduction in the RF noise level at 20 MHz offset and close to 3-times reduction in the average optical linewidth of the injection locked CPM slave laser. The FWM process is subsequently verified experimentally and conclusively shown to be the primary mechanism responsible for the observed injection locking. Other linear scattering effects are found to be negligible, as predicted in the orthogonal waveguide configuration. The novel injection locking technique is further exploited by employing optical hybrid mode-locking and increasing the Q of the master ring cavity, to realize an improved stabilization architecture. Dramatic reduction is shown with more than 14-times reduction in the photodetected beat linewidth and almost 5-times reduction in the optical linewidth of the injection locked slave laser with generation of close to transform limited pulses at ~ 30 GHz. These results demonstrate the effectiveness of the novel injection locking technique for an all-on-chip stability transfer and provides a new way of stabilizing monolithic optical pulse sources for applications in future high speed optical networks.

Orientador: Evandro Conforti / Dissertação (mestrado) - Universidade Estadual de Campinas, Faculdade de Engenharia Eletrica e de Computação / Made available in DSpace on 2018-08-08T01:55:52Z (GMT). No. of bitstreams: 1 Castelli_ClaudioSelmi_M.pdf: 2856453 bytes, checksum: 1efb001a79f5f2d885e231abadd78d1f (MD5) Previous issue date: 2007 / Resumo: Uma nova técnica de geração de sinais pulsados de microondas é desenvolvida. Baseia-se na composição de dois sinais arbitrários, um trem de pulsos ultra-rápidos e uma portadora de microondas, originados a partir de diferentes fontes e combinados no domínio óptico de forma a preservar ao máximo as características espectrais e temporais dos sinais. São apresentados os conceitos utilizados na técnica e toda a configuração empregada na sua validação experimental. Os resultados obtidos são discutidos e comparados com os sinais pulsados de microondas gerados a partir de um moderno gerador comercial. Os principais componentes utilizados são também caracterizados e propostas de melhorias são apresentadas. A forma de onda obtida a partir da técnica desenvolvida atingiu os resultados esperados / Abstract: A novel technique of pulsed microwave waveform generation has been developed. It is based on the mixture of two arbitrary signals, an ultra-fast pulse train and a microwave carrier, all generated from different sources and combined in the optical domain in order to preserve the spectral and temporal features as much as possible. The technique's concepts and the setup used for the experimental validation have been presented. The obtained results are discussed and compared to the pulsed microwave signals generated by a modern commercial microwave generator. The main components are also characterized and proposals of improvements have been presented. The waveform resulted from this developed technique reached the expected results / Mestrado / Telecomunicações e Telemática / Mestre em Engenharia Elétrica

This work is dedicated to a comprehensive experimental study on the interaction of femtosecond laser pulses with the nonlinear optical medium lithium niobate. The nonlinear optical response in the nanosecond regime was already studied extensively with a variety of techniques, whereas femtosecond pulses were mainly used in transient absorption or transient grating experiments. Naturally, the temporal resolution of these measurements depends on the pulse duration, however, dynamics during the pulse excitation were barely investigated. The motivation of this work is to widen the limits of femtosecond spectroscopy, not only to temporally resolve faster nonlinear optical processes, but further to show a sensitivity to other coupling mechanisms between the pulses and the material. Especially, the role of transient, dynamic holographic gratings is investigated with a careful determination of the pulse duration, bandwidth and frequency chirp. A basis of this work is established in the first part by studying the material response via light-induced absorption before focusing on the main topic, the pulse interaction with elementary (holographic) gratings, both self-induced and static, in the second part. By this detailed study, several features of femtosecond laser pulses, holographic gratings and the ultrafast material response can be revealed: (i) grating recording is feasible even with pulses of different frequencies, provided that their pulse duration is sufficiently short, (ii) grating based pulse coupling causes a pronounced energy transfer even in a common pump-probe setup for transient absorption measurements with (non-)degenerated frequencies, (iii) beyond expectation, oscillations in the phonon frequency range become apparent in different measurements. The presented results point towards appropriate future experiments to obtain a more consistent, microscopic model for the ultrafast response of the crystal, involving the interplay between photo-generated polarons, self-induced gratings, and phonons.

The present work broaches the physics of light-matter interaction, chiefly using nonlinear optical spectroscopy in a newly developed framework termed as Photon Management Concept. This way, existing fragments dealing with specific properties of harmonic and upconversion nanoparticles (HNPs/UCNPs) are consolidated into a full and coherent picture with the primary goal of understanding the underlying physical processes and their impact on the application side, especially in terms of imaging techniques, via suitable experimental and numerical studies. Contemporary optical setups involving contrast-enhancing agents are frequently limited in their excitation and detection configurations owing to a specialization to a select number of markers. As a result, the bandwidth of experimental methods and specimens that may be investigated is severely restricted in a large number of state-of-the-art setups. Here, an alternative approach involving HNPs and UCNPs, respectively, is presented providing an overview from their synthesis to optical characterization and to potential fields of application. Based on their inherent flexibility based on their nonlinear optical response, especially in terms of wavelength and intensity tunability, the PMC alleviates prevalent limitations by dynamically adapting the setup to a sample instead of the preliminary culling to a reduced number of eligible specimens that must not change their optical properties significantly during investigation. The use of HNPs supersedes such concerns due to their nearly instantaneously generated, strongly anti-Stokes shifted, coherent emission capable of producing radiation throughout the visible spectral range, including infrared and ultraviolet wavelengths. This way, HNPs transcend the traditional field of imaging and introduces potential applications in optomanipulation or holographic techniques. Thorough (nonlinear) optical characterization of UCNPs and alkali niobate HNP ensembles is performed to assess the fundamental physical mechanisms interwoven with numerical studies leading to their wide-ranging applicability. Final remarks show that HNPs are ideal candidates for realization of the PMC and yet hold an even further potential beyond current prospects.