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The eastward winds that form each winter in the Arctic stratosphere are intermittently disrupted by planetary-scale waves propagating up from the surface in events known as stratospheric sudden warmings. It is shown here that following roughly half of these sudden warmings, the winds take as long as three months to recover, during which time the polar stratosphere evolves in a robust and predictable fashion. These extended recoveries, termed here Polar-night Jet Oscillation (PJO) events, are relevant to understanding the response of the extratropical troposphere to forcings such as solar variability and climate change. They also represent a possible source of improvement in our ability to predict weather regimes at seasonal timescales. Four projects are reported on here. In the first, the approximation of stratospheric radiative cooling by a linear relaxation is tested and found to hold well enough to diagnose effective damping rates. In the polar night, the rates found are weaker than those typically assumed by simplified modelling studies of the extratropical stratosphere and troposphere. In the second, PJO events are identified and characterized in observations, reanalyses, and a comprehensive chemistry-climate model. Their observed behaviour is reproduced well in the model. Their duration correlates with the depth in the stratosphere to which the disruption descends, and is associated with the strong suppression of further planetary wave propagation into the vortex. In the third, the response of the zonal mean winds and temperatures to the eddy-driven torques that occur during PJO events is studied. The collapse of planetary waves following the initial warming permits radiative processes to dominate. The weak radiative damping rates diagnosed in the first project are required to capture the redistribution of angular momentum responsible for the circulation anomalies. In the final project, these damping rates are imposed in a simplified model of the coupled stratosphere and troposphere. The weaker damping is found to change the warmings generated by the model to be more PJO-like in character. Planetary waves in this case collapse following the warmings, confirming the dual role of the suppression of wave driving and extended radiative timescales in determining the behaviour of PJO events.

The eastward winds that form each winter in the Arctic stratosphere are intermittently disrupted by planetary-scale waves propagating up from the surface in events known as stratospheric sudden warmings. It is shown here that following roughly half of these sudden warmings, the winds take as long as three months to recover, during which time the polar stratosphere evolves in a robust and predictable fashion. These extended recoveries, termed here Polar-night Jet Oscillation (PJO) events, are relevant to understanding the response of the extratropical troposphere to forcings such as solar variability and climate change. They also represent a possible source of improvement in our ability to predict weather regimes at seasonal timescales. Four projects are reported on here. In the first, the approximation of stratospheric radiative cooling by a linear relaxation is tested and found to hold well enough to diagnose effective damping rates. In the polar night, the rates found are weaker than those typically assumed by simplified modelling studies of the extratropical stratosphere and troposphere. In the second, PJO events are identified and characterized in observations, reanalyses, and a comprehensive chemistry-climate model. Their observed behaviour is reproduced well in the model. Their duration correlates with the depth in the stratosphere to which the disruption descends, and is associated with the strong suppression of further planetary wave propagation into the vortex. In the third, the response of the zonal mean winds and temperatures to the eddy-driven torques that occur during PJO events is studied. The collapse of planetary waves following the initial warming permits radiative processes to dominate. The weak radiative damping rates diagnosed in the first project are required to capture the redistribution of angular momentum responsible for the circulation anomalies. In the final project, these damping rates are imposed in a simplified model of the coupled stratosphere and troposphere. The weaker damping is found to change the warmings generated by the model to be more PJO-like in character. Planetary waves in this case collapse following the warmings, confirming the dual role of the suppression of wave driving and extended radiative timescales in determining the behaviour of PJO events.

This research is concerned with the self-adaptive numerical solution of the neutral particle radiation transport problem. Radiation transport is an extremely challenging computational problem since the governing equation is seven-dimensional (3 in space, 2 in direction, 1 in energy, and 1 in time) with a high degree of coupling between these variables. If not careful, this relatively large number of independent variables when discretized can potentially lead to sets of linear equations of intractable size. Though parallel computing has allowed the solution of very large problems, available computational resources will always be finite due to the fact that ever more sophisticated multiphysics models are being demanded by industry. There is thus the pressing requirement to optimize the discretizations so as to minimize the effort and maximize the accuracy. One way to achieve this goal is through adaptive phase-space refinement. Unfortunately, the quality of discretization (and its solution) is, in general, not known a priori; accurate error estimates can only be attained via the a posteriori error analysis. In particular, in the context of the finite element method, the a posteriori error analysis provides a rigorous error bound. The main difficulty in applying a well-established a posteriori error analysis and subsequent adaptive refinement in the context of radiation transport is the strong coupling between spatial and angular variables. This research attempts to address this issue within the context of the second-order, even-parity form of the transport equation discretized with the finite-element spherical harmonics method. The objective of this thesis is to develop a posteriori error analysis in a coupled space-angle framework and an efficient adaptive algorithm. Moreover, the mesh refinement strategy which is tuned for minimizing the error in the target engineering output has been developed by employing the dual argument of the problem. This numerical framework has been implemented in the general-purpose neutral particle code EVENT for assessment.

This dissertation describes a theoretical and experimental study on coherent thermal emission from thin-film multilayer structures. A novel multilayer structure consisting of a one-dimensional photonic crystal and a polar material (or a metal) is proposed as a coherent thermal-emission source. Surface electromagnetic waves can be excited at the edge of photonic crystal, enabling coherent emission characteristics (i.e., spectral- and directional-selectivity in the emissivity). A near-infrared coherent emission source is designed and fabricated using vacuum deposition and chemical vapor deposition techniques. Measurements were performed using a Fourier-transform infrared spectrometer and a laser scatterometer. The agreement between the resonance conditions obtained from experiments and the calculated dispersion relation confirms that surface waves at the photonic crystal-metal interface can be utilized to build coherent thermal-emission sources. The second part of this dissertation focuses on the energy propagation direction in near-field thermal radiation. The energy streamline method based on the Poynting vector is applied to near-field thermal radiation by incorporating the fluctuational electrodynamics, in which thermal emission is viewed as originated from random motion of electric dipoles at temperatures above absolute zero. It is shown that the Poynting vector is decoupled for each parallel wavevector component due to the randomness of thermal emission. The spectral radiative energy travels in infinite directions along curved lines; this is a fundamental characteristic of near-field thermal radiation. The findings in this dissertation are important for the design of near-field optical sensors and energy conversion devices.

The spectral and directional control of radiative properties by utilizing engineered micro/nanostructures has enormous applications in photonics, microelectronics, and energy conversion systems. The present dissertation aims at: (1) design and analysis of micro/nanostructures based on wave interference and magnetic resonance effects to achieve tunable coherent thermal emission or enhanced optical transmission; (2) microfabrication of the designed structures; and (3) development of a high-temperature emissometer to experimental demonstrate coherent thermal emission from fabricated samples at temperatures from 300 K to 800 K. Asymmetric Fabry-Perot resonant cavities were studied as a potential coherent emission source. The reflectance was measured at room temperature using a Fourier-transform infrared spectrometer, and the emittance can be indirectly obtained from Kirchhoff's law. A high-temperature emissometer was built to measure the thermal emission of fabricated samples, and the temperature effect on the emission peaks was discussed. The direct and indirect approaches were unified and a generalized Kirchhoff's law was deduced to calculate thermal emission from layered structures with nonuniform temperatures. Magnetic polaritons were identified as a mechanism for achieving extraordinary optical transmission/absorption, through the comparison between equivalent capacitor-inductor models and the rigorous coupled-wave analysis. With carefully tuned geometric parameters, the resonance frequencies can be tailored for specific applications. A coherent emission source was designed with grating structures by excitation of magnetic polaritons, and is well suitable for thermophotovoltaic applications, thanks to the spectral selectivity and directional insensitivity of magnetic polaritons. Test samples were fabricated, and coherent thermal emission was experimentally observed at room temperatures up to 800 K. The results obtained in this dissertation will facilitate the design and application of micro/nanostructures in energy-harvesting systems.

Arrays of nanotubes/rods made of appropriate materials can yield unique radiative properties, such as large absorption and optical anisotropy, with broad applications from high-efficiency emitters and absorbers for energy conversion to the polarization conversion via anisotropic responses. The objective of this dissertation is to investigate the radiative properties of arrays formed by aligned carbon nanotubes (CNTs) and silver nanorods (AgNRs). The CNT arrays used in the present study consist of multi-walled CNTs synthesized vertically on silicon substrates using thermal chemical vapor deposition. Their close-to-unity absorptance is demonstrated by measuring the directional-hemispherical reflectance in the visible and near-infrared spectral ranges using an integrating sphere. The bidirectional reflectance distribution function and angle-resolved reflectance were measured at the 635-nm wavelength. The results demonstrate that high-absorptance CNT arrays may be diffusely or specularly reflecting and have important applications in radiometry. Theoretical modeling based on the effective medium theory (EMT) and reflectivity of an anisotropic medium are developed to explain the high absorption and polarization dependence. The effective optical constants of the CNT array for both ordinary and extraordinary polarizations are quantitatively determined by fitting the angle-resolved reflectance. The AgNR arrays used in the present study were fabricated using oblique angle deposition, which results in inclined Ag nanorods that can be modeled as an effective homogenous and optically anisotropic thin film. The spectral and directional radiative properties of AgNRs grown on different substrates, including a glass slab with a silver film, and compact disc gratings, were characterized at the 635-nm and 977-nm wavelengths for different polarizations. The results are analyzed based on the EMT, rigorous coupled-wave analysis, and anisotropic thin-film optics. The results of this dissertation help gain a better understanding of radiative properties of anisotropic nanostructures for potential applications in high-efficiency energy conversion, radiometric devices, and optical systems.

No description available.

An accurate and generalized global retrieval algorithm from satellite observations is a prerequisite to understand the radiative effect of atmospheric aerosols on the climate system. Current operational aerosol retrieval algorithms are limited by the inversion schemes and suffering from the non-uniqueness problem. In order to solve these issues, a new algorithm is developed for the retrieval of non-spherical dust aerosol over land using multi-angular radiance and polarized measurements of the POLDER (POLarization and Directionality of the Earth’s Reflectances) and wide spectral high-resolution measurements of the MODIS (MODerate resolution Imaging Spectro-radiometer). As the first step to account for the non-sphericity of irregularly shaped dust aerosols in the light scattering problem, the spheroidal model is introduced. To solve the basic electromagnetic wave scattering problem by a single spheroid, we developed an algorithm, by transforming the transcendental infinite-continued-fraction-formeigen equation into a symmetric tri-diagonal linear system, for the calculation of the spheroidal angle function, radial functions of the first and second kind, as well as the corresponding first order derivatives. A database is developed subsequently to calculate the bulk scattering properties of dust aerosols for each channel of the satellite instruments. For the purpose of simulation of satellite observations, a code is developed to solve the VRTE (Vector Radiative Transfer Equation) for the coupled atmosphere-surface system using the adding-doubling technique. An alternative fast algorithm, where all the solid angle integrals are converted to summations on an icosahedral grid, is also proposed to speed-up the code. To make the model applicable to various land and ocean surfaces, a surface BRDF (Bidirectional Reflectance Distribution Function) library is embedded into the code. Considering the complimentary features of the MODIS and the POLDER, the collocated measurements of these two satellites are used in the retrieval process. To reduce the time spent on the simulation of dust aerosol scattering properties, a single-scattering property database of tri-axial ellipsoid is incorporated. In addition, atmospheric molecule correction is considered using the LBLRTM (Line-By-Line Ra- diative Transfer Model). The Levenberg-Marquardt method was employed to retrieve all the interested dust aerosol parameters and surface parameters simultaneously. As an example, dust aerosol properties retrieved over the Sahara Desert are presented.

When probing the inner structures of unresolved astrophysical sources, spectropolarimetry has proven to be a solid tool, both independent and complementary to spectral and timing analyses. In this thesis, I theoretically explore the polarization of Active Galactic Nuclei (AGN), which are powered by accretion onto supermassive black holes and often reveal significant mass outflows. Their emission is strongly anisotropic and the standard model of AGN postulates that the anisotropy is caused by a confinement of the radiation in the funnel of an obscuring body of circumnuclear dust; the radiation is thus forced to escape along the funnel where it photo-ionizes conically shaped outflows. The asymmetrical configuration explains an observational dichotomy where AGN properties are characterized according to the observer's line-of-sight. However, AGN observations differ significantly from one waveband to another and the broadband validity of the unified model has to be tested by a method that gives strong constraints on the AGN morphology. In this thesis, I subsequently investigate how morphological and composition constraints on the different substructures in thermal, radio-quiet Active Galactic Nuclei can be deduced from optical, UV and X-ray polarization properties.