Using Vertical Feature Mask (VFM) data from Cloud - Aerosol Lidar Infrared Pathfinder Satellite Observations (CALIPSO), I have documented 3-dimensional (3D) structures in occurrence probabilities of aerosol over a broad region of Africa, the Atlantic, Europe, and Americas. The 3D structures illustrate the seasonal means and seasonal cycle in the zonal and meridional variability of the vertical profiles of mineral dust, biomass burning smoke, and polluted dust (external mixture of dust and smoke), and their emissions sources and transport pathways. Emission sources vary by geographical location. The persistent Saharan dust source is evident throughout the year and observed and recorded by CALIPSO 70-80% of the time over Africa. Horizontal and vertical occurrence of dust is variable in time with maximum heights and westward transport occurring in boreal summer and minimum heights and transport occurring in boreal winter. The southern African biomass burning source is also evident throughout the year, through westward transport over the Atlantic is only evident in boreal summer and fall; mixing with dust over the continent limits westward transport of pure smoke to the continent in winter and spring. Other smaller smoke and dust sources are discussed. The role of the Inter-Tropical Convergence Zone (ITCZ) in limiting the southward transport of dust and northward transport of smoke over Africa is demonstrated. Surprisingly, the highest probability of polluted dust is found in the ITCZ, even though the probabilities of dust and smoke are low. Wind trajectories reveal smoke of southern African origin is transported northward at the lower levels, but rarely penetrating through ITCZ rainband while Saharan dust is transported southward at higher levels, crossing the ITCZ frequently. This quasi-circulation of aerosol is shown to be the mixing mechanism of dust and smoke into polluted dust in the area of the ITCZ.

Thin cirrus clouds play an important radiative role in the earth's atmosphere and climate system, yet are one of the least understood components of the climate system. With the use of data from Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO), thin cirrus and thick cloud distributions in the tropics are analyzed at 121, 100, and 82 hPa. Observations obtained between December 2006 and November 2007 show that thin cirrus between 30°N and 30°S occur in close proximity to regions of intense convection and are positively correlated with low values of outgoing longwave radiation (OLR). In conjunction with the CALIPSO data, water vapor data from the Earth Observing System (EOS) Microwave Limb Sounder (MLS), OLR data provided by the NOAA/OAR/ESRL PSD, Boulder, Colorado, USA, from their Web site at http://www.cdc.noaa.gov/, and linearly interpolated NCEP reanalysis temperature data were used. These data were used to examine how thick and thin cirrus cloud fractions at 121-hPa and 100-hPa are related to relative humidity with respect to ice (RHI), temperature, and OLR. Our observations show that both RHI and convection play important roles in the development and maintenance of thick and thin cirrus clouds at the pressure levels of interest. The highest fractions of clouds are almost always seen within OLR values representative of convection and at relatively high values of RHI. However, when peaks in cloud fraction are found above the convective threshold, higher RHI values are needed than are needed when convection is responsible for the formation and maintenance of these clouds.

The veracity of a Radiometric Microwave Profiling Radiometer (MWRP) while mounted onboard a ship in the Arctic marine environment was assessed. The MWRP was validated against radiosonde data by calculating the RMS and bias for simultaneous measurements taken for temperature and absolute humidity profiles. The vertical resolution of the MWRP was calculated using the inter-level covariance method. Based on the comparisons, the MWRP provided reliable measurements of both temperature and absolute humidity while mounted on the CCGS Amundsen. Satellites CloudSat and Calipso were assessed over the Arctic marine cryosphere. Temperature and absolute humidity from the ECMWF-aux data product was compared with profiles from the ship based MWRP. The cloud base heights measured by the ceilometer and MWRP were compared to CloudSat and Calipso's GeoProf-lidar. Due to a large number of possible false detections, the constraints used by the GeoProf-lidar data product for cloud detection may need to be further refined.

The veracity of a Radiometric Microwave Profiling Radiometer (MWRP) while mounted onboard a ship in the Arctic marine environment was assessed. The MWRP was validated against radiosonde data by calculating the RMS and bias for simultaneous measurements taken for temperature and absolute humidity profiles. The vertical resolution of the MWRP was calculated using the inter-level covariance method. Based on the comparisons, the MWRP provided reliable measurements of both temperature and absolute humidity while mounted on the CCGS Amundsen. Satellites CloudSat and Calipso were assessed over the Arctic marine cryosphere. Temperature and absolute humidity from the ECMWF-aux data product was compared with profiles from the ship based MWRP. The cloud base heights measured by the ceilometer and MWRP were compared to CloudSat and Calipso's GeoProf-lidar. Due to a large number of possible false detections, the constraints used by the GeoProf-lidar data product for cloud detection may need to be further refined.

Due to the unique environmental conditions and different feedback mechanisms, the Arctic region is especially sensitive to climate changes. The influence of clouds on the radiation budget is substantial, but difficult to quantify and parameterize in models. In the framework of the PhD, elastic backscatter and depolarization lidar observations of Arctic clouds were performed during the international Arctic Study of Tropospheric Aerosol, Clouds and Radiation (ASTAR) from Svalbard in March and April 2007. Clouds were probed above the inaccessible Arctic Ocean with a combination of airborne instruments: The Airborne Mobile Aerosol Lidar (AMALi) of the Alfred Wegener Institute for Polar and Marine Research provided information on the vertical and horizontal extent of clouds along the flight track, optical properties (backscatter coefficient), and cloud thermodynamic phase. From the data obtained by the spectral albedometer (University of Mainz), the cloud phase and cloud optical thickness was deduced. Furthermore, in situ observations with the Polar Nephelometer, Cloud Particle Imager and Forward Scattering Spectrometer Probe (Laboratoire de Météorologie Physique, France) provided information on the microphysical properties, cloud particle size and shape, concentration, extinction, liquid and ice water content. In the thesis, a data set of four flights is analyzed and interpreted. The lidar observations served to detect atmospheric structures of interest, which were then probed by in situ technique. With this method, an optically subvisible ice cloud was characterized by the ensemble of instruments (10 April 2007). Radiative transfer simulations based on the lidar, radiation and in situ measurements allowed the calculation of the cloud forcing, amounting to -0.4 W m-2. This slight surface cooling is negligible on a local scale. However, thin Arctic clouds have been reported more frequently in winter time, when the clouds' effect on longwave radiation (a surface warming of 2.8 W m-2) is not balanced by the reduced shortwave radiation (surface cooling). Boundary layer mixed-phase clouds were analyzed for two days (8 and 9 April 2007). The typical structure consisting of a predominantly liquid water layer on cloud top and ice crystals below were confirmed by all instruments. The lidar observations were compared to European Centre for Medium-Range Weather Forecasts (ECMWF) meteorological analyses. A change of air masses along the flight track was evidenced in the airborne data by a small completely glaciated cloud part within the mixed-phase cloud system. This indicates that the updraft necessary for the formation of new cloud droplets at cloud top is disturbed by the mixing processes. The measurements served to quantify the shortcomings of the ECMWF model to describe mixed-phase clouds. As the partitioning of cloud condensate into liquid and ice water is done by a diagnostic equation based on temperature, the cloud structures consisting of a liquid cloud top layer and ice below could not be reproduced correctly. A small amount of liquid water was calculated for the lowest (and warmest) part of the cloud only. Further, the liquid water content was underestimated by an order of magnitude compared to in situ observations. The airborne lidar observations of 9 April 2007 were compared to space borne lidar data on board of the satellite Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO). The systems agreed about the increase of cloud top height along the same flight track. However, during the time delay of 1 h between the lidar measurements, advection and cloud processing took place, and a detailed comparison of small-scale cloud structures was not possible. A double layer cloud at an altitude of 4 km was observed with lidar at the West coast in the direct vicinity of Svalbard (14 April 2007). The cloud system consisted of two geometrically thin liquid cloud layers (each 150 m thick) with ice below each layer. While the upper one was possibly formed by orographic lifting under the influence of westerly winds, or by the vertical wind shear shown by ECMWF analyses, the lower one might be the result of evaporating precipitation out of the upper layer. The existence of ice precipitation between the two layers supports the hypothesis that humidity released from evaporating precipitation was cooled and consequently condensed as it experienced the radiative cooling from the upper layer. In summary, a unique data set characterizing tropospheric Arctic clouds was collected with lidar, in situ and radiation instruments. The joint evaluation with meteorological analyses allowed a detailed insight in cloud properties, cloud evolution processes and radiative effects. / Die Arktis mit ihren speziellen Umweltbedingungen ist besonders empfindlich gegenüber Klimaveränderungen. Dabei spielen Wolken eine große Rolle im Strahlungsgleichgewicht, die aber nur schwer genau bestimmt und in Klimamodellen dargestellt werden kann. Die Daten für die Promotionsarbeit wurden im Frühjahr 2007 bei Flugzeug-Messungen von Wolken über dem Arktischen Ozean von Spitzbergen aus erhoben. Das dafür verwendete Lidar (Licht-Radar) des Alfred-Wegener-Instituts lieferte ein höhenaufgelöstes Bild der Wolkenstrukturen und ihrer Streu-Eigenschaften, andere Messgeräte ergänzten optische sowie mikrophysikalische Eigenschaften der Wolkenteilchen (Extinktion, Größenverteilung, Form, Konzentration, Flüssigwasser- und Eisgehalt, Messgeräte vom Laboratoire de Météorologie Physique, France) und Strahlungsmessungen (Uni Mainz). Während der Messkampagne herrschte Nordwind vor. Die untersuchten Luftmassen mit Ursprung fern von menschlichen Verschmutzungsquellen war daher sehr sauber. Beim Überströmen der kalten Luft über den offenen warmen Arktischen Ozean bildeten sich in der Grenzschicht (ca. 0-1500 m Höhe) Mischphasenwolken, die aus unterkühlten Wassertröpfchen im oberen Bereich und Eis im unteren Bereich der Wolken bestehen. Mit den Flugzeug-Messungen und numerischen Simulationen des Strahlungstransports wurde der Effekt einer dünnen Eiswolke auf den Strahlungshaushalt bestimmt. Die Wolke hatte lokal eine geringe Abkühlung der Erdoberfläche zur Folge. Ähnliche Wolken würden jedoch im Winter, wenn keine Sonnenstrahlung die Arktis erreicht, durch den Treibhauseffekt eine nicht vernachlässigbare Erwärmung der Oberfläche verursachen. Die Messungen der Mischphasenwolken wurden mit einem Wettervorhersagemodell (ECMWF) verglichen. Für die ständig neue Bildung von flüssigen Wassertropfen im oberen Teil der Wolke ist das Aufsteigen von feuchten Luftpaketen nötig. Während einer Messung wurden entlang der Flugstrecke verschiedene Luftmassen durchflogen. An der Luftmassengrenze wurde eine reine Eiswolke inmitten eines Mischphasen-Systems beobachtet. Die Messungen zeigen, dass das Mischen von Luftmassen den Nachschub an feuchter Luft blockiert, was unmittelbare Auswirkungen auf die thermodynamische Phase des Wolkenwassers hat. Weiterhin wurde bestimmt, wie groß die Abweichungen der Modellrechnungen von den Messungen bezüglich Wassergehalt und der Verteilung von Flüssigwasser und Eis waren. Durch die vereinfachte Wolken-Parameterisierung wurde die typische vertikale Struktur von Mischphasenwolken im Modell nicht wiedergegeben. Die flugzeuggetragenen Lidar-Messungen vom 9. April 2007 wurden mit Lidar-Messungen an Bord des Satelliten CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations) verglichen. Die Messungen zeigten beide eine ansteigende Wolkenobergrenze entlang desselben Flugwegs. Da die Messungen jedoch nicht genau gleichzeitig durchgeführt wurden, war wegen Advektion und Prozessen in den Wolken kein genauer Vergleich der kleinskaligen Wolkenstrukturen möglich. Außerdem wurde eine doppelte Wolkenschicht in der freien Troposphäre (4 km Höhe) analysiert. Die Wolke bestand aus zwei separaten dünnen Schichten aus flüssigem Wasser (je 150 m dick) mit jeweils Eis darunter. Die untere Schicht entstand wahrscheinlich aus verdunstetem Eis-Niederschlag. Diese feuchte Schicht wurde durch die Abstrahlung der oberen Wolkenschicht gekühlt, so dass sie wieder kondensierte. Solche Wolkenformationen sind in der Arktis bisher vor allem in der Grenzschicht bekannt. Ein einzigartiger Datensatz von arktischen Wolken wurde mit einer Kombination verschiedener Flugzeug-Messgeräte erhoben. Zusammen mit meteorologischen Analysen konnten für verschiedene Fallstudien Wolkeneigenschaften, Entwicklungsprozesse und Auswirkungen auf den Strahlungshaushalt bestimmt werden.

To predict the performance of an electro-optical sensor system (EO-system) requires taking the weather situation into consideration. The possibility to use weather data from satellites instead of ground – and flight stations has been investigated. Nearly 170 satellites (about 10% of the functional satellites in orbit) were found to have atmosphere and weather monitoring. A method to select satellite data has been created based on three criteria: (1) the satellite should have a least one payload that measure a weather parameter for EO-system, (2) it should be possible to download data, free of charge, from the specified payload and (3) the satellite should cover geographical areas of interest for a potential user. The investigated performance property is the range, which is affected by many weather parameters, and focus has been on aerosols. The mean value for the aerosol extinction coefficient, for day- and nighttime conditions in December 2016, from the satellite CALIPSO’s lidar instrument Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) has been downloaded from www.earthdata.nasa.gov and implemented in a new developed application to predict the range for an EO-system. In the satellite data, from December 2016, it could be seen that the presence of aerosols, on a global scale, appears below 5 km and that the concentration of aerosols for nighttime condition is higher in local areas. For the test wavelength band of 0.9–2.5 µm, the application showed that the aerosol impact reduced the range by nearly 87%, if the EO-system was in a layer with aerosols. The application for the range prediction of EO-systems is on an early stage and need further development, especially its weather and scene parameters, to become a successful tool for a potential user in the future. / Att förutsäga prestandan hos ett elektro-optiskt sensorsystem (EO-system) kräver att man tar hänsyn till bland annat förhållandet i atmosfären. Möjligheten att använda väderdata från satelliter istället för mark- och flygstationer har undersökts. Det hittades nästan 170 satelliter (cirka 10% av de fungerande satelliterna i omloppsbana) med inriktning på atmosfär- och väderövervakning. En metod för att välja ut satellitdata har skapats som baseras på tre kriterier: (1) satelliten ska ha minst ett instrument som mäter en väderparameter för EO-system, (2) man ska, från internet, kunna ladda ner mätdata från det specifika instrumentet och (3) satelliten ska passera över ett område som är av intresse för en potentiell användare. Den prestandaegenskap som har undersökts är räckvidden, som påverkas av flera väderparametrar, där fokus har legat på inverkan från aerosoler. Medelvärdet för extinktionskoefficienten av aerosoler, för dag och natt i december 2016, från satelliten CALIPSO’s lidarinstrument Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) laddades ner från www.earthdata.nasa.gov och användes i en nyutvecklad applikation för att förutsäga räckvidden hos ett EO-system. Från satellitens mätningar i december 2016 kunde man se att förekomsten av aerosoler mestadels befann sig, globalt sett, uppdelat i olika lager under 5 km höjd och att koncentrationen av aerosoler är högre på natten i lokala områden. Applikationens beräkningar visade att förekomsten av aerosoler påverkade räckvidden för exempel våglängdsbandet 0.9–2.5 µm med en försämring upp till 87% när EO-systemet befann sig i ett skikt av aerosoler. Applikationen för att förutsäga räckvidden hos EO-system är i dess begynnelse och kräver vidareutveckling av både väder- och scenparametrar för att det ska bli ett framgångsrikt verktyg.

Aerosols show type-specific characteristics, which depend on intensive aerosol optical and microphysical properties that influence the radiation processes in the atmosphere in several ways. There are still large uncertainties in the calculation of the aerosol direct radiative effect. The classification of aerosols and the characterization of the vertical aerosol distribution is needed in order to provide more accurate information for radiative-transfer simulations. In the framework of the present thesis, the vertical and spatial distribution as well as optical properties of atmospheric aerosols over the European continent were investigated based on lidar measurements. Possibilities for an aerosol classification or so-called aerosol typing were presented and major aerosol types were specified. Former studies about the classification of aerosols were summarized and representative values for aerosol-type-dependent parameters were given. Case studies were used to demonstrate how observations of the European lidar network EARLINET from 2008 until 2010 were analyzed for aerosol layers and how model simulations and auxiliary data including the assessment of meteorological conditions were applied to determine the origin of each single aerosol layer. Thus, aerosol-type dependent parameters were evaluated and a novel method for the typing of aerosols was developed, which can be used, e.g., within algorithms of satellite data retrievals. Additionally, conversion factors were determined, which are needed for the harmonization of satellite data of present and upcoming missions. Furthermore, findings of the aerosol typing based on EARLINET data were compared to results of the aerosol classification scheme for satellite-borne lidar measurements onboard CALIPSO. It could be shown that deficient classifications of the aerosol type emerged systematically within the automated CALIPSO algorithm. Those wrong classification leads to an underestimation of the single-scattering albedo and hence to an overestimation of the warming effect of the respective aerosol layer. This overestimated warming effect has to be kept in mind for simulations of the global aerosol radiative effect based on CALIPSO data. / Die Bestimmung des direkten Strahlungsantriebs von Aerosolen ist mit großen Unsicherheiten behaftet. Inwiefern Aerosole die Strahlungsprozesse in der Atmosphäre beeinflussen ist abhängig von ihren optischen und mikrophysikalischen Eigenschaften. Zur Optimierung von Strahlungstransfersimulationen werden daher ergänzende Informationen über typspezifische Aerosoleigenschaften sowie die vertikale Aerosolverteilung benötigt. Im Rahmen der vorliegenden Arbeit wurden anhand von Lidarmessungen die vertikale und räumliche Verteilung atmosphärischer Aerosole über Europa analysiert sowie deren optische Eigenschaften ermittelt. Einleitend werden Möglichkeiten der Aerosolklassifizierung erläutert und Aerosoltypen spezifiziert, die über Europa beobachtet werden können. Vorherige Studien zur Aerosolklassifizierung sind in einer Literaturübersicht zusammengefasst. Anhand von Fallstudien wurde zunächst die Analyse von Beobachtungen des europäischen Lidarnetzwerkes EARLINET von 2008 bis 2010 auf das Vorhandensein von Aerosolschichten verdeutlicht. Die Herkunft jeder einzelnen Aerosolschicht wurde anschließend unter Verwendung von Modellrechnungen sowie weiteren Informationen bestimmt und aerosoltypspezifische Kenngrößen berechnet. Mit Hilfe dieser Kenngrößen ist es möglich, den Typ des Aerosols abzuleiten. Daraus wurde eine neuartige Methode zur Typisierung von Aerosolen entwickelt, die z.B. in Algorithmen zur Verarbeitung von Satellitendaten verwendet werden kann. Zusätzlich wurden Umrechnungsfaktoren bestimmt, die zur Zusammenführung und zum Vergleich von Daten aktueller und zukünftiger Satellitenmissionen benötigt werden. Die Ergebnisse der Aerosoltypisierung auf Basis von EARLINET-Daten wurden anschließend mit Ergebnissen der automatischen Typisierung weltraumbasierter Lidarmessungen des CALIPSO-Satelliten verglichen. Es konnte gezeigt werden, dass innerhalb des CALIPSO-Algorithmus systematisch fehlerhafte Klassifizierungen des Aerosoltyps auftreten. Diese falsche Klassifizierung führt zu einer Unterschätzung der Einfachstreualbedo und zu einer Überschätzung der erwärmenden Wirkung der betreffenden Aerosolschicht. Die überschätzte Wärmewirkung hat wiederum fehlerhafte Ergebnisse bei Strahlungstransferrechnungen, die auf CALIPSO-Daten basieren, zur Folge.

Midlevel clouds are observed globally and impact the general circulation through their influence on the radiation budget and their precipitation production. However, because midlevel clouds occur less frequently than high and low clouds they are relatively understudied. Satellite observations from the MODIS, CALIPSO, and CloudSat instruments onboard the A-Train are combined to study midlevel cloud characteristics in the Tropical Western Pacific (TWP) between January 2007 and December 2010. Characteristic cloud and microphysical properties including cloud top height (CTH), geometric thickness, optical depth, effective radius, and liquid or ice water path (LWP or IWP), and environmental properties, including temperature and specific humidity profiles, are determined for precipitating and non-precipitating midlevel clouds. In the study region, approximately 14% of all cloudy scenes are classified as midlevel clouds (4 km < CTH < 8 km). These are concentrated in areas of deeper convection associated with the Pacific warm pool, ITCZ, and SPCZ. Non-precipitating clouds dominate the region, accounting for approximately 70% of all single and two-layer midlevel clouds scenes. Midlevel clouds occur most frequently in three different scenarios: high over midlevel clouds (~65%), single-layer (~25%), and midlevel over mid- or low-level clouds (~10%). Environmental moisture appears to play a larger role than temperature in determining midlevel cloud distributions due to large variations in moisture between the different cloud scenarios. In all scenes, a trimodal distribution in CTH frequency is found within the midlevel. Two of these peaks have been identified in previous studies; however a third midlevel mode is recognized here. CTHs occur most frequently in peaks between 5-6 km, 6-6.25 km, and 6.5-7.5 km. Although the past studies have only noted two midlevel peaks, this third mode is a robust feature in this dataset. Two types of clouds dominate these peaks: non-precipitating altostratus or altocumulus-like clouds less than 1 km thick and geometrically thick precipitating cumulus congestus clouds. Environmental temperature stable layers and dry maxima are found at each one of these peak frequency heights. Again, moisture seems to play a more dominant role in determining the height of the midlevel clouds due to larger variances between the moisture gradients associated with each peak. Microphysical properties (optical depth, effective radius, and LWP or IWP) are characterized for single-layer clouds. Approximately 30% of all single-layer midlevel clouds are precipitating and these clouds tend to occur on the edges of the deep tropics. In general, precipitating clouds have greater optical depths, effective radii, and water path. This research implies that some past studies at single point locations can be representative of the broader tropics, whereas others are not.

The satellite-based cloud condensation nuclei (CCN) proxies used to quantify the aerosolcloud interactions (ACIs) are column integrated and do not guarantee the vertical co-location of aerosols and clouds. This has encouraged the use of height-resolved measurements of spaceborne lidars for ACI studies and led to advancements in lidar-based CCN retrieval algorithms. In this study, we present a comparison between the number concentration of CCN (nCCN) derived from ground-based in situ and spaceborne lidar cloud-aerosol lidar with orthogonal polarization (CALIOP) measurements. On analysing their monthly time series, we found that about 88% of CALIOP nCCN estimates remained within a factor of 1.5 of the in situ measurements. Overall, the CALIOP estimates of monthly nCCN were in good agreement with the in situ measurements with a normalized mean error of 71%, normalized mean bias of 39% and correlation coefficient of 0.68. Based on our comparison results, we point out the necessary measures that should be considered for global nCCN retrieval. Our results show the competence of CALIOP in compiling a global height- and type-resolved nCCN dataset for use in ACI studies.

The Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) mission provides unique measurements of vertical profiles of aerosols and clouds and their properties during day and night-time over all types of surfaces. This information has the potential to significantly improve our understanding of the properties and effects of aerosol and clouds. This dissertation presents the results of a comprehensive analysis of CALIPSO lidar (version 2 and version 3.01) data in conjunction with A-Train satellite and ground-based observations aimed at characterizing mineral aerosol in East Asia and other major dust sources. The specific objectives were to characterize the spatial distribution and properties of atmospheric dust in the dust source regions using new CALIOP (version 3.01) data in conjunction with satellite MODIS, OMI, and CloudSat data and ground-based meteorological and lidar data; investigate changes in the vertical distribution and properties of dust during mid- and long-range transport; perform a modeling of the optical properties of nonspherical dust particles, and assess the radiative forcing and heating/cooling rates of atmospheric dust by performing radiative transfer modeling constrained by satellite data in major dust source regions.