Eine der wichtigsten nuklearen Prozesse stellt der Neutroneneinfang dar. In der kosmischen Nukleosynthese (s-Prozess) schwerer Elemente werden Kerne mit Massenzahlen größer als die von Eisen (A = 56) produziert, welche durch Kernfusion nicht produziert werden können. Dabei fängt ein Kern ein Neutron ein, wird durch die frei werdende Bindungsenergie angeregt und kann sich anschließend unter Aussenden von Photonen (Gamma-Quanten) wieder abregen. Aus der Abregung über Gammastrahlung können Rückschlüsse auf die Struktur des aktivierten Nuklids gezogen werden. Im Rahmen dieser Arbeit werden die ausgesendeten Photonen des angeregten Elements 78Se, welches durch Neutroneneinfang an 77Se am Reaktor des Instituts Laue-Langevin in Grenoble, Frankreich produziert wurde, näher untersucht. Dazu mussten zunächst Effi zienzkalibrierung und Addback-Korrekturen vorgenommen werden. Im Anschluss konnten mit Hilfe des EXILL-Multidetektoraufbaus Koinzidenzbeziehungen mehrerer aufeinander folgender Photonen untersucht und in einem Niveauschema zusammengefasst werden. Mit Hilfe der Winkelverteilung konnten diversen Zuständen Spins zugeordnet werden. Des Weiteren wurden die Ergebnisse einer Simulation von Gammakaskaden (DEX) und eines Photonenstreuungsexperiments am Elektronenbeschleuniger ELBE des HZDR mit den in Grenoble aufgenommenen experimentellen Daten verglichen.

Within this thesis two twin experiments consisting of neutron capture and photon scattering on the neighbour isotopes 77Se / 78Se and 195Pt / 196Pt have been analysed to gain qualitative and quantitative information about the photon strength function and level density in the respective compound nuclei. For the analysis and simulation of both experimental types a new Monte Carlo simulation using a fast and efficient, extreme statistical treatment of radiative nuclear deexcitations, was developed. Furthermore the influence of fluctuations of transition widths on photon scattering were investigated and quantified. It could be shown that those lead to an enhancement of elastic scattering processes. The data analysis of both twin experiments reveals non-Lorentzian extra E1 photon strength below the neutron separation energy.

The transverse emittance is one of the most important quantities which characterize the quality of an electron source. For high quality experiments low beam emittance is required. By means of theoretical considerations and simulation calculations we have studied how the emittance of the Rossendorf superconducting radio-frequency photoelectron source (SRF gun) can be minimized. It turned out that neither a solenoid magnet nor the effect of space charge forces is needed to create a pronounced emittance minimum. The minimum appears by just adjusting the starting phase of the electron bunch with respect to the RF phase of the gun in a suitable way. Investigation of various correlations between the properties of the beam particles led to an explanation on how the minimum comes about. It is shown that the basic mechanism of minimization is the fact that the longitudinal properties of the particles (energy) are strongly influenced by the starting phase. Due to the coupling of the longitudinal and transverse degrees of freedom by the relativistic equation of motion the transverse degrees of freedom and thereby the emittance can be strongly influenced by the starting phase as well. The results obtained in this study will be applied to minimize the emittance in the commissioning phase of the SRF gun.

The Institute of Resource Ecology (IRE) is one of the eight institutes of the Helmholtz-Zentrum Dresden – Rossendorf (HZDR). The research activities are mainly integrated into the program “Nuclear Waste Management, Safety and Radiation Research (NUSAFE)” of the Helmholtz Association (HGF) and focused on the topics “Safety of Nuclear Waste Disposal” and “Safety Research for Nuclear Reactors”. Additionally, various activities have been started investigating chemical and environmental aspects of processing and recycling of strategic metals, namely rare earth elements. These activities are located in the HGF program “Energy Efficiency, Materials and Resources (EMR)”. Both programs, and therefore all work which is done at IRE, belong to the research sector “Energy” of the HGF. The research objectives are the protection of humans and the environment from hazards caused by pollutants resulting from technical processes that produce energy and raw materials. Treating technology and ecology as a unity is the major scientific challenge in assuring the safety of technical processes and gaining their public acceptance. We investigate the ecological risks exerted by radioactive and nonradioactive metals in the context of nuclear waste disposal, the production of energy in nuclear power plants, and in processes along the value chain of metalliferous raw materials. A common goal is to generate better understanding about the dominating processes essential for metal mobilization and immobilization on the molecular level by using advanced spectroscopic methods. This in turn enables us to assess the macroscopic phenomena, including models, codes, and data for predictive calculations, which determine the transport and distribution of contaminants in the environment.

Ziel des BMWi-Fördervorhabens 1501393 ist es, durch den Einsatz von Untersuchungsmethoden auf der nm-Skala einen Beitrag zur Aufklärung von Flusseffekten und von Late-Blooming-Effekten in bestrahlten RDB-Stählen zu leisten. Zur Untersuchung dieser Effekte wurde auf RDB-Stähle deutscher Reaktoren aus zwei bei der AREVA GmbH abgeschlossenen Vorhaben zurückgegriffen. Die Auswahl der Grundwerkstoffe und Schweißgüter erfolgte so, dass sich optimale Voraussetzungen für das Erreichen des Gesamtziels des Vorhabens ergeben. Die ausgewählten Untersuchungsmethoden umfassen mit der Neutronenkleinwinkelstreuung, der Atomsondentomographie und der Positronen-annihilationsspektroskopie solche Techniken, die die nm-skaligen bestrahlungsinduzierten Defekt-Fremdatom-Cluster bestmöglich und in komplementärer Weise zu detektieren und zu charakterisieren gestatten. Es wurde ein Flusseffekt auf die Größe der bestrahlungsinduzierten Fremdatomcluster, jedoch nicht auf den Volumenanteil und die mechanischen Eigenschaften gefunden. In einem Cu-armen RDB-Schweißgut wurde ein Late-Blooming-Effekt nachgewiesen, der sich in einem steilen Anstieg des Clustervolumenanteils und der Übergangstemperaturverschiebung nach einer Phase schwacher oder fehlender Zunahme niederschlägt. The BMWi project 1501393 aimed at contributing to the clarification of flux effects and late blooming effects in irradiated RPV steels by means of experimental techniques of sensitivity at the nm scale. The investigation of these effects was focussed on RPV steels, both base metal and weld of German reactors selected according to the objectives of the present project from two previous projects performed at AREVA GmbH. The complementary techniques of small-angle neutron scattering, atom probe tomography and positron annihilation spectroscopy were applied to detect and characterize the irradiation-induced nm-scale defect-solute clusters. A flux effect on the size of the irradiation-induced clusters but no flux effect on both cluster volume fraction and mechanical properties was found. For a low-Cu RPV weld, a late blooming effect was observed, which results in a steep slope of both cluster volume fraction and transition temperature shift after an initial stage of small or no change.

This past year 2014 was the year when we finally completely arrived as a “full member” in the Helmholtz Association. This is related to the successfully passed research evaluation in the framework of the Program Oriented Funding (POF), which will give us a stable and predictable funding for the next five years (2015 – 2019). This is particularly true for our large-scale user facilities, like the Ion Beam Center (IBC) and the electron accelerator ELBE with the free-electron laser. Most of our activities are assigned to the program “From Matter to Materials and Life” within the research area “Matter”, in cooperation with several other German Helmholtz Centers. Our in-house research is performed in three so-called research themes, as depicted in the schematic below. What is missing there for simplicity is a small part of our activities in the program “Nuclear Waste Management and Safety” within the research area “Energy”. Our research and facilities were well appreciated by the evaluation committee, who made the following judgement about the Ion Beam Center: “The Ion Beam Centre (IBC) of HZDR is an internationally leading ion-beam facility (with ion energies ranging from several eV to several tens of MeV). At both the national and international level it is one of the key players and is unique in its kind. The synergy between forefront research and user service has been leading to a very good publication output for both in-house research and user research. … The very broad range of beam energies, the versatility of techniques and applications – both for ion beam modification of materials and for ion-beam analysis – makes the IBC unique in its kind. … The strength of IBC is that its activities are based on a combination of forefront research and user service, which mutually interact in synergy and strengthen one another. In turn, this synergy has been leading to a very good publication output for both in-house research and user research.” In order to make our Annual Report a bit more compact, we have decided to include only four full journal papers this year. This was also triggered by the fact that our publication activities have turned out be become more diverse, in more diverse journals than in the past, and often through longer papers, which would be too long to reprint them here. However, apart from the constantly quantitatively high publication output, we succeeded to publish in excellent journals such as Nature Physics, Nano Letters and Physical Review Letters, in fields as diverse as ion beam physics, magnetism and terahertz spectroscopy. Two of our scientists, Dr. Artur Erbe and Dr. Alexej Pashkin obtained their Habilitation in 2014, both at University of Konstanz. For the first time, we are hosting an Emmy Noether Young Investigator Group funded by the Deutsche Forschungsgemeinschaft (DFG); the group works on the hot topic of magnonics and is headed by Dr. Helmut Schultheiß. Finally we would like to cordially thank all partners, friends, and organizations who supported our progress in 2014. Special thanks are due to the Executive Board of the Helmholtz-Zentrum Dresden-Rossendorf, the Minister of Science and Arts of the Free State of Saxony, and the Minister of Education and Research of the Federal Government of Germany. Numerous partners from universities, industry and research institutes all around the world contributed essentially, and play a crucial role for the further development of the institute. Last but not least, the directors would like to thank again all IIM staff for their efforts and excellent contributions in 2014.

This work presents the first demonstration of a semiconductor based plasmonic near-field superlens, utilizing highly doped GaAs to generate infrared optical images with a spatial resolution beyond the difraction limit. Being easily transferable to other semiconductor materials, the concept described in this thesis can be exploited to realize spectrally adjustable superlenses in a wide spectral range. The idea of superlensing has been introduced theoretically in 2000, followed by numerous publications including experimental studies. The effect initiated great interest in optics, since in contrast to difraction limited conventional optical microscopy it enables subwavelength resolved imaging by reconstructing the evanescent waves emerging from an object. With techniques like scanning near-field optical microscopy (SNOM) and stimulated emission depletion (STED) being already successfully established to overcome the conventional restrictions, the concept of superlensing provides a novel, different route towards high resolution. Superlensing is a resonant phenomenon, relying either on the excitation of surface plasmons in metallic systems or on phonon resonances in dielectric structures. In this respect a superlens based on doped semiconductor benefits from the potential to be controlled in its operational wavelength by shifting the plasma frequency through adjustment of the free carrier concentration. For a proof of principle demonstration, we investigate a superlens consisting of a highly n-doped GaAs layer (n = 4 x 10^18 cm-3) sandwiched between two intrinsic layers. Recording near-field images of subwavelength sized gold stripes through the trilayer structure by means of SNOM in combination with a free-electron laser, we observe both enhanced signal and improved spatial resolution at radiation wavelengths close to l = 22 µm, which is in excellent agreement with simulations based on the Drude-Lorentz model of free electrons. Here, comparative investigations of a purely intrinsic reference sample confirm that the effect is mediated by the charge carriers within the doped layer. Furthermore, slightly differently doped samples provide indications for the expected spectral shift of the resonance. According to our calculations, the wavelength range to be exploited by n-GaAs based superlenses reaches far into the terahertz region, whereas other semiconductor materials are required to explore the near infrared.

The thesis at hand addresses design, characterization and experimental testing of pulsed high-field magnets for utilization in the field of laser-plasma physics. The central task was to establish a technology platform that allows to manipulate laser-driven ion sources in a way that the accelerated ions can be used in complex application studies, e.g. radiobiological cell or tumor irradiation. Laser-driven ion acceleration in the regime of target normal sheath acceleration (TNSA) offers the unique opportunity to accelerate particles to kinetic energies of few 10MeV on the micrometer scale. The generated bunches are short, intense, show broad exponentially decaying energy spectra and high divergence. In order to efficiently use the generated particles, it is crucial to gain control over their divergence directly after their production. For most applications it additionally is favorable to reduce the energy spread of the beam. This work shows that the developed pulsed high-field magnets, so-called solenoids (cylindrical magnets), can efficiently capture, transport and focus laser-accelerated protons. The chromaticity of the magnetic lens thereby provides for energy selection. Three prototype solenoids, adapted to fit different application scenarios, and associated current pulse drivers have been developed. The magnets generate fields of several 10 T. Pulse durations are of the order of one millisecond and thus the fields can be considered as quasi-static for laser-plasma interaction processes taking place on the ps- to ns-scale. Their high field strength in combination with abandoning magnetic cores make the solenoids compact and light-weight. The presented experiments focus on a solenoid magnet designed for the capture of divergent laser-driven ion beams. They have been carried out at the 6MV tandetron accelerator and the laser acceleration source Draco of Helmholtz-Zentrum Dresden – Rossendorf as well as at the PHELIX laser of GSI Helmholtzzentrum für Schwerionenforschung, Darmstadt.

In relativistischen Schwerionenkollisionen spielen seltsame Teilchen bei der Untersuchung heißer und dichter Materie eine wichtige Rolle. Dazu wird die Produktion von Hadronen mit Strangeness-Inhalt mit Hilfe eines Transportmodells vom Boltzmann-Ühling-Uhlenbeck (BUU)-Typ numerisch behandelt. Aktuelle Messungen der HADES-Kollaboration bezüglich K+- - und phi-Spektren bilden dabei den entsprechenden experimentellen Rahmen. Darüber hinaus wird das doppelt-seltsame Hyperon Xi- unterhalb der freien NN-Produktionsschwelle analysiert. Hadronische Multiplizitäten, Transversalimpuls- und Rapiditätsspektren werden mit neuen experimentellen Ergebnissen verglichen. Weiterhin werden Massenverschiebungen im Medium, die nukleare Zustandsgleichung sowie das mittlere Feld der Nukleonen berücksichtigt. Neben der Untersuchung von Kern-Kern-Stößen bietet sich in Proton-Kern-Kollisionen ein Vergleich mit jüngsten ANKE-Daten im Hinblick auf die phi-Ausbeute an. Mit Hilfe des BUU-Transportcodes wurden Tranzparenzverhältnisse ermittelt und die Absorption von phi-Mesonen untersucht. Dabei sind sekundäre phi-Produktionskanäle, Isospin-Asymmetrie und Detektorakzeptanzen von Bedeutung und werden systematisch für verschiedene Systemgrößen analysiert. Die impulsintegrierten Boltzmann-Gleichungen dienen im Rahmen einer kinetischen Nichtgleichgewichtsdynamik der Beschreibung hochkomprimierter nuklearer Materie auf hadronischem Niveau, wie sie sowohl beim Urknall als auch bei ultra-relativistischen Schwerionenkollisionen auftritt. Diese Theorie wird am Beispiel von Antiprotonen untersucht und unter Berücksichtigung verschiedener Expansionsmodelle numerisch ausgewertet. Dabei wird die Evolution der Proton- und Antiprotondichten bis zum Ausfrieren für SPS- und RHIC-Energien mittels eines hadro-chemischen Resonanzgasmodells als möglicher Lösungsansatz des "Antiproton-Puzzles" analysiert. Diskutiert wird darüber hinaus das Verhalten baryonischer Materie und Antimaterie im frühen Universum und der adiabatische Pfad kosmischer Materie im QCD-Phasendiagramm. / Strange particles play an important role as probes of relativistic heavy-ion collisions where hot and dense matter is studied. The focus of this thesis is on the production of strange particles within a transport model of Boltzmann-Ühling-Uhlenbeck (BUU) type. Current data of the HADES Collaboration concerning K+- and phi spectra provide the appropriate experimental framework. Moreover, the double-strange hyperon Xi- is analyzed below the free NN production threshold. Hadron multiplicities, transverse-momentum and rapidity spectra are compared with recent experimental data. Further important issues are in-medium mass shifts, the nuclear equation of state as well as the mean field of nucleons. Besides the study of AA collisions a comparison with recent ANKE data regarding the phi yield in pA collisions is done. Transparency ratios are determined and primarily investigated for absorption of phi mesons by means of the BUU transport code. Thereby, secondary phi production channels, isospin asymmetry and detector acceptance are important issues. A systematic analysis is presented for different system sizes. The momentum integrated Boltzmann equations describe dense nuclear matter on a hadronic level appearing in the Big Bang as well as in little bangs, in the context of kinetic off-equilibrium dynamics. This theory is applied to antiprotons and numerically calculated under consideration of various expansion models. Here, the evolution of proton- and antiproton densities till freeze-out is analyzed for ultra-relativistic heavy-ion collisions within a hadrochemic resonance gas model acting as a possible ansatz for solving the "antiproton puzzle". Furthermore, baryonic matter and antimatter is investigated in the early universe and the adiabatic path of cosmic matter is sketched in the QCD phase diagram.

Als Graphen bezeichnet man eine einzelne freistehende Lage des Schichtkristalls Graphit. Im Gegensatz zur mechanischen Isolation von Graphit bietet die Züchtung auf Siliziumkarbid eine Methode zur großflächigen Herstellung von Graphen. Aufgrund der besonderen physikalischen Eigenschaften werden für Graphen viele verschieden Einsatzmöglichkeiten in diversen Bereichen prognostiziert. Mit seiner hohen Ladungsträgerbeweglichkeit ist Graphen besonders als Kanalmaterial für Feldeffekttransistoren (FET) interessant. Allerdings muss hierfür unter anderem ein geeignetes FET-Isolatormaterial gefunden werden. In dieser Arbeit wird eine detaillierte, theoretische Beschreibung der Graphen-FETs vorgestellt, die es erlaubt die steuerspannungsabhängige Hall-Konstante zu berechnen. Mit der dadurch möglichen Analyse können wichtige Kenngrößen, wie z. B. die Grenzflächenzustandsdichte des Materialsystems bestimmt werden. Außerdem wurden zwei Methoden zur Isolatorabscheidung auf Graphen untersucht. Siliziumnitrid, welches mittels plasmaangeregter Gasphasenabscheidung aufgetragen wurde, zeichnet sich durch seine n-dotierende Eigenschaft aus. Damit ist es vor allem für quasi-freistehendes Graphen auf Siliziumkarbid interessant. Bei der zweiten Methode handelt es sich um einen atomaren Schichtabscheidungsprozess, der ohne eine Saatschicht auskommt. An beiden Graphen- Isolator-Kombinationen wurde die neue Charakterisierung mittels der Hall-Datenanalyse angewandt.:1 Einleitung 2 Graphen 3 Methoden 4 Die Hall-Konstante von Graphen 5 Siliziumnitrid als Dielektrikum für Graphentransistoren 6 Aluminiumoxid auf epitaktischem Graphen 7 Zusammenfassung A Anhang