Le Large Hadron Collider (LHC) au CERN (Organisation Européenne pour la Recherche Nucléaire) fonctionne depuis 2009 à la frontière franco-suisse. Cet accélérateur de particules a produit des quantités importantes de collisions proton-proton, à des énergies dans le centre de masse de 7 TeV (2010 et 2011), et 8 TeV (depuis avril 2012). L'un des buts de l'expérience Compact Muon Solenoid (CMS), qui enregistre et analyse ces collisions, est la recherche de bosons de Higgs. Dans le cadre du Modèle Standard, cette particule serait le quantum du champ de Higgs, qui permet d'expliquer le mécanisme de brisure de symétrie électrofaible. Un canal parmi les plus sensibles pour la recherche d'un boson de Higgs léger (c'est-à-dire pour des masses du boson de Higgs entre 90GeV/c2 et 150GeV/c2) au LHC est la désintégration en deux photons. En effet, la production de deux photons isolés de haute énergie dans l'état final constitue un signal clair en milieu hadronique, malgré le faible rapport d'embranchement. De plus, à ces masses, la largeur du pic en masse invariante reconstruite est dominée par la résolution du détecteur. Une compréhension fine de l'objet photon, tel que reconstruit par l'expérience, est donc un pré requis obligatoire. La première partie de mes travaux de thèse porte sur l'étude des désintégrations radiatives Z$^0 \rightarrow \mu\mu\gamma$ ces désintégrations sont la seule source de photons certifiés de haute pureté du Modèle Standard, pour laquelle l'impulsion transverse des photons est relativement proche de celle prévue pour des photons issus d'un boson de Higgs. L'étude de ces désintégrations a permis la détermination de l'échelle d'énergie différentielle des photons dans les données à 7 TeV. Elles ont également été utilisées dans les données à 8 TeV comme outil de validation des variables de forme de cluster pour les photons dans la simulation, ainsi que pour déterminer l'efficacité des critères de réjection des électrons. La deuxième partie de mes travaux de thèse traite de la recherche d'un boson de Higgs se désintégrant en deux photons. Cette recherche est effectuée en plusieurs classes d'évènements pour améliorer la sensibilité, et l'étude de cette procédure de séparation en classes est présentée. Enfin, une analyse de faisabilité de recherche d'un boson de Higgs se désintégrant en deux photons, produit lors de la désintégration d'un quark vecteur lourd à 14 TeV a été effectuée / The Large Hadron Collider (LHC) at CERN (European Organisation for Nuclear Research) has been in operation since 2009 at the border between France and Switzerland. This particle accelerator has provided a significant quantity of proton-proton collisions, at center of mass energies of 7 TeV (2010 and 2011) and 8 TeV (since April 2012). One of the purposes of the Compact Muon Solenoid (CMS) experiment, which records and analyses those collisions, is the search for Higgs bosons. In the Standard Model, this particle would be the quantum of the Higgs field, thought to explain the electroweak symmetry-breaking mechanism. One of the most sensitive channels for the search for a light Higgs boson (i.e. for masses between 90 GeV=c2 and 150 GeV=c2) at the LHC is through its decay into two photons. Indeed, the production of two highly energetic and isolated photons in the final state is a clean signal in hadronic collisions, despite the small branching ratio. Moreover, at these masses, the width of the reconstructed invariant mass peak is dominated by the detector resolution. Hence, a precise understanding of the photon object as reconstructed by the experiment is required. The first part of the work presented here is the study of radiative decays Z$^0 \rightarrow \mu\mu\gamma$ these decays are the only Standard Model source of high purity certified photons, for which the transverse momentum of the photon is relatively similar to the one of the photons coming from a Higgs boson decay. The study of these decays enables the determination of the differential photon energy scale in the 7 TeV data. These decays have also been used in the 8 TeV data as a validation tool of photon cluster shape variables in the simulation, and also as a way to determine the electron rejection criteria efficiency. The second part of the work concerns the search for a Higgs boson decaying into two photons. This search is done in several event classes in order to increase the sensitivity of the analysis, the study of the class separation procedure is presented. Finally, a benchmark study for the search for a Higgs boson decaying into two photons via vector-like top-partner decays at 14 TeV has been performed

Title: Coupling atmospheric chemistry/aerosols to regional climate models Author: Peter Huszár Department: Department of Meteorology and Environment Protection Supervisor: doc. RNDr. Tomáš Halenka, CSc. Supervisor's e-mail address: tomas.halenka@mff.cuni.cz Abstract: In this thesis, the connections between air quality and climate are studied. For this purpose, regional climate model RegCM3 and chemistry transport model CAMx has been coupled offline with one- and two-way interaction. Our work represents a first attempt to connect RegCM3 not only with CAMx, but with any other chemistry transport model. As a first step, an offline one way couple of RegCM3 and CAMx has been developed, meaning that the climate model drives the transport, emission, chemical transformation and deposition of species while the radiative feedbacks of gases and aerosols are not considered. A meteorological interface has been developed at our department in order to convert the meteorological data generated by RegCM3 to fields required by CAMx. For those parameters that are essential for CAMx but the regional climate model does not supply them, diagnostic methods were implemented into this interface. Further, it is used to calculate biogenic emissions. Regarding anthropogenic emissions, a simple utility has been developed to...

Suite à la signature du Protocole de Montréal en 1987, la concentration atmosphérique des substances destructrices d’ozone (ODS) est en baisse. La couche d’ozone montre des signes de récupération (Morgenstern et al. 2008a). Toutefois, l’émission des gaz à effet de serre (GHG) est en augmentation et devrait affecter au cours du 21ème siècle la distribution et les niveaux d’ozone dans l’atmosphère terrestre. En particulier, la modélisation du climat futur montre des signes d’accélération de la circulation de Brewer-Dobson transportant l’ozone de l’équateur vers les pôles. L’ozone est un constituant chimique important de l’atmosphère. Bien que nocif dans la troposphère, il est essentiel à la vie sur Terre grâce à sa capacité d’absorption d’une grande partie du rayonnement ultraviolet (UV) provenant du Soleil. Des modifications dans sa variabilité temporelle ou géographique impliqueraient des changements d’intensité du rayonnement UV à la surface de la Terre (Hegglin et al. (2009), Bais et al. (2011)). Le rayonnement UV à la surface affecte toute la biosphère. Les interactions entre rayonnement UV et écosystèmes terrestres et aquatiques sont nombreuses. Ces interactions ont des effets sur les cycles biogéochimiques et engendrent des rétroactions positives et négatives sur le climat (Erickson III et al., 2015a). La capture du CO2 atmosphérique par photosynthèse des plantes terrestres en est un exemple (Zepp et al., 2007a). Dans l’océan la pompe biologique du CO2 par la photosynthèse du phytoplancton est aussi directement affecté par la variabilité du rayonnement UV (Hader et al., 2007a). Pour l’homme le rayonnement UV est nécessaire car il participe à la photosynthèse de la vitamine D (Holick et al., 1980), mais une surexposition à des niveaux d’intensité élevés du rayonnement UV est la cause principale du développement de cancer de la peau (Matsumura and Ananthaswamy, 2004). L’objectif de ce travail de thèse est d’analyser l’évolution possible du rayonnement UV au cours du 21ème siècle, en particulier aux tropiques sud, dans le cadre des modifications climatiques attendues. Une première partie de ce travail consiste à modéliser le rayonnement UV en ciel clair dans les tropiques grâce au modèle TUV (Madronich et al., 1998) et à comparer les résultats aux mesures sols réalisées à la Réunion. Cette première partie permet l’utilisation future du modèle aux tropiques avec un bon niveau de confiance. La sensibilité du modèle de transfert radiatif en fonction de différents paramètres d’entrée est analysée (section efficace d’absorption de l’ozone,spectre extraterrestriel du soleil, ...). Les sorties du modèle sont ensuite validées à partir de mesures UV spectral au sol obtenues grâce à un spectromètre BENTHAM DM300n. Un filtrage ciel-clair des données au sol est opéré à partir de mesures de flux et de l’algorithme de Long and Ackerman (2000). Les projections climatiques des indices UV (Mc Kinlay and Diffey, 1987) sont réalisées par la suite. Pour cela, on utilise les sorties de plusieurs modèles de Chimie-Climat participant à l’exercice d’inter-comparaison CCMI (Chemistry Climate Model Initiative), couplées aux modèle TUV, validé en première partie dans les tropiques. L’exercice CCMI consiste à projeter le climat et la chimie Terrestre jusqu’en 2100 selon différents scénarios. Ces sorties décrivant la chimie et physique de l’atmosphère servent d’entrée au modèle de transfert radiatif, on obtient alors le rayonnement UV jusqu’en 2100 pour différents scénarios. Une première analyse comparative de l’UV obtenue pour quatre scénarios d’émissions (RCP2.6/4./6.0/8.5, Meinshausen et al., 2011) est effectuée. La fin du travail consiste à étudier l’impact des ODS, GHG et aérosols sur l’évolution du rayonnement UV au cours du 21ème siècle, avec un focus particulier sur les tropiques de l’hémisphère sud. / Following the 1987 Montreal Protocol, atmospheric concentrations of ozone-depleting substances are decreasing. The ozone layer shows signs of recovery. Nonetheless, greenhouse gases emissions (GHG) are rising et should affect the ozone distribution in the atmosphere. Ozone is an important due to his ability to absorb ultraviolet (UV) radiation. The goal of this work is to analyse the possible evolution of UV radiation through the 21st century, particularly in the tropics, for possible climate modification. The first part of this work is to UV in clear-sky in the tropics with the TUV (Madronich et al., 1998) model and to compare against ground-based observations made on Reunion Island. This validation allows the utilisation of TUV in the tropics with a good confidence level. The sensitivity of the model is analysed for multiple parameters. Modelling output is validated against spectral ground-based measurement. Climate Projection of UVI (Mc Kinlay and Diffey, 1987) are then realized with the use of output from model participating in the CCMI ( Model Initiative) exercise and the TUV model. CCMI output describes the chemistry and physics of the atmosphere through the 21st century for four climate scenarios (RCP2.6/4.5/6.0/8.5), they are used as input for the TUV model in order to obtain UV radiation. ODS, GHG and aerosols impact on UVI evolution is analysed.

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Comprendre et modéliser le comportement des matériaux sous irradiation électronique est un enjeu important pour l’industrie spatiale. La fiabilité des satellites nécessite de maîtriser et prédire les potentiels de surface s'établissant sur les diélectriques. Ce travail de doctorat a donc pour objectif de caractériser et de modéliser les différents mécanismes physiques (en surface et en volume) gouvernant le potentiel de charges dans les matériaux polymères spatiaux tels que le Téflon® FEP et le Kapton® HN. La mise au point d'un nouveau dispositif et d'un protocole expérimental a permis de corroborer l'existence d’une conductivité latérale des charges, souvent négligée dans les modèles physiques et numériques. Les études paramétriques, révélant l’influence de l’énergie et le flux des électrons incidents, ont permis de brosser un portrait des processus mis en jeu pour le transport (par saut ou par piégeage/dépiégeage) de charges en surface. A la lumière de cette étude, une conductivité équivalente est extraite, assimilant le matériau à un système prenant en compte les mécanismes de transport volumique et surfacique. L'analyse des évolutions non-monotones de potentiel mesurées sur les polymères spatiaux en condition spatiale a permis de révéler une dépendance de la conductivité volumique induite sous irradiation avec la dose reçue. L'étude paramétrique réalisée sur les mécanismes de transport en volume révèle une influence minoritaire du déplacement du barycentre de charges et du vieillissement physicochimique. Un modèle «0D» à un seul niveau de pièges, prenant en compte les mécanismes de piégeage/dépiégeage et recombinaison entre les porteurs de charges, a été développé. Ce modèle simplifié permet de reproduire qualitativement les évolutions de potentiel expérimentales en fonction du débit de dose et lors d'irradiations successives. / Charging behaviours of space dielectric materials, under electron beam irradiation, is of special interest for future spacecraft needs, since this mechanism could induce electrostatic discharges and consequently damages on the sensitive systems on board. In order to assess the risks of charging and discharging, this work aims at understanding the overall charge transport mechanisms and predicting the electrical behaviour of the insulator materials, especially Teflon® FEP and Kapton® HN. For an optimized prediction, the first part of our work is thus to check whether lateral conduction process can take place in the overall charge transport mechanism. Through the definition of a new experimental set-up and protocol, we have been able to discriminate between lateral and bulk conductivity and to reveal the presence of lateral conductivity that is enhanced by radiation ionization processes. We have been able to demonstrate as well that lateral intrinsic conductivity is enhanced with the increase current density and when approaching the sample surface. The second part of our work deals with the characterization of the electrical charging behaviour of Teflon® FEP under multi-energetic electron beam irradiation and the modelling of the overall bulk charge transport mechanisms. An experimental study on charge potential evolution as a function of electron spectrum, electric field, relaxation time, dose and dose rate, was performed. A numerical model has been developed to describe the effect of the different abovementioned mechanisms on the evolution of the surface potential. This model agrees correctly with the experimental phenomenology at qualitative level and therefore allows understanding the physical mechanisms steering charge transport in Teflon® and Kapton®.

Fundação Carlos Chagas Filho de Amparo a Pesquisa do Estado do Rio de Janeiro / A formulação explícita matricial desenvolvida nesta tese de doutorado foi proposta visando ser uma alternativa na solução de Problemas Inversos de estimativa de propriedades radiativas em meios participantes homogêneos unidimensionais usando a Equação de Transferência Radiativa para modelar a interação da radiação com o meio participante. A equação de transporte é formulada em forma matricial e o domínio angular é discretizado usando conceitos do método de ordenadas discretas e a expansão da função de fase do espalhamento anisotrópico em uma série de polinômios de Legendre. A formulação proposta consiste em uma formulação explícita para o problema inverso. Um arranjo apropriado das condições de contorno prescritas (fluxos incidentes) e dos fluxos emergentes nos contornos de uma placa permitem o cálculo direto do operador de transmissão, do operador albedo e do operador de colisão. A partir do operador de colisão calculado são obtidos os valores estimados dos coeficientes de extinção total e de espalhamento. São apresentadas as formulações para problemas em regime estacionário e em regime transiente, bem como os resultados para alguns casos-teste. / The explicit matrix formulation developed in the present thesis has been proposed as an alternative for the solution of Inverse Problems for radiative properties estimation in one-dimensional homogeneous participating media using Radiative transfer equation for the modeling of the radiation interaction with the participating medium. This transport equation is formulated in a matrix form and the angular domain is discretized using concepts of the discrete ordinates methods and the expansion of the function of phase function of anisotropic scattering in a series of Legendre polynomial. The formulation proposed consists on an explicit formulation for the inverse problem. An adequate assembly of the prescribed boundary conditions (incidents flux) and of the emerging flux at the boundaries of the slab allows the direct computation of the transmission, albedo and collision operators. From the computed collision operator estimated values for total extinction and scattering coefficients are obtained. The formulations for steady state and transient situations are presented, as well as test case results.

Nesta tese é proposta uma implementação para a solução do problema inverso com as estimativas das propriedades radiativas (o albedo de espalhamento simples, a espessura ótica do meio e as reflectividades difusas) a partir dos valores das intensidades de radiação que deixam o meio participante utilizando uma abordagem híbrida de sistemas neuro-fuzzy (SNF), o qual combina a utilização de sistemas de inferência fuzzy com as redes neurais artificiais. Busca-se com a utilização desse sistema híbrido integrar a habilidade dos sistemas fuzzy no tratamento de informações inexatas, imprecisas, e vagas, e a capacidade das redes neurais artificiais de tratar o aprendizado por experiência e a generalização do conhecimento. É proposta também uma metodologia de máquinas de comitês neuro-fuzzy na solução deste problema inverso em transferência radiativa. Foi observado paralelamente que a solução dos sistemas neuro-fuzzy e dos sistemas híbridos de máquinas de comitê neuro-fuzzy, apresentam baixa qualidade nos resultados quando são utilizados os dados experimentais com os menores coeficientes de sensibilidade para os parâmetros que serão estimados. Por outro lado, quando são utilizados dados com maior sensibilidade, são obtidos melhores resultados. Esta abordagem procura evitar a possibilidade da não convergência desses métodos. / In this thesis is proposed an implementation for solving the inverse problem with the estimates of radiative properties (the single scattering albedo, the optical thickness of the media and the diffuse reflectivities) by the values of the intensities of radiation that leaves the participant medium using a hybrid approach of neuro-fuzzy systems, which combines the use of fuzzy inference systems with artificial neural networks. The use of this hybrid system try to include the ability of fuzzy systems in the treatment of inaccurate, imprecise, and vague data, and the ability of artificial neural networks to deal with learning from experience and widespread knowledge. Also is proposed a methodology for machines committees in neuro-fuzzy solution of this inverse problem in radiative transfer. It was observed in parallel that the solution of neuro-fuzzy systems and hybrid systems neuro-fuzzy committee machines, have a poor quality results when using the experimental data with the lowest sensitivity coefficients for the parameters that will be estimated. Moreover, when data are used with greater sensitivity, better results are obtained. This approach seeks to avoid the possibility of non-convergence in such methods.

Este trabalho fundamenta-se no conceito de máquina de comitê de redes neurais artificiais e tem por objetivo resolver o problema inverso de transferência radiativa em um meio unidimensional, homogêneo, absorvedor e espalhador isotrópico. A máquina de comitê de redes neurais artificiais agrega e combina o conhecimento adquirido por um certo número de especialistas aqui representados, individualmente, por cada uma das redes neurais artificiais (RNA) que compõem a máquina de comitê de redes neurais artificiais. O objetivo é atingir um resultado final melhor do que o obtido por qualquer rede neural artificial separadamente, selecionando-se apenas àquelas redes neurais artificiais que apresentam os melhores resultados na fase de generalização descartando-se as demais, o que foi feito neste trabalho. Aqui são utilizados dois modelos estáticos de máquinas de comitê, usando a média aritmética de conjunto, que se diferenciam entre si apenas na composição do combinador de saída de cada máquina de comitê. São obtidas, usando-se máquinas de comitê de redes neurais artificiais, estimativas para os parâmetros de transferência radiativa, isto é, a espessura óptica do meio, o albedo de espalhamento simples e as refletividades difusas. Finalmente, os resultados obtidos com ambos os modelos de máquina de comitê são comparados entre si e com aqueles encontrados usando-se apenas redes neurais artificiais do tipo perceptrons de múltiplas camadas (MLP), isoladamente. Aqui essas redes neurais artificiais são denominadas redes neurais especialistas, mostrando que a técnica empregada traz melhorias de desempenho e resultados a um custo computacional relativamente baixo. / This work is based on the concept of neural networks committee machine and has the objective to solve the inverse radiative transfer problem in one-dimensional, homogeneous, absorbing and isotropic scattering media. The artificial neural networks committee machine adds and combines the knowledge acquired by an exact number of specialists which are represented, individually, by each one of the artificial neural networks (ANN) that composes the artificial neural network committee machine. The aim is to reach a final result better than the one obtained by any of the artificial neural network separately, selecting only those artificial neural networks that presents the best results during the generalization phase and discarding the others, what was done in this present work. Here are used two static models of committee machines, using the ensemble arithmetic average, that differ between themselves only by the composition of the output combinator by each one of the committee machine. Are obtained, using artificial neural networks committee machines, estimates for the radiative transfer parameters, that is, medium optical thickness, single scattering albedo and diffuse reflectivities. Finally, the results obtained with both models of committee machine are compared between themselves and with those found using artificial neural networks type multi-layer perceptrons (MLP), isolated. Here that artificial neural networks are named as specialists neural networks, showing that the technique employed brings performance and results improvements with relatively low computational cost.

Esta tese apresenta um estudo sobre modelagem computacional onde são aplicadas meta-heurísticas de otimização na solução de problemas inversos de transferência radiativa em meios unidimensionais com albedo dependente da variável óptica, e meios unidimensionais de duas camadas onde o problema inverso é tratado como um problema de otimização. O trabalho aplica uma meta-heurística baseada em comportamentos da natureza conhecida como algoritmo dos vagalumes. Inicialmente, foram feitos estudos comparativos de desempenho com dois outros algoritmos estocásticos clássicos. Os resultados encontrados indicaram que a escolha do algoritmo dos vagalumes era apropriada. Em seguida, foram propostas outras estratégias que foram inseridas no algoritmo dos vagalumes canônico. Foi proposto um caso onde se testou e investigou todas as potenciais estratégias. As que apresentaram os melhores resultados foram, então, testadas em mais dois casos distintos. Todos os três casos testados foram em um ambiente de uma camada, com albedo de espalhamento dependente da posição espacial. As estratégias que apresentaram os resultados mais competitivos foram testadas em um meio de duas camadas. Para este novo cenário foram propostos cinco novos casos de testes. Os resultados obtidos, pelas novas variantes do algoritmo dos vagalumes, foram criticamente analisados. / This thesis presents a study on computational modeling where optimization metaheuristics are applied to the solution of inverse radiative transfer problems in heterogeneous media: in one-layer media with space-dependent single scattering albedo, and two-layer media, where the inverse problem is formulated as an optimization problem. It is applied a metaheuristic based on the natural behavior of fireflies, known as the firefly algorithm. Initially, comparative studies of performance were made with two other classic stochastic algorithms. The results indicated that the choice of the firefly algorithm was appropriate. Then, it was proposed other strategies that have been inserted into the original firefly algorithm. A first case was proposed where all the strategies were investigated and tested. The strategies with the best results were investigated in other two different cases. All the three proposed cases involved one-layer media with space-dependent scattering albedo. The strategies have been tested and evaluated, and those which presented the best competitive results were then implemented for radiative problems in two-layer media. For this new scenario five test cases were investigated, and the results obtained with the new strategies developed in this work were critically analyzed.

Esta pesquisa consiste na solução do problema inverso de transferência radiativa para um meio participante (emissor, absorvedor e/ou espalhador) homogêneo unidimensional em uma camada, usando-se a combinação de rede neural artificial (RNA) com técnicas de otimização. A saída da RNA, devidamente treinada, apresenta os valores das propriedades radiativas [ω, τ0, ρ1 e ρ2] que são otimizadas através das seguintes técnicas: Particle Collision Algorithm (PCA), Algoritmos Genéticos (AG), Greedy Randomized Adaptive Search Procedure (GRASP) e Busca Tabu (BT). Os dados usados no treinamento da RNA são sintéticos, gerados através do problema direto sem a introdução de ruído. Os resultados obtidos unicamente pela RNA, apresentam um erro médio percentual menor que 1,64%, seria satisfatório, todavia para o tratamento usando-se as quatro técnicas de otimização citadas anteriormente, os resultados tornaram-se ainda melhores com erros percentuais menores que 0,04%, especialmente quando a otimização é feita por AG. / This research consists in the solution of the inverse problem of radiative transfer for a participating media (emmiting, absorbing and/or scattering) homogeneous one-dimensional in one layer, using the combination of artificial neural network (ANN), with optimization techniques. The output of the ANN, properly trained presents the values of the radiative properties [w, to, p1 e p2] that are optimized through the following techniques: Particle Collision Algorithm (PCA), Genetic Algorithm (GA), Greedy Randomized Adaptive Search Procedure (GRASP) and Tabu Search (TS). The data used in the training are synthetics, generated through the direct problem without the introduction of noise. The results obtained by the (ANN) alone, presents an average percentage error minor than 1,64%, what it would be satisfying, however, for the treatment using the four techniques of optimization aforementioned, the results have become even better with percentage errors minor than 0,03%, especially when the optimization is made by the GA.