La fission nucléaire est le mécanisme de séparation d'un noyau lourd en deux noyaux appelés fragments de fission. Ces fragments excités émettent des neutrons et des gammas dits prompts pour rejoindre leur état fondamental ou métastable. L'énergie libérée lors de la fission est utilisée dans les centrales nucléaires pour fournir de l'électricité. La durée de vie et le contrôle des réacteurs nucléaires dépendent entre autres des observables de fission telles que les rendements en masse des fragments, la multiplicité et l'énergie des neutrons et des gammas prompts. La première partie de cette thèse est dédiée à l'étude du processus de désexcitation des fragments de fission avec le code de simulation Monte-Carlo FIFRELIN. Ce code, constitué de plusieurs modèles nucléaires permettant de décrire les fragments, prédit les propriétés (multiplicité, énergie) des particules promptes émises lors de la désexcitation. Lors de ce travail de thèse l'influence des modèles sur les prédictions du code a été étudiée. Les modèles étudiés sont ceux définissant le moment angulaire initial, la densité de niveaux et les fonctions de force gamma des fragments. Les résultats de ces études permettent d'identifier les modèles qui influencent significativement les prédictions du code et donc, de sélectionner la combinaison des modèles reproduisant le maximum d'observables et d'améliorer la description nucléaire des fragments. Ces études sont d'abord menées sur la fission spontanée du 252Cf pour laquelle de nombreuses données expérimentales existent ce qui permet de contraindre fortement les modèles. Des études sur la fission rapide (énergie des neutrons incidents de l'ordre du MeV) de 238U et 237Np sont ensuite réalisées. Elles sont motivées, entre autres, par le développement de nouveaux concepts de réacteurs rapides, dits de quatrième génération, permettant de réduire les quantités de déchets nucléaires et d'utiliser les réserves abondantes de 238U pour fournir de l'électricité. Les données expérimentales relatives à la fission rapide sont rares. De nouveaux dispositifs expérimentaux sont actuellement en développement afin d’étudier l’évolution des différentes observables de fission sur un large domaine en énergie d’excitation. Le dispositif FALSTAFF qui fait l'objet de la deuxième partie de cette thèse est l'un d'entre eux. Dans cette seconde partie les étapes de développement, d'optimisation et de caractérisation du premier bras du dispositif expérimental FALSTAFF sont présentées. Ce spectromètre, installé auprès de l'installation NFS (Neutrons For Science), permettra d'étudier la fission rapide en cinématique directe de nombreux actinides. La détection des deux fragments de fission en coïncidence permettra de caractériser leur énergie, leurs masses (avant et après évaporation des neutrons) et leur charge. La multiplicité des neutrons émis sera alors déterminée et nous renseignera sur le partage de l'énergie d’excitation entre les fragments. Les données mesurées serviront ultérieurement de données d'entrée au code FIFRELIN. La mesure de la vitesse des deux fragments en coïncidence (méthode 2V), avec des détecteurs de temps de vol MWPC-SeD donnent accès à la masse avant évaporation. Une chambre à ionisation axiale placée après ces détecteurs permet de mesurer l'énergie cinétique et le profil de perte d'énergie des fragments, ce qui permet de déterminer respectivement la masse après évaporation (méthode EV) et la charge nucléaire des fragments.La partie expérimentale de cette thèse est dédiée au développement des programmes de simulation et d'analyse des données, à la mise en place du système d'acquisition, à la caractérisation et à l'optimisation des détecteurs. Ce dernier point concerne essentiellement l'étude des performances de la chambre à ionisation axiale. / Nuclear fission is the process in which a heavy nucleus splits into two nuclei called fission fragments. These excited fragments emit prompt neutrons and gammas to reach their ground or a metastable state. The energy released during fission is used in nuclear power plants to provide electricity. The nuclear reactor lifespan and control depend partly on fission observables such as the fragment mass yields, the neutron and gamma multiplicity and energy. The first part of this thesis is dedicated to the study of the fission fragment de-excitation process with the FIFRELIN Monte-Carlo code. This code, containing many nuclear models describing the fragments, predicts the prompt particle properties (multiplicity, energy).During this PhD work the impact of different models on the code predictions was investigated. The models which are studied are those defining the initial angular momentum, the level density and the radiative strength function of fragments. These studies identified those nuclear properties that have a significant impact on the code predictions, and as a consequence permitted selection of the model combination suited to reproduce the maximum number of fission observables, and improving our understanding about the nuclear description of fission fragments. These studies are firstly performed on the spontaneous fission of 252Cf for which numerous experimental data are available allowing constraints to be set on the models. Studies on fast fission (incident neutron with an energy around MeV) of 238U and 237Np are then performed. They are motivated partly by the development of new fast reactor concepts, called Generation IV reactors, that will reduce the quantity of nuclear waste and burn the large amount of natural uranium to provide electricity. Experimental data concerning fast fission are scarce. As a consequence new experimental setups are currently under development. They will measure fission observables over a large excitation energy domain. One of them, called FALSTAFF, is the topic of the second part of this thesis. In the second part of this PhD thesis, the different steps concerning the development, the optimization and the characterization of the first arm of the FALSTAFF setup are presented. This spectrometer, placed at the NFS facility (Neutrons For Science), will study fast fission in direct kinematic for various actinides. The detection of both fragments in coincidence will allow characterization of their energy, their masses (before and after neutron evaporation) and their nuclear charge. The neutron multiplicity will be deduced and will provide information on the energy sharing between the fragments. This data will be later used as input for the FIFRELIN code. The velocity determination of both fragments (2V method), with MWPC-SeD time-of-flight detectors, will provide pre-neutron emission fragment masses. An axial ionization chamber, placed after those detectors, will measure the kinematic energy and the energy loss profile of fragments, which will provide respectively the post-neutron emission mass (EV method) and the nuclear charge. The experimental part of this thesis is dedicated to the development of simulation and data analysis software, the configuration of the data acquisition system, the characterization and the optimization of the detectors. This last item mainly concerns the axial ionization chamber.

La production hadronique des Quarkonia est un puzzle de longue date, qui teste la capacité des physiciens des particules à décrire les interactions de couleur. Même si la structure de la chromodynamique quantique (QCD) est bien définie et inspirée par l’électrodynamique quantique (QED), les différences par rapport à cette dernière rendent très difficile la description théorique des propriétés des hadrons.Un grand nombre de modèles et de théories effectives des champs ont été proposés pour décrire la production de quarkonia lourds, mais aucune n'a réussi à prédire, de façon fiable, différentes observables. En particulier, la QCD non relativiste (NRQCD) est arrivée à décrire les sections efficaces des quarkonia au Tevatron, mais a failli pour la prédiction du degré de polarisation du J/psi. Par contre, le modèle singulet de couleur (CSM: Color Singlet Model) présentait des résultats légèrement meilleurs du coté de la polarisation mais avait des problèmes avec la normalisation et la forme des sections efficaces différentielles.Le démarrage du LHC au CERN est une excellente opportunité expérimentale pour résoudre ces problèmes. En effet le saut en énergie, par rapport au Tevatron, permet d'avoir des sections efficaces de quarks lourds bien plus élevées que dans le passé, de plus les performances excellentes des expériences LHC nous permettent de procéder à des analyses difficiles.ALICE est l’expérience du LHC dédiée à l’étude de la matière dense et chaude produite dans les collisions d’ions lourds ultra-relativistes : le plasma de quarks et de gluons (PQG). Pendant les deux premières années de prises de données, elle a montré des performances excellentes pour la détection des J/psi, aussi bien en collisions PbPb qu’en collisions pp.Dans cette thèse est présenté la mesure de la polarisation de J/psi inclusif, produits dans les collisions pp à une énergie dans le centre de masse de 7 TeV. L’analyse a été effectuée sur presque 80% de la statistique recueillie par le spectromètre à muons d’ALICE en 2010. Elle a été basée sur l’extraction de la distribution angulaire des muons provenant de la désintégration du J/psi.Les résultats obtenus par cette étude représentent la première mesure de la polarisation des quarkonia au LHC et offrent la possibilité de tester les modèles théoriques dans un régime d’énergie plus de trois fois supérieur à celui du Tevatron.Une première comparaison avec les derniers calculs théoriques est également présentée dans cette thèse. / Quarkonium hadroproduction is a long standing puzzle which tests the ability of particle physicists to describe colour interactions. Even if the structure of quantum chromodynamics (QCD) is well established and inspired to quantum electrodynamics (QED), its differences with respect to the latter make the theoretical description of hadron properties very difficult.Many models and effective field theories have been proposed in order to describe heavy quarkonia production, but none of them have been able to predict different observables in a reliable way. In particular, nonrelativistic QCD (NRQCD) succeeded in describing quarkonia cross sections at the Tevatron, but failed in predicting the degree of polarization of the J/psi. On the other hand, the color-singlet model (CSM) had slightly better results from the polarization side, but had problems with the magnitude and differential shapes of the cross sections.The startup of the LHC at CERN provides a very important experimental opportunity in solving these problems. Indeed, the big jump in energy with respect to Tevatron leads to much higher heavy-quarks cross sections than in the past and, moreover, the very good performances of the LHC experiments allow to perform delicate analysis.ALICE is the LHC experiment dedicated to the study of the dense and hot matter produce in ultrarelativistic heavy ions collisions: the quark gluon plasma (QGP). During the first two years of data taking it showed very good performance in the detection of J/psi, both in PbPb and pp collisions.In this thesis, the polarization measurement of J/psi inclusively produced in pp collisions at a center of mass energy of 7 TeV is presented. The analysis was performed on almost 80% of the statistics collected by the ALICE forward muon spectrometer during 2010. It was based on the extraction of the angular distribution of the muons coming from the J/psi decay. The results obtained with this study represent the first measurement of quarkonia polarization at the LHC and they offer the possibility to test the theoretical models in a more than three times higher energy regime with respect to Tevatron. A first comparison with recent theoretical calculations is also presented in this document.

Les sondes dures apparaissent comme l'un des sujets les plus excitant de la Physique des hautes énergies. Les mécanismes de production des quarkonia (mésons formés par l'état lié quark-antiquark charmé ou beau) dans les collisions hadroniques sont particulièrement intéressants. La suppression du J/ψ et des autres charmonia a été prédites comme l'une des signatures de la formation du Plasma de Quark et de Gluons (PQG), suppression déjà observée au SPS et au RHIC. De nombreuses études de la suppression des charmonia ont également été menées au LHC. Cependant, d'autres effets sont susceptibles de modifier la production de charmonia sans requérir la formation d'un QGP. Ces effets, inhérents aux collisions impliquant des noyaux, sont appelés effets nucléaires froids ou CNM («Cold Nuclear Matter»). Ils peuvent être étudiés dans les collisions p-Pb. Cette thèse est dédiée à l'analyse de la production de J/ψ dans les collisions p-Pb collisions à une énergie dans le centre de masse de 5.02 TeV par paire de nucléon au LHC. La production de J/ψ est étudiée en fonction de l'impulsion transverse, de la rapidité et de l'activité de la collision. Ces résultats apportent une contribution significative dans la compréhension des effets CNM et dans l'établissement d'une référence pour l'interprétation de la production de J/ψ dans les collisions Pb-Pb. / Hard probes represent one of the hottest topics of the modern high energy physics. The production mechanism of quarkonia (mesons composed of a charm or beauty quark and its antiquark) in hadronic collisions is of particular interest. The suppression of J/ψ and other charmonium states was predicted as one of the first signatures of the Quark Gluon Plasma (QGP) formation and was seen at RHIC and SPS. It was also studied at the LHC in Pb-Pb collisions. However, other effects can affect the charmonium production in Pb-Pb collisions without the presence of the QGP. These effects are inherent to the use of nuclei and are called «Cold Nuclear Matter» (CNM) effects. They can be studied in p-Pb collisions. This thesis is dedicated to the studies of J/ψ production in p-Pb collisions at the LHC at a center of mass energy of 5.02 TeV per nucleon pair. J/ψ production is studied as a function of transverse momentum, rapidity and event activity. These results represent a significant step to better understanding of the CNM effects and to the establishment of a reference for J/ψ production in Pb-Pb collisions.

This thesis describes the development of control applications for the deposition machine and mass spectrometer. Thesis describes operation principles of both devices and their hardware specifications. Thesis also describes the design of developed applications. Functionality was tested on series of real measurements.

Despite the decades of intensive research, nucleic acids represent still a permanent object of structural studies. Within the framework of the doctoral work, the apparatus for measurement of UV excited resonance Raman spectra (UV RRS) was built up and optimized. A realistic and complex interpretation table was prepared based on analysis of published data and extensive series of UV RRS measurements on NA model structures, mononucleotides, and polynucleotides. The established methodology was verified when applied in several structural studies of nucleic acids, mainly the study of the influence of magnesium ions on the equilibrium between duplexes and triplexes formed by PolyA and PolyU homopolynucleotides, a study of temperature-induced structural changes in DNA double helix and DNA hairpin, and investigation of slow structural transitions of guanine quadruplexes induced by the presence of potassium ions. The results of the test measurements and the above-mentioned studies have shown that the created methodology for studying UV RRS of nucleic acids brings most of the expected benefits of the resonance excitation: the possibility of Raman scattering measurements at the same concentrations as in the case of UV absorption, high sensitivity to fine temperature-induced structural changes and good interpretability...

The work deals with the design, control, precision and dynamics of linear piezoelectric motors from PiezoMotor Uppsala AB. The aim of this thesis is to evaluate the applicability of the loaned engine in a mass spectrometer. In introduction‘s section of this work is discussing the design principles of functionality, materials used, procedure and types of piezoelectric motors. It focuses the choice of hardware and design of mechanical assemblies, which could replace the current mechanism with electromagnetic motors. Then we designed and fabricated a test report with hired piezoelectric motor. In NI LabView development environment is created test application for control and measurement. The final section is devoted to a summary of the positive and negative features of the hired piezoelectric motor and evaluation of accuracy and dynamics.

No description available.

The recent development of extreme ultraviolet (EUV) sources has increased the need for diagnostic tools, and has opened up a previously limited portion of the spectrum. With ultrafast laser systems and spectroscopy moving into shorter timescales and wavelengths, the need for nanosecond scale imaging of EUV is increasing. EUV’s high absorption has limited the number of imaging options due to the many atomic resonances in this spectrum. Currently EUV is imaged with photodiodes and X-ray CCDs. However photodiodes are limited in that they can only resolve intensity with respect to time and X-ray CCDs are limited to temporal resolution in the microsecond range. This work shows a novel approach to imaging EUV light over a nanosecond time scale, by using an EUV scintillator to convert EUV to visible light imaged by a conventional streak camera. A laser produced plasma, using a mass-limited tin based target, provided EUV light which was imaged by a grazing incidence flat field spectrometer onto a Ce:YAG scintillator. The EUV spectrum (5 nm-20 nm) provided by the spectrometer is filter by a zirconium filter and then converted by the scintillator to visible light (550 nm) which can then be imaged with conventional optics. Visible light was imaged by an electron image tube based streak camera. The streak camera converts the visible light image to an electron image using a photocathode, and sweeps the image across a recording medium. The streak camera also provides amplification and gating of the image by the means of a micro channel plate, within the image tube, to compensate for low EUV intensities. The system provides 42 ns streaked images of light with a iii temporal resolution of 440 ps at a repetition rate of 1 Hz. Upon calibration the EUV streak camera developed in this work will be used in future EUV development.

The neutron plays a central role in numerous fields of physics, a fact that entails a need for methods of measuring neutron energy spectra. In this project, a technique for neutron spectrometry through measurements of neutron-induced radioactivity in activation detectors was developed and tested. The developed technique involves irradiating element samples with neutrons, measuring activation products with a gamma spectrometer, and then performing a neutron spectrum unfolding procedure. The elements indium, iron, magnesium, aluminium, zinc, titanium, and copper were used as activation detectors and irradiated with neutrons from an americium-beryllium (AmBe) neutron source. Subsequent gamma spectrometry was performed with the UGGLA high-purity germanium detector setup at Uppsala University. The GRAVEL unfolding algorithm was implemented in MATLAB and used to unfold neutron spectra based on an initial spectrum guess. The unfolded neutron spectrum agrees well with the expected AmBe spectrum, though some difference between the spectra is attributed to neutron scattering in the irradiation environment. A possible ability to find approximate neutron spectra from inaccurate initial guesses is found, but additional work is needed to understand better how the initial guess affects the result for different neutron sources. Because activation detectors do not require electrical power when measuring neutrons, can be made sensitive to a wide range of neutron energies, and do not detect other types of radiation, future applications could find the developed neutron spectrometry method practical.

In the atomic energy pile at Chalk River, heavy water (deuterium oxide, D2O) is to be used as a moderator. Early in 1944, it became evident that frequent determinations of the isotopic composition of D2O samples would be required. For this purpose, there was obtained from the American authorities a mass spectrometer specially designed for routine hydrogen isotope analysis. This instrument was assembled and put into operation at McMaster in the summer of 1944. During the course of subsequent work, two other deuterium mass spectrometers were built in this laboratory, following the design of the instrument sent from the United States; one of these has now been installed at the plant site, and a second is to follow at an early date. The studies reported below involved the determination of operating conditions, the measurement of grid leaks, of the order of 10^10 ohms, and the investigation of further applications of the deuterium mass spectrometer. / Thesis / Master of Science (MSc)