Indiana University-Purdue University Indianapolis (IUPUI) / Today transportation is one of the rapidly evolving technologies in the world. With the stringent mandatory emission regulations and high fuel prices, researchers and manufacturers are ever increasingly pushed to the frontiers of research in pursuit of alternative propulsion systems. Electrically propelled vehicles are one of the most promising solutions among all the other alternatives, as far as; reliability, availability, feasibility and safety issues are concerned. However, the shortcomings of a fully electric vehicle in fulfilling all performance requirements make the electrification of the conventional engine powered vehicles in the form of a plug-in hybrid electric vehicle (PHEV) the most feasible propulsion systems. The optimal combination of the properly sized components such as internal combustion engine, electric motor, energy storage unit are crucial for the vehicle to meet the performance requirements, improve fuel efficiency, reduce emissions, and cost effectiveness. In this thesis an application of Particle Swarm Optimization (PSO) approach to optimally size the vehicle powertrain components (e.g. engine power, electric motor power, and battery energy capacity) while meeting all the critical performance requirements, such as acceleration, grade and maximum speed is studied. Compared to conventional optimization methods, PSO handles the nonlinear constrained optimization problems more efficiently and precisely. The PHEV powertrain configuration with the determined sizes of the components has been used in a new vehicle model in PSAT (Powertrain System Analysis Toolkit) platform. The simulation results show that with the optimized component sizes of the PHEV vehicle (via PSO), the performance and the fuel efficiency of the vehicle are significantly improved. The optimal solution of the component sizes found in this research increased the performance and the fuel efficiency of the vehicle. Furthermore, after reaching the desired values of the component sizes that meet all the performance requirements, the overall emission of hazardous pollutants from the PHEV powertrain is included in the optimization problem in order to obtain updated PHEV component sizes that would also meet additional design specifications and requirements.

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This work presents novel modeling and experimental techniques that provide insight into liquid-phase mass transport and electron transfer processes in lithium-ion batteries. These included liquid-phase ionic mass transport (conduction and diffusion), lithium diffuion in the solid phase and electronic transport in the solid phase. Fundamental understanding of these processes is necessary to efficiently design and optimize lithium-ion batteries for different applications. To understand the effect of electrode structure on the electronic resistance of the cathode, we tested power performance of cathodes with combinations of three different carbon conductivity additives: vapor-grown carbon fibers (CF), carbon black (CB) and graphite (GR). With all other factors held constant, cathodes with a mixture of CF+CB were found to have the best power-performance, followed by cells containing CF only and then by CB+GR. Thus, the use of carbon fibers as conductive additive was found to improve the power performance of cells compared to the baseline (CB+GR). The enhanced electrode performance due to the fibers also allows an increase in energy density while still meeting power goals. About one-third of the available energy was lost to irreversible processes when cells were pulse-charged or discharged at the maximum rate allowed by voltage-cutoff constraints. We developed modeling and experimental techniques to quantify tortuosity in electrolyte-filled porous battery structures (separator and active-material film). Tortuosities of separators were measured by two methods, AC impedance and polarization-interrupt, which produced consistent results. The polarization-interrupt experiment was used similarly to measure effective electrolyte transport in porous films of cathode materials, particularly films containing lithium iron phosphate. An empirical relationship between porosity and the tortuosity of the porous structures was developed. Our results demonstrate that the tortuosity-dependent mass transport resistance in porous separators and electrodes is significantly higher than that predicted by the oft-used Bruggeman relationship. To understand the dominant resistances in a lithium battery, we developed and validated a model for lithium iron phosphate cathode. In doing so we considered unique physical features of this active material. Our model is unusual in terms of the range of experimental conditions for which it is validated. Various submodel and experimental techniques were used to find physically realistic parameters. The model was tested with different discharge rates and thicknesses of cathodes, in all cases showing good agreement, which suggests that the model takes into account physical realities with different thicknesses. The model was then used to find the dominant resistance for the tested cathodes. The model suggests that the inter-particle contact resistance between carbon and the active-material particles was a dominant resistance for the tested cathodes.

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During the past two decades desperate need for energy-efficient vehicles which has less emission have led to a great attention to and development of electrified vehicles like pure electric, Hybrid Electric Vehicle (HEV) and Plug-in Hybrid Electric Vehicles (PHEVs). Resultantly, a great amount of research efforts have been dedicated to development of control strategies for this type of vehicles including PHEV which is the case study in this thesis. This thesis presents a real-time control scheme to improve the fuel economy of plug-in hybrid electric vehicles (PHEVs) by accounting for the instantaneous states of the system as well as the future trip information. To design the mentioned parametric real-time power management policies, we use dynamic programming (DP). First, a representative power-split PHEV powertrain model is introduced, followed by a DP formulation for obtaining the optimal powertrain trajectories from the energy cost point of view for a given drive cycle. The state and decision variables in the DP algorithm are selected in a way that provides the best tradeoff between the computational time and accuracy which is the first contribution of this research effort. These trajectories are then used to train a set of linear maps for the powertrain control variables such as the engine and electric motor/generator torque inputs, through a least-squares optimization process. The DP results indicate that the trip length (distance from the start of the trip to the next charging station) is a key factor in determining the optimal control decisions. To account for this factor, an additional input variable pertaining to the remaining length of the trip is considered during the training of the real-time control policies. The proposed controller receives the demanded propulsion force and the powertrain variables as inputs, and generates the torque commands for the engine and the electric drivetrain system. Numerical simulations indicate that the proposed control policy is able to approximate the optimal trajectories with a good accuracy using the real-time information for the same drive cycles as trained and drive cycle out of training set. To maintain the battery state-of-charge (SOC) above a certain lower bound, two logics have been introduced a switching logic is implemented to transition to a conservative control policy when the battery SOC drops below a certain threshold. Simulation results indicate the effectiveness of the proposed approach in achieving near-optimal performance while maintaining the SOC within the desired range. / MS / During the past two decades desperate need for energy-efficient vehicles which has less emission have led to a great attention to and development of electrified vehicles like pure electric, Hybrid Electric Vehicle (HEV) and Plug-in Hybrid Electric Vehicles (PHEVs). Resultantly, a great amount of research efforts have been dedicated to development of control strategies for this type of vehicles including PHEV which is the case study in this thesis. This thesis presents a real-time control scheme to improve the fuel economy of plug-in hybrid electric vehicles (PHEVs) by accounting for the instantaneous states of the system as well as the future trip information. To design the mentioned parametric real-time power management policies, we use dynamic programming (DP). First, a representative power-split PHEV powertrain model is introduced, followed by a DP formulation for obtaining the optimal powertrain trajectories from the energy cost point of view for a given drive cycle. The state and decision variables in the DP algorithm are selected in a way that provides the best tradeoff between the computational time and accuracy which is the first contribution of this research effort. These trajectories are then used to train a set of linear maps for the powertrain control variables such as the engine and electric motor/generator torque inputs, through a least-squares optimization process. The DP results indicate that the trip length (distance from the start of the trip to the next charging station) is a key factor in determining the optimal control decisions. To account for this iv factor, an additional input variable pertaining to the remaining length of the trip is considered during the training of the real-time control policies. The proposed controller receives the demanded propulsion force and the powertrain variables as inputs, and generates the torque commands for the engine and the electric drivetrain system. Numerical simulations indicate that the proposed control policy is able to approximate the optimal trajectories with a good accuracy using the real-time information for the same drive cycles as trained and drive cycle out of training set. To maintain the battery state-of-charge (SOC) above a certain lower bound, two logics have been introduced a switching logic is implemented to transition to a conservative control policy when the battery SOC drops below a certain threshold. Simulation results indicate the effectiveness of the proposed approach in achieving near-optimal performance while maintaining the SOC within the desired range.

In today’s world of volatile fuel prices and climate concerns, there is little study on the relation between vehicle ownership patterns and attitudes toward potential policies and vehicle technologies. This work provides new data on ownership decisions and owner preferences under various scenarios, coupled with calibrated models to microsimulate Austin’s household-fleet evolution. Results suggest that most Austinites (63%, population-corrected share) support a feebate policy to favor more fuel efficient vehicles. Top purchase criteria are vehicle purchase price, type/class, and fuel economy (with 30%, 21% and 19% of respondents placing these in their top three). Most (56%) respondents also indicated that they would seriously consider purchasing a Plug-In Hybrid Electric Vehicle (PHEV) if it were to cost $6,000 more than its conventional, gasoline-powered counterpart. And many respond strongly to signals on the external (health and climate) costs of a vehicle’s emissions, more strongly than they respond to information on fuel cost savings. 25-year simulations suggest that 19% of Austin’s vehicle fleet could be comprised of Hybrid Electric Vehicles (HEVs) and PHEVs under adoption of a feebate policy (along with PHEV availability in Year 1 of the simulation, and current gas prices throughout). Under all scenarios vehicle usage levels (in total vehicle miles traveled [VMT]) are predicted to increase overall, along with average vehicle ownership levels (per household, and per capita); and a feebate policy is predicted to raise total regional VMT slightly (just 4.43 percent, by simulation year 25), relative to the trend scenario, while reducing CO2 emissions only slightly (by 3.8 percent, relative to trend). Doubling the trend-case gas price to $5/gallon is simulated to reduce the year-25 vehicle use levels by 17% and CO2 emissions by 22% (relative to trend). Two- and three-vehicle households are simulated to be the highest adopters of HEVs and PHEVs across all scenarios. And HEVs, PHEVs and Smart Cars are estimated to represent a major share of the fleet’s VMT (25%) by year 25 under the feebate scenario. The combined share of vans, pickup trucks, sport utility vehicles (SUVs), and cross over utility vehicles (CUVs) is lowest under the feebate scenario, at 35% (versus 47% in Austin’s current household fleet), yet feebate-policy receipts exceed rebates in each simulation year. A 15% reduction in the usage levels of SUVs, CUVs and minivans is observed in the $5/gallon scenario (relative to trend). Mean use levels per vehicle of HEVs and PHEVs are simulated to have a variation of 753 and 495 across scenarios. In the longer term, gas price dynamics, tax incentives, feebates and purchase prices along with new technologies, government-industry partnerships, and more accurate information on range and recharging times (which increase customer confidence in EV technologies) should have even more significant effects on energy dependence and greenhouse gas emissions. / text

Transportation fleet emissions have a dominant role in air quality because of their significant contribution to ozone precursor and greenhouse gas emissions. Regulatory policies have emphasized improvements in vehicle fuel economy, alternative fuel use, and engine and vehicle technologies as approaches for obtaining transportation systems that support sustainable development. This study examined the air quality impacts of the partial electrification of the transportation fleet and the use of biofuels for the Austin Metropolitan Statistical Area under a 2030 vision of regional population growth and urban development using the Comprehensive Air Quality Model with extensions (CAMx). Different strategies were considered including the use of Plug-in Hybrid Electric Vehicles (PHEVs) with nighttime charging using excess capacity from electricity generation units and the replacement of conventional petroleum fuels with different percentages of the biofuels E85 and B100 along or in combination. Comparisons between a 2030 regional vision of growth assuming a continuation of current development trends (denoted as Envision Central Texas A or ECT A) in the Austin MSA and the electrification and biofuels scenarios were evaluated using different metrics, including changes in daily maximum 1-hour and 8-hour ozone concentrations, total area, time integrated area and total daily population exposure exceeding different 1-hour ozone concentration thresholds. Changes in ozone precursor emissions and predicted carbon monoxide and aldehyde concentrations were also determined for each scenario. Maximum changes in hourly ozone concentration from the use of PHEVs ranged from -8.5 to 2.2 ppb relative to ECT A. Replacement of petroleum based fuels with E85 had a lesser effect than PHEVs on maximum daily ozone concentrations. The maximum reduction due to replacement of 100% of gasoline fuel in light and heavy duty gasoline vehicles by E85 ranged from -2.1 to 2.8 ppb. The magnitude of the effect was sensitive to the biofuel penetration level. Unlike E85, B100 negatively impacted hourly ozone concentrations relative to the 2030 ECT A case. As the replacement level of petroleum-diesel fuel with B100 in diesel vehicles increased, hourly ozone concentrations increased as well. However, changes due to the penetration of B100 were relatively smaller than those due to E85 since the gasoline fraction of the fleet is larger than the diesel fraction. Because of the reductions in NOx emissions associated with E85, the results for the biofuels combination scenario were similar to those for the E85 scenario. Also, the results showed that as the threshold ozone concentration increased, so too did the percentage reductions in total daily population exposure for the PHEV, E85, and biofuel combination scenarios relative to ECT A. The greatest reductions in population exposure under higher threshold ozone concentrations were achieved with the E85 100% and 17% PHEV with EGU controls scenarios, while the B100 scenarios resulted in greater population exposure under higher threshold ozone concentrations. / text

Today, hybrid electric propulsion technology provides a promising and practical solution for improving vehicle performance, increasing energy efficiency, and reducing harmful emissions, due to the additional flexibility that the technology has provided in the optimal power control and energy management, which are the keys to its success. In this work, a systematic approach for real-time optimal energy management of hybrid electric vehicles (HEVs) and plug-in hybrid electric vehicles (PHEVs) has been introduced and validated through two HEV/PHEV case studies. Firstly, a new analytical model of the optimal control problem for the Toyota Prius HEV with both offline and real-time solutions was presented and validated through Hardware-in-Loop (HIL) real-time simulation. Secondly, the new online or real-time optimal control algorithm was extended to a multi-regime PHEV by modifying the optimal control objective function and introducing a real-time implementable control algorithm with an adaptive coefficient tuning strategy. A number of practical issues in vehicle control, including drivability, controller integration, etc. are also investigated. The new algorithm was also validated on various driving cycles using both Model-in-Loop (MIL) and HIL environment. This research better utilizes the energy efficiency and emissions reduction potentials of hybrid electric powertrain systems, and forms the foundation for development of the next generation HEVs and PHEVs. / Graduate / laindeece@gmail.com

The batteries used in plug-in hybrid electric vehicles (PHEVs) need to overcome significant technical challenges in order for PHEVs to become economically viable and have a large market penetration. The internship at Argonne National Laboratory (ANL) involved two experiments which looked at a vehicle systems approach to analyze two such technical challenges: Battery life and low battery power at cold (-7 ⁰C) temperature. The first experiment, concerning battery life and its impact on gasoline savings due to a PHEV, evaluates different vehicle control strategies over a pre-defined vehicle drive cycle, in order to identify the control strategy which yields the maximum dollar savings (operating cost) over the life of the vehicle, when compared to a charge sustaining hybrid. Battery life degradation over the life of the vehicle, and fuel economy savings on every trip (daily) are taken into account when calculating the net present value of the gasoline dollars saved. The second experiment evaluates the impact of different vehicle control strategies in heating up the PHEV battery (due to internal ohmic losses) for cold ambient conditions. The impact of low battery power (available to the vehicle powertrain) due to low battery and ambient temperatures has been well documented in literature. The trade-off between the benefits of heating up the battery versus heating up the internal combustion engine are evaluated, using different control strategies, and the control strategy, which provided optimum temperature rise of each component, is identified.