Cette thèse s’intéresse à l’endommagement laser d’optiques réflectives en régime sub-picoseconde. Ces composants optiques, réalisés à partir d’empilements sub-micrométriques de matériaux diélectriques, sont couramment utilisés dans les installations laser de puissance telles que le laser PETAL. Ce dernier, construit sur le centre du CEA-CESTA en France, a été conçu pour délivrer des impulsions de 500 fs et de quelques kJ à une longueur d’onde de 1053 nm, dans le but d’atteindre des puissances supérieures à 6PW. Dans ce type d’installations de puissance, afin de limiter l’accumulation d’effets non-linéaires liés à la propagation d’impulsions intenses, des optiques réflectives en fin de chaîne se substituent aux optiques en transmission. Les composants optiques illuminés par les plus fortes densités de puissance sont des réseaux de compression, des miroirs et une parabole qui servent respectivement à la compression temporelle des impulsions, au transport du faisceau ainsi qu’à sa focalisation. Le phénomène d'endommagement laser est le paramètre principal qui limite la puissance accessible par ces lasers. Il est nécessaire de comprendre et de maîtriser ce phénomène afin de fiabiliser une installation laser et également d’améliorer ses performances. Trois axes d’études ont donc été explorés. Le premier concerne la conception d’optiques réflectives. Des définitions de structures sont recherchées afin d’obtenir de hautes efficacités de diffraction dans le cas des réseaux et des forts coefficients de réflexion dans le cas des miroirs, tout en diminuant le renforcement du champ électrique dans les structures, l’une des causes de l’endommagement laser. Le second axe d’étude porte sur la mise en place d’une métrologie fine de l’endommagement laser avec le développement de nouvelles procédures de test. Elles amènent de nouveaux points de vue pour la qualification de la résistance au flux laser des optiques. En dernier lieu, nous étudions le phénomène de croissance des dommages lorsqu’ils sont soumis à plusieurs irradiations laser. L’évolution de la surface des dommages lors de séquences de croissance est observée, quantifiée et comparée à un modèle numérique. Cela nous permet de mieux comprendre la phénoménologie de la croissance des dommages en régime sub-picoseconde. A terme, elles permettront de développer des modèles de prédiction de l’endommagement et des outils pour l’amélioration des optiques utilisées sur chaîne laser. / In this thesis, laser-induced damage phenomenon of reflective components is investigated in the sub-picosecond regime. These components, made of stacks of dielectric materials, are widely used in powerful laser facilities such as PETAL laser. PETAL laser has been built at the CEA-CESTA in France to deliver multi-kJ/500fs pulses at 1053nm and reach a power higher than 6PW. For this kind of laser systems, reflective components are commonly used instead of optics operating in transmission to limit the accumulation of non-linear phase along the beam propagation due to the high intensities. Optical components irradiated by the highest power densities are the pulse compression gratings, transport mirrors and the focusing parabola, located at the end of the laser chain. Nowadays, laser-induced damage is the main factor that limits the overall performances of powerful laser systems. This manuscript presents three study axes to better understand and control damage phenomenon. The first one concerns the conception of reflective optics for the petawatt applications. The design of new structures has been investigated to reach high diffraction efficiencies in the case of pulse compression gratings and a high reflectivity in the case of mirrors, while reducing the Electric-field enhancement which is one of the causes of the laser-induced damage. The second axis deals with the development of a precise damage metrology with new testing tools which brings new perspectives and a new viewpoint for the assessment of the laser resistance of optical components. Finally, the third axis concerns the study the damage growth after several irradiations in the sub-picosecond regime. The evolution of the damage area during growth sequences is observed and compared to numerical simulations. It enables to improve the understanding in the growth phenomenon. In the end, these studies will allow to develop predictive models of the laser-induced damage and new tools for the conception of reflective optics for petawatt applications.

Les réseaux de diffraction pour la compression d'impulsions constituent actuellement un verrou technologique pour le développement des chaînes laser de puissance énergétiques dans le régime Petawatt. En effet, la tenue au flux laser et les dimensions des réseaux métalliques actuels sont limitées. C'est pourquoi, une nouvelle génération de réseaux de diffraction à multicouches diélectriques (MLD) a été développée. Ce travail d'étude et de caractérisation des réseaux MLD pour le laser Petawatt Pico2000 du LULI constitue la première partie de ma thèse. D'autre part, les réseaux de diffraction pour la compression d'impulsions Petawatt doivent avoir des dimensions de l'ordre du mètre, ce qui complique les procédés de fabrication et de caractérisation. Comme alternative! aux grands réseaux, le concept de la mise en phase de réseaux de diffraction a été étudié. Les différents résultats obtenus sur la mise en phase en lumière monochromatique par technique interférométrique sont exposés ainsi que la démonstration de la compression d'impulsions multi-terawatt par mosaïques de réseaux. Une étude du contrôle temporel des impulsions du laser Pico2000 a également été réalisée, portant sur la thématique du contraste temporel et sur la mise en forme spectrale des impulsions.

A two-year experimental campaign is described during which diamond-like carbon and plastic targets with thicknesses from 20 nanometers to 15 micrometers were irradiated by the Texas Petawatt Laser. Target composition and thickness were varied to modify the specifics of the laser-matter interaction. Plasma mirrors were selectively implemented to affect the contrast of the laser system and provide additional control of the physical processes under investigation. A number of particle diagnostics were implemented to measure the distribution of laser accelerated ions and electrons. In addition, optical diagnostics were fielded to measure the intensity profile of the laser and measure the density of the target pre-plasma. The results of these experiments suggest that the Texas Petawatt laser pulse has pre-pulse and pedestal features with intensities at least 10⁻⁸ of the main pulse. Micronscale targets were able to survive these features and maintain a relatively sharp density gradient until the arrival of the main laser pulse, allowing for ion acceleration. Electron spectra measured in this configuration show an average temperature of 10 MeV, with no v angular dependence out to at least 60 degrees. By contrast, interferometric plasma density measurements and a lack of any observable ion acceleration suggest that nanoscale targets were destroyed well before the main pulse. In this case, the peak of the laser pulse interacted with a cloud of plasma between 10⁻³ and 10⁻² of critical density. The contrast improvement offered by the implementation of plasma mirrors was seen to increase the maximum energy of laser accelerated protons from targets thicker than 1 micrometer. In addition, the plasma mirrors allowed nanoscale targets to survive pre-pulse and pedestal features and support the production of ion beams. Proton spectra show that ions were accelerated to greater maximum energies from nanoscale targets than from more traditional micron-scale targets. This effect can be attributed to a reduction in the target pre-plasma scale length upon the introduction of plasma mirrors. These results indicate that the manipulation of target properties and laser contrast can significantly affect the interaction between an ultrahigh intensity laser and a target. / text

An overview of the beam diagnostics for the laser wakefield acceleration project at the Texas Petawatt Laser facility is presented. In this experiment, short and intense laser pulses of 165 fs and up to 190 J will be used to accelerate electrons up to the GeV energy range using laser wakefield acceleration. The density variation of the plasma generated in a helium gas cell will be measured with different optical detection systems such as frequency domain holography. Spectra of the transmitted laser beam and optical transition radiation will yield information about the energy transfer to the plasma and the energy of the electrons, respectively. In addition, a calorimeter will measure accelerated electron energies. Prior to the final experiment, preliminary frequency shift measurements and simulations on optical transition radiation were performed. / text

The generation of high current multi-MeV protons and ions by irradiation of short pulse high intense laser on an ultra-thin target has been observed and subjected great interest in recent. When ultra-thin overdense target is irradiated by focused ultraintense laser pulse, hot electrons are generated by various mechanisms and they generate energetic ion beams. In TNSA, a quasi-electrostatic field is produced on the target rear surface when the the laser pulse interacts with overdense target, driving hot electrons go torward the target rear surface. However, this mechanism results in a range of field gradients leading to a broad proton energy distribution typically. To overcome the issue, an alternative accelration mechanism has been presented to achieve the quasi-monoenergetic proton acceleration and the mechanism is called Radiation Pressure Acceleration. In the RPA, the radiation pressure push electrons into the target smoothly and setting up an electrostatic field by the laser pressure. In this thesis, we study two alternative experimental methods for the quasi-monoenergetic proton acceleration and find experimental feasibility of the presented methods from other research groups. / text

Since 2004, table-top laser-plasma accelerators (LPAs) driven by ˜30fs terwatt laser pulses have produced colimated, nearly mono-energetic eletron bunches with energy up to 1 GeV in laboratories around the world. Large-scale computer simulations show that LPAs can scale to higher energy while retaining high beam quality, but will require laser pulses of higher energy and longer duration than current LPAs. The group of Prof. Mike Downer, in collaboration with the Texas Petawatt (TPW) laser team headed by Prof. Todd Ditmire, is setting up an experiment that uses the TPW laser (1.1 PW, 150 fs) to drive the world’s first multi-GeV LPA. This thesis provides a general overview of the TPW-LPA project, including several diagnostic systems for the beam, plasma and laser pulse. Special attention is given to three of the diagnostic systems: (1)A transverse interferometry diagnostic of the plasma density profile created by the TPW laser pulse; (2)A Thomson scattering diagnostic of the self-guided path of the TPW laser pulse through the plasma; (3)An optical transition radiation diagnostic of the accelerated electron bunch exiting the plasma. In each case, basic principles, theoretical background, calculation and simulation results, and preliminary experimental results will be presented. / text

No description available.

The ultrashort chirped pulse amplification (CPA) laser technology opens the path to high intensities of 10^21 W/cm² and above in the laser focus. Such intensities allow laser-matter interaction in the relativistic intensity regime. Direct diode-pumped ultrashort solid-state lasers combine high-energy, high-power and efficient amplification together, which are the main advantages compared to flashlamp-pumped high-energy laser systems based on titanium-doped sapphire. Development within recent years in the field of laser diodes makes them more and more attractive in terms of total costs, compactness and lifetime. This work is dedicated to the Petawatt, ENergy-Efficient Laser for Optical Plasma Experiments (PENELOPE) project, a fully and directly diode-pumped laser system under development at the Helmholtz–Zentrum Dresden – Rossendorf (HZDR), aiming at 150 fs long pulses with energies of up to 150 J at repetition rates of up to 1 Hz. The focus of this thesis lies on the spectral and width manipulation of the front-end amplifiers, trivalent ytterbium-doped calcium fluoride (Yb3+:CaF2) as gain material as well as the pump source for the final two main amplifiers of the PENELOPE laser system. Here, all crucial design parameters were investigated and a further successful scaling of the laser system to its target values was shown. Gain narrowing is the dominant process for spectral bandwidth reduction during the amplification at the high-gain front-end amplifiers. Active or passive spectral gain control filter can be used to counteract this effect. A pulse duration of 121 fs was achieved by using a passive spectral attenuation inside a regenerative amplifier, which corresponds to an improvement by a factor of almost 2 compared to the start of this work. A proof-of-concept experiment showed the capability of the pre-shaping approach. A spectral bandwidth of 20nm was transferred through the first multipass amplifier at a total gain of 300. Finally, the predicted output spectrum calculated by a numerical model of the final amplifier stages was in a good agreement with the experimental results. The spectroscopic properties of Yb3+:CaF2 matches the constraints for ultrashort laser pulse amplification and direct diode pumping. Pumping close to the zero phonon line at 976nm is preferable compared to 940nm as the pump intensity saturation is significantly lower. A broad gain cross section of up to 50nm is achievable for typical inversion levels. Furthermore, moderate cryogenic temperatures (above 200K) can be used to improve the amplification performance of Yb3+:CaF2. The optical quality of the doped crystals currently available on the market is sufficient to build amplifiers in the hundred joule range. The designed pump source for the last two amplifiers is based on two side pumping in a double pass configuration. However, this concept requires the necessity of brightness conservation for the installed laser diodes. Therefore, a fully relay imaging setup (4f optical system) along the optical path from the stacks to the gain material including the global beam homogenization was developed in a novel approach. Beside these major parts the amplifier architecture and relay imaging telescopes as well as temporal intensity contrast (TIC) was investigated. An all reflective concept for the relay imaging amplifiers and telescopes was selected, which results in several advantages especially an achromatic behavior and low B-Integral. The TIC of the front-end was improved, as the pre- and postpulses due to the plane-parallel active-mirror was eliminated by wedging the gain medium.

The ultrashort chirped pulse amplification (CPA) laser technology opens the path to high intensities of 10^21 W/cm² and above in the laser focus. Such intensities allow laser-matter interaction in the relativistic intensity regime. Direct diode-pumped ultrashort solid-state lasers combine high-energy, high-power and efficient amplification together, which are the main advantages compared to flashlamp-pumped high-energy laser systems based on titanium-doped sapphire. Development within recent years in the field of laser diodes makes them more and more attractive in terms of total costs, compactness and lifetime. This work is dedicated to the Petawatt, ENergy-Efficient Laser for Optical Plasma Experiments (PENELOPE) project, a fully and directly diode-pumped laser system under development at the Helmholtz–Zentrum Dresden – Rossendorf (HZDR), aiming at 150 fs long pulses with energies of up to 150 J at repetition rates of up to 1 Hz. The focus of this thesis lies on the spectral and width manipulation of the front-end amplifiers, trivalent ytterbium-doped calcium fluoride (Yb3+:CaF2) as gain material as well as the pump source for the final two main amplifiers of the PENELOPE laser system. Here, all crucial design parameters were investigated and a further successful scaling of the laser system to its target values was shown. Gain narrowing is the dominant process for spectral bandwidth reduction during the amplification at the high-gain front-end amplifiers. Active or passive spectral gain control filter can be used to counteract this effect. A pulse duration of 121 fs was achieved by using a passive spectral attenuation inside a regenerative amplifier, which corresponds to an improvement by a factor of almost 2 compared to the start of this work. A proof-of-concept experiment showed the capability of the pre-shaping approach. A spectral bandwidth of 20nm was transferred through the first multipass amplifier at a total gain of 300. Finally, the predicted output spectrum calculated by a numerical model of the final amplifier stages was in a good agreement with the experimental results. The spectroscopic properties of Yb3+:CaF2 matches the constraints for ultrashort laser pulse amplification and direct diode pumping. Pumping close to the zero phonon line at 976nm is preferable compared to 940nm as the pump intensity saturation is significantly lower. A broad gain cross section of up to 50nm is achievable for typical inversion levels. Furthermore, moderate cryogenic temperatures (above 200K) can be used to improve the amplification performance of Yb3+:CaF2. The optical quality of the doped crystals currently available on the market is sufficient to build amplifiers in the hundred joule range. The designed pump source for the last two amplifiers is based on two side pumping in a double pass configuration. However, this concept requires the necessity of brightness conservation for the installed laser diodes. Therefore, a fully relay imaging setup (4f optical system) along the optical path from the stacks to the gain material including the global beam homogenization was developed in a novel approach. Beside these major parts the amplifier architecture and relay imaging telescopes as well as temporal intensity contrast (TIC) was investigated. An all reflective concept for the relay imaging amplifiers and telescopes was selected, which results in several advantages especially an achromatic behavior and low B-Integral. The TIC of the front-end was improved, as the pre- and postpulses due to the plane-parallel active-mirror was eliminated by wedging the gain medium.

No description available.